在高级氧化工艺中活化过乙酸的碳基材料的进展:综述

IF 7.7 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES
Chenghuan Qiao , Wenrui Jia , Jingrui Tang , Chuchu Chen , Yaohua Wu , Yongqi Liang , Juanshan Du , Qinglian Wu , Xiaochi Feng , Huazhe Wang , Wan-Qian Guo
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引用次数: 0

摘要

近年来,基于过乙酸(PAA)的高级氧化工艺(AOPs)因其快速响应时间和环境友好性而在水处理领域备受关注。各种碳基材料(包括各种类型、结构和改性形式的碳材料)对 PAA 系统的活化在处理新出现的环境污染物方面发挥着至关重要的作用。然而,碳基材料在活化 PAA 过程中的结构特征和结构-活性关系错综复杂,降解途径和主要活性物种也表现出多样性。因此,当务之急是通过资源整合和逻辑分类,阐明碳基材料/PAA 系统的发展过程,从而为今后的研究指明潜在的途径。本文全面回顾了 PAA 体系中碳基材料的结构特征和作用机理,同时还分析了该体系中掺杂杂原子的碳基材料的发展、性能和活化机理。总之,本研究有效地梳理了环境水污染综合治理这一突出研究方向的相关资源,从而阐明了其内在逻辑和思维过程。因此,它为今后涉及碳基材料/PAA 系统的研究和应用奠定了坚实的理论基础。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Advances of carbon-based materials for activating peracetic acid in advanced oxidation processes: A review

Advances of carbon-based materials for activating peracetic acid in advanced oxidation processes: A review
In recent years, the peracetic acid (PAA)-based advanced oxidation process (AOPs) has garnered significant attention in the field of water treatment due to rapid response time and environmentally-friendliness. The activation of PAA systems by diverse carbon-based materials plays a crucial role in addressing emerging environmental contaminants, including various types, structures, and modified forms of carbon materials. However, the structural characteristics and structure-activity relationship of carbon-based materials in the activation of PAA are intricate, while the degradation pathways and dominant active species exhibit diversity. Therefore, it is imperative to elucidate the developmental process of the carbon-based materials/PAA system through resource integration and logical categorization, thereby indicating potential avenues for future research. The present paper comprehensively reviews the structural characteristics and action mechanism of carbon-based materials in PAA system, while also analyzing the development, properties, and activation mechanism of heteroatom-doped carbon-based materials in this system. In conclusion, this study has effectively organized the resources pertaining to prominent research direction of comprehensive remediation of environmental water pollution, thereby elucidating the underlying logic and thought process. Consequently, it establishes robust theoretical foundation for future investigations and applications involving carbon-based materials/PAA system.
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来源期刊
Environmental Research
Environmental Research 环境科学-公共卫生、环境卫生与职业卫生
CiteScore
12.60
自引率
8.40%
发文量
2480
审稿时长
4.7 months
期刊介绍: The Environmental Research journal presents a broad range of interdisciplinary research, focused on addressing worldwide environmental concerns and featuring innovative findings. Our publication strives to explore relevant anthropogenic issues across various environmental sectors, showcasing practical applications in real-life settings.
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