用于多用途运动监测的超拉伸、坚韧和高导电离子凝胶

IF 11.3 1区 化学 Q1 CHEMISTRY, PHYSICAL
Min Su Kim, Jeong Hui Kim, Hye-young Yoo, Dal-Seong Yoon, Dong Hyun Park, Chae Yoon Lee, Su Jung Kim, Seung-Bok Choi*, Kihyon Hong* and Keun Hyung Lee*, 
{"title":"用于多用途运动监测的超拉伸、坚韧和高导电离子凝胶","authors":"Min Su Kim,&nbsp;Jeong Hui Kim,&nbsp;Hye-young Yoo,&nbsp;Dal-Seong Yoon,&nbsp;Dong Hyun Park,&nbsp;Chae Yoon Lee,&nbsp;Su Jung Kim,&nbsp;Seung-Bok Choi*,&nbsp;Kihyon Hong* and Keun Hyung Lee*,&nbsp;","doi":"10.1021/acsmaterialslett.4c0142510.1021/acsmaterialslett.4c01425","DOIUrl":null,"url":null,"abstract":"<p >Stretchable strain sensors have attracted considerable interest for electronic and electrochemical applications, but improving their sensitivity, stretchability, toughness, conductivity, and stability remains a challenge. While ionic conductor-based sensors offer high stretchability (&gt;100%), achieving both robustness and high conductivity is difficult. In this study, ultrastretchable, tough, and highly conductive nonvolatile polymer electrolytes, referred to as ionogels, were devised using a solvent-exchange method. Compared to other gel-type materials, such as organogels and hydrogels, the ionogels exhibit outstanding elasticity (&gt;1000% strain at break), toughness (∼100 MJ m<sup>–3</sup>), and ionic conductivity of (∼20.5 mS cm<sup>–1</sup>). These ionogels were successfully applied to sensing devices, and the resulting sensors exhibited excellent linearity, sensitivity, repeatability, and operational durability. Furthermore, the sensors accurately detected the movements of various vehicle parts, including the suspension damper, door hinge, and seat coil, indicating the potential of mechanically tough ionogels for multipurpose sensing systems.</p>","PeriodicalId":9,"journal":{"name":"ACS Catalysis ","volume":null,"pages":null},"PeriodicalIF":11.3000,"publicationDate":"2024-09-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Ultrastretchable, Tough, and Highly Conductive Ionogels for Multipurpose Motion Monitoring\",\"authors\":\"Min Su Kim,&nbsp;Jeong Hui Kim,&nbsp;Hye-young Yoo,&nbsp;Dal-Seong Yoon,&nbsp;Dong Hyun Park,&nbsp;Chae Yoon Lee,&nbsp;Su Jung Kim,&nbsp;Seung-Bok Choi*,&nbsp;Kihyon Hong* and Keun Hyung Lee*,&nbsp;\",\"doi\":\"10.1021/acsmaterialslett.4c0142510.1021/acsmaterialslett.4c01425\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Stretchable strain sensors have attracted considerable interest for electronic and electrochemical applications, but improving their sensitivity, stretchability, toughness, conductivity, and stability remains a challenge. While ionic conductor-based sensors offer high stretchability (&gt;100%), achieving both robustness and high conductivity is difficult. In this study, ultrastretchable, tough, and highly conductive nonvolatile polymer electrolytes, referred to as ionogels, were devised using a solvent-exchange method. Compared to other gel-type materials, such as organogels and hydrogels, the ionogels exhibit outstanding elasticity (&gt;1000% strain at break), toughness (∼100 MJ m<sup>–3</sup>), and ionic conductivity of (∼20.5 mS cm<sup>–1</sup>). These ionogels were successfully applied to sensing devices, and the resulting sensors exhibited excellent linearity, sensitivity, repeatability, and operational durability. Furthermore, the sensors accurately detected the movements of various vehicle parts, including the suspension damper, door hinge, and seat coil, indicating the potential of mechanically tough ionogels for multipurpose sensing systems.</p>\",\"PeriodicalId\":9,\"journal\":{\"name\":\"ACS Catalysis \",\"volume\":null,\"pages\":null},\"PeriodicalIF\":11.3000,\"publicationDate\":\"2024-09-09\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Catalysis \",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acsmaterialslett.4c01425\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Catalysis ","FirstCategoryId":"92","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsmaterialslett.4c01425","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0

摘要

可拉伸应变传感器在电子和电化学应用领域引起了广泛关注,但提高其灵敏度、可拉伸性、韧性、导电性和稳定性仍是一项挑战。虽然基于离子导体的传感器具有很高的可拉伸性(100%),但要同时实现坚固性和高导电性却很困难。本研究采用溶剂交换法设计出了超伸展性、韧性和高导电性的非挥发性聚合物电解质(称为离子凝胶)。与有机凝胶和水凝胶等其他凝胶型材料相比,离子凝胶具有出色的弹性(断裂应变达 1000%)、韧性(100 MJ m-3)和离子导电性(20.5 mS cm-1)。这些离子凝胶被成功应用于传感装置,所制成的传感器具有出色的线性度、灵敏度、可重复性和操作耐久性。此外,这些传感器还能准确检测到悬挂减震器、车门铰链和座椅线圈等各种汽车部件的运动,这表明机械韧性离子凝胶在多用途传感系统中的应用潜力。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Ultrastretchable, Tough, and Highly Conductive Ionogels for Multipurpose Motion Monitoring

Ultrastretchable, Tough, and Highly Conductive Ionogels for Multipurpose Motion Monitoring

Stretchable strain sensors have attracted considerable interest for electronic and electrochemical applications, but improving their sensitivity, stretchability, toughness, conductivity, and stability remains a challenge. While ionic conductor-based sensors offer high stretchability (>100%), achieving both robustness and high conductivity is difficult. In this study, ultrastretchable, tough, and highly conductive nonvolatile polymer electrolytes, referred to as ionogels, were devised using a solvent-exchange method. Compared to other gel-type materials, such as organogels and hydrogels, the ionogels exhibit outstanding elasticity (>1000% strain at break), toughness (∼100 MJ m–3), and ionic conductivity of (∼20.5 mS cm–1). These ionogels were successfully applied to sensing devices, and the resulting sensors exhibited excellent linearity, sensitivity, repeatability, and operational durability. Furthermore, the sensors accurately detected the movements of various vehicle parts, including the suspension damper, door hinge, and seat coil, indicating the potential of mechanically tough ionogels for multipurpose sensing systems.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
ACS Catalysis
ACS Catalysis CHEMISTRY, PHYSICAL-
CiteScore
20.80
自引率
6.20%
发文量
1253
审稿时长
1.5 months
期刊介绍: ACS Catalysis is an esteemed journal that publishes original research in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. It offers broad coverage across diverse areas such as life sciences, organometallics and synthesis, photochemistry and electrochemistry, drug discovery and synthesis, materials science, environmental protection, polymer discovery and synthesis, and energy and fuels. The scope of the journal is to showcase innovative work in various aspects of catalysis. This includes new reactions and novel synthetic approaches utilizing known catalysts, the discovery or modification of new catalysts, elucidation of catalytic mechanisms through cutting-edge investigations, practical enhancements of existing processes, as well as conceptual advances in the field. Contributions to ACS Catalysis can encompass both experimental and theoretical research focused on catalytic molecules, macromolecules, and materials that exhibit catalytic turnover.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信