{"title":"通过岩石圈的通道化熔融迁移过程中的钕同位素平衡:使用理想化数值模型的可行性研究","authors":"Mousumi Roy, G. Lang Farmer, Kellen Malone","doi":"10.1029/2024GC011593","DOIUrl":null,"url":null,"abstract":"<p>This study is motivated by the observed variability in trace element isotopic and chemical compositions of primitive (Si<span></span><math>\n <semantics>\n <mrow>\n <msub>\n <mi>O</mi>\n <mn>2</mn>\n </msub>\n <mo><</mo>\n </mrow>\n <annotation> ${\\mathrm{O}}_{2}< $</annotation>\n </semantics></math>52 wt %) basalts in southwest North America (SWNA) during the Cenozoic transition from subduction to extension. Specifically, we focus on processes that may explain the enigmatic observation that in some localities, basalts with low Ta/Th, consistent with parental melts in a subduction setting, have <span></span><math>\n <semantics>\n <mrow>\n <msub>\n <mi>ε</mi>\n <mrow>\n <mi>N</mi>\n <mi>d</mi>\n </mrow>\n </msub>\n </mrow>\n <annotation> ${\\varepsilon }_{Nd}$</annotation>\n </semantics></math> signatures consistent with continental lithospheric mantle (CLM). In locations with the oldest CLM (Proterozoic and Archean), Cenozoic basalts with low Ta/Th have <span></span><math>\n <semantics>\n <mrow>\n <msub>\n <mi>ε</mi>\n <mrow>\n <mi>N</mi>\n <mi>d</mi>\n </mrow>\n </msub>\n </mrow>\n <annotation> ${\\varepsilon }_{Nd}$</annotation>\n </semantics></math> well below zero. We model channelized magma transport through the CLM using simple 1D transport models to explore the extent to which diffusive and reactive mass exchange can modify Nd isotopic compositions via open system melt-wallrock interactions. For geologically reasonable channel spacings and volume fractions, we quantify the reactive assimilation rates required for incoming melt with a different <span></span><math>\n <semantics>\n <mrow>\n <msub>\n <mi>ε</mi>\n <mrow>\n <mi>N</mi>\n <mi>d</mi>\n </mrow>\n </msub>\n </mrow>\n <annotation> ${\\varepsilon }_{Nd}$</annotation>\n </semantics></math> than the wall-rock to undergo a substantial isotopic shift during <span></span><math>\n <semantics>\n <mrow>\n <mo>≈</mo>\n </mrow>\n <annotation> ${\\approx} $</annotation>\n </semantics></math>10 km channelized melt transport. In the presence of grain boundaries, enhanced diffusion between melt-rich channels and melt-poor surrounding rock contributes to isotopic equilibration, however this effect is not enough to explain observations; our models suggest a significant contribution from reactive assimilation of wall-rock. Additionally our models support the idea that the observed covariability in Ta/Th and <span></span><math>\n <semantics>\n <mrow>\n <msub>\n <mi>ε</mi>\n <mrow>\n <mi>N</mi>\n <mi>d</mi>\n </mrow>\n </msub>\n </mrow>\n <annotation> ${\\varepsilon }_{Nd}$</annotation>\n </semantics></math> in Cenozoic basalts cannot be attributed to transport alone and must also reflect the transition from subduction-related to extension-related parental melts in SWNA.</p>","PeriodicalId":50422,"journal":{"name":"Geochemistry Geophysics Geosystems","volume":"25 10","pages":""},"PeriodicalIF":2.9000,"publicationDate":"2024-09-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1029/2024GC011593","citationCount":"0","resultStr":"{\"title\":\"Nd Isotopic Equilibration During Channelized Melt Transport Through the Lithosphere: A Feasibility Study Using Idealized Numerical Models\",\"authors\":\"Mousumi Roy, G. 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In the presence of grain boundaries, enhanced diffusion between melt-rich channels and melt-poor surrounding rock contributes to isotopic equilibration, however this effect is not enough to explain observations; our models suggest a significant contribution from reactive assimilation of wall-rock. Additionally our models support the idea that the observed covariability in Ta/Th and <span></span><math>\\n <semantics>\\n <mrow>\\n <msub>\\n <mi>ε</mi>\\n <mrow>\\n <mi>N</mi>\\n <mi>d</mi>\\n </mrow>\\n </msub>\\n </mrow>\\n <annotation> ${\\\\varepsilon }_{Nd}$</annotation>\\n </semantics></math> in Cenozoic basalts cannot be attributed to transport alone and must also reflect the transition from subduction-related to extension-related parental melts in SWNA.</p>\",\"PeriodicalId\":50422,\"journal\":{\"name\":\"Geochemistry Geophysics Geosystems\",\"volume\":\"25 10\",\"pages\":\"\"},\"PeriodicalIF\":2.9000,\"publicationDate\":\"2024-09-30\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://onlinelibrary.wiley.com/doi/epdf/10.1029/2024GC011593\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Geochemistry Geophysics Geosystems\",\"FirstCategoryId\":\"89\",\"ListUrlMain\":\"https://onlinelibrary.wiley.com/doi/10.1029/2024GC011593\",\"RegionNum\":2,\"RegionCategory\":\"地球科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"GEOCHEMISTRY & GEOPHYSICS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Geochemistry Geophysics Geosystems","FirstCategoryId":"89","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1029/2024GC011593","RegionNum":2,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"GEOCHEMISTRY & GEOPHYSICS","Score":null,"Total":0}
引用次数: 0
摘要
在新生代从俯冲向伸展的转变过程中,北美西南部(SWNA)的原始玄武岩(Si O 2 < ${\mathrm{O}}_{2}< $ 52 wt %)的痕量元素同位素和化学成分发生了变化。具体来说,我们重点研究了一些过程,这些过程可能解释了这样一个令人费解的现象:在一些地方,Ta/Th含量低的玄武岩与俯冲环境中的母熔体一致,而ε N d ${\varepsilon }_{Nd}$特征与大陆岩石圈地幔(CLM)一致。在具有最古老CLM的地区(新元古代和奥陶纪),具有低Ta/Th的新生代玄武岩的ε N d ${\varepsilon }_{Nd}$远低于零。我们使用简单的一维输运模型来模拟岩浆在CLM中的通道化输运,以探索扩散和反应质量交换通过开放系统熔体-壁岩相互作用改变Nd同位素组成的程度。对于地质上合理的通道间距和体积分数,我们量化了与壁岩不同的ε N d ${\varepsilon }_{Nd}$流入熔体在≈ $\{approx} $ 10 km通道化熔体运移过程中发生重大同位素转变所需的反应同化率。在存在晶界的情况下,富熔体通道与贫熔体围岩之间的扩散增强有助于同位素平衡,但这种效应不足以解释观测结果;我们的模型表明,壁岩的反应性同化也有很大的贡献。此外,我们的模型还支持这样一种观点,即在新生代玄武岩中观测到的Ta/Th和ε N d ${varepsilon }_{Nd}$的共变性不能仅仅归因于运移,还必须反映出西南地区与俯冲有关的母熔体向与延伸有关的母熔体的转变。
Nd Isotopic Equilibration During Channelized Melt Transport Through the Lithosphere: A Feasibility Study Using Idealized Numerical Models
This study is motivated by the observed variability in trace element isotopic and chemical compositions of primitive (Si52 wt %) basalts in southwest North America (SWNA) during the Cenozoic transition from subduction to extension. Specifically, we focus on processes that may explain the enigmatic observation that in some localities, basalts with low Ta/Th, consistent with parental melts in a subduction setting, have signatures consistent with continental lithospheric mantle (CLM). In locations with the oldest CLM (Proterozoic and Archean), Cenozoic basalts with low Ta/Th have well below zero. We model channelized magma transport through the CLM using simple 1D transport models to explore the extent to which diffusive and reactive mass exchange can modify Nd isotopic compositions via open system melt-wallrock interactions. For geologically reasonable channel spacings and volume fractions, we quantify the reactive assimilation rates required for incoming melt with a different than the wall-rock to undergo a substantial isotopic shift during 10 km channelized melt transport. In the presence of grain boundaries, enhanced diffusion between melt-rich channels and melt-poor surrounding rock contributes to isotopic equilibration, however this effect is not enough to explain observations; our models suggest a significant contribution from reactive assimilation of wall-rock. Additionally our models support the idea that the observed covariability in Ta/Th and in Cenozoic basalts cannot be attributed to transport alone and must also reflect the transition from subduction-related to extension-related parental melts in SWNA.
期刊介绍:
Geochemistry, Geophysics, Geosystems (G3) publishes research papers on Earth and planetary processes with a focus on understanding the Earth as a system. Observational, experimental, and theoretical investigations of the solid Earth, hydrosphere, atmosphere, biosphere, and solar system at all spatial and temporal scales are welcome. Articles should be of broad interest, and interdisciplinary approaches are encouraged.
Areas of interest for this peer-reviewed journal include, but are not limited to:
The physics and chemistry of the Earth, including its structure, composition, physical properties, dynamics, and evolution
Principles and applications of geochemical proxies to studies of Earth history
The physical properties, composition, and temporal evolution of the Earth''s major reservoirs and the coupling between them
The dynamics of geochemical and biogeochemical cycles at all spatial and temporal scales
Physical and cosmochemical constraints on the composition, origin, and evolution of the Earth and other terrestrial planets
The chemistry and physics of solar system materials that are relevant to the formation, evolution, and current state of the Earth and the planets
Advances in modeling, observation, and experimentation that are of widespread interest in the geosciences.