用于电催化氮转化反应的铂铜合金纳米树枝状化合物的可见光驱动合成（Adv. Sustainable Syst.）

IF 6.5 3区材料科学 Q2 GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY

Advanced Sustainable Systems Pub Date : 2024-09-24 DOI:10.1002/adsu.202470034

Guoqiang Wang, Chuanjun Wang, Xin Zhao, Shenjie Liu, Geoffrey I. N. Waterhouse, Yining Zhang, Xiaoqing Lv, Chenyang Wang, Xiaojun Lv, Jing Xu

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引用次数: 0

摘要

PtCu 合金纳米树突在编号为 2400272 的文章中，Geoffrey I. N. Waterhouse、Jing Xu 及其合作者介绍了一种以荧光素为出射态光敏剂的水溶液可见光驱动系统，该系统在光照射下还原 Pt4+ 和 Cu2+ 盐生成 PtCu 合金纳米树突，从而原位催化制氢。收集纯净的 PtCu 合金纳米枝晶并将其用作电催化剂，该催化剂在氮氧化成硝酸盐和亚硝酸盐/硝酸盐还原成氨的过程中表现出令人印象深刻的双功能电催化活性。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

Visible Light-Driven Synthesis of PtCu Alloy Nanodendrites for Electrocatalytic Nitrogen-Conversion Reactions (Adv. Sustainable Syst. 9/2024)

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Visible Light-Driven Synthesis of PtCu Alloy Nanodendrites for Electrocatalytic Nitrogen-Conversion Reactions (Adv. Sustainable Syst. 9/2024)

PtCu Alloy Nanodendrites

In article number 2400272, Geoffrey I. N. Waterhouse, Jing Xu, and co-workers present an aqueous visible-light-driven system with fluorescein as the exited state photosensitizer, which upon light irradiation reduces Pt⁴⁺ and Cu²⁺ salts to generate PtCu alloy nanodendrites, resulting in in situ catalyzing hydrogen production. The PtCu alloy nanodendrites are collected in pure and used as the electrocatalyst, which exhibits impressive bifunctional electrocatalytic activity for nitrogen oxidation to nitrate and nitrite/nitrate reduction to ammonia.

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来源期刊

Advanced Sustainable Systems Environmental Science-General Environmental Science

CiteScore

10.80

自引率

4.20%

发文量

186

期刊介绍： Advanced Sustainable Systems, a part of the esteemed Advanced portfolio, serves as an interdisciplinary sustainability science journal. It focuses on impactful research in the advancement of sustainable, efficient, and less wasteful systems and technologies. Aligned with the UN's Sustainable Development Goals, the journal bridges knowledge gaps between fundamental research, implementation, and policy-making. Covering diverse topics such as climate change, food sustainability, environmental science, renewable energy, water, urban development, and socio-economic challenges, it contributes to the understanding and promotion of sustainable systems.