Shu-Xing Wang, Carsten Brandau, Stephan Fritzsche, Sebastian Fuchs, Zoltán Harman, Christophor Kozhuharov, Alfred Müller, Markus Steck, Stefan Schippers
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引用次数: 0
摘要
在重离子存储环上对类氢氙离子的 KLL 介电重组(DR)共振进行了电子-离子碰撞光谱分析,其分辨能力可与高电荷离子内壳跃迁的 X 射线光谱分析相媲美。(KL_{1/2}L_{1/2}\)、\(KL_{1/2}L_{3/2}\)和\(KL_{3/2}L_{3/2}\)共振组甚至它们的部分精细结构都被单独解析出来。共振强度是在绝对尺度上测量的,并与多构型狄拉克-福克(MCDF)计算的结果进行了比较。当考虑到 QED 对共振能量的影响和 Breit 相互作用时,这些结果与实验结果非常吻合。正如在类氢铀的 DR 中已经发现的那样(Bernhardt 等人,Phys Rev A 83:020701(R), 2011),这种相互作用对于 \(KL_{1/2}L_{1/2}\) 共振组尤其强烈。对于铀(^{91+}\),它使\(KL_{1/2}L_{1/2}\) DR共振强度增加了40%。对于 Xe\(^{53+}\) 来说,这种增加达到了 25%,证实了布雷特相互作用的影响随着核电荷的增加而增加的预测。一个全面的附录讨论了相对论电子和离子相互作用束的实验和理论合并束重组率系数的推导。
Breit interaction in dielectronic recombination of hydrogenlike xenon ions: storage-ring experiment and theory
Electron-ion collision spectroscopy of the KLL dielectronic recombination (DR) resonances of hydrogenlike xenon ions was performed at a heavy-ion storage ring with a resolving power that is competitive with x-ray spectroscopy of inner-shell transitions in highly charged ions. The \(KL_{1/2}L_{1/2}\), \(KL_{1/2}L_{3/2}\), and \(KL_{3/2}L_{3/2}\) resonance groups and even parts of their fine structure are individually resolved. The resonance strengths were measured on an absolute scale and compared with results from multi-configuration Dirac–Fock (MCDF) calculations. These are in excellent agreement with the experimental findings when QED effects on the resonance energies and the Breit interaction are considered. As already found for DR of hydrogenlike uranium (Bernhardt et al. in Phys Rev A 83:020701(R), 2011), this interaction is particularly strong for the \(KL_{1/2}L_{1/2}\) resonance group. For U\(^{91+}\), it increases the \(KL_{1/2}L_{1/2}\) DR resonance strength by 40%. For Xe\(^{53+}\), the increase is found to amount to 25%, confirming the prediction that the influence of the Breit interaction grows with increasing nuclear charge. A comprehensive appendix treats the derivation of experimental and theoretical merged-beams recombination rate coefficients for interacting beams of relativistic electrons and ions.
期刊介绍:
The European Physical Journal D (EPJ D) presents new and original research results in:
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The range of topics covered in these areas is extensive, from Molecular Interaction and Reactivity to Spectroscopy and Thermodynamics of Clusters, from Atomic Optics to Bose-Einstein Condensation to Femtochemistry.