{"title":"发光过氧化物量子点:先进光子和量子计算应用的制造、建模和机器学习方法的进展","authors":"Deepthi Jayan K., Kesiya Babu","doi":"10.1016/j.jlumin.2024.120906","DOIUrl":null,"url":null,"abstract":"<div><div>Luminescent metal halide quantum dots (QDs), particularly perovskite quantum dots (PQDs), garnered remarkable attention for unique optical properties as well as critical use for advanced photonic and electronic devices. This comprehensive review explores the synthesis, properties, and applications of PQDs, with a focus on their role in luminescent metal halide QD devices. The review begins by discussing advanced synthesis techniques and surface engineering strategies for PQDs, highlighting recent developments in the field. Structural and optical characterization techniques are then examined, emphasizing the importance of understanding quantum confinement effects and emission mechanisms in PQDs. The review also includes a discussion on modelling and simulation, discussing computational methods for predicting and optimizing PQD properties. Experimental studies and device fabrication techniques are discussed in detail, showcasing the progress made in integrating PQDs into optoelectronic devices. Advanced applications of PQDs in light-emitting devices, solar cells, sensors, and photodetectors are explored, highlighting their potential for efficiency enhancements and novel functionalities. A detailed discussion on the emerging role of machine learning (ML) in PQD research, focusing on its applications in materials discovery and device optimization are also included. This review explores the potential of luminescent PQDs for quantum computing applications, focusing on their role as qubits, quantum gates, and quantum memory devices, emphasizing the latest advancements, challenges, and future prospects of integrating PQDs into quantum computing architectures. The review concludes with an overview of emerging trends and future directions in the field, emphasizing the need for continued research to unlock the full potential of PQDs in advanced photonic and electronic devices.</div></div>","PeriodicalId":16159,"journal":{"name":"Journal of Luminescence","volume":"277 ","pages":"Article 120906"},"PeriodicalIF":3.3000,"publicationDate":"2024-09-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Luminescent perovskite quantum dots: Progress in fabrication, modelling and machine learning approaches for advanced photonic and quantum computing applications\",\"authors\":\"Deepthi Jayan K., Kesiya Babu\",\"doi\":\"10.1016/j.jlumin.2024.120906\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Luminescent metal halide quantum dots (QDs), particularly perovskite quantum dots (PQDs), garnered remarkable attention for unique optical properties as well as critical use for advanced photonic and electronic devices. This comprehensive review explores the synthesis, properties, and applications of PQDs, with a focus on their role in luminescent metal halide QD devices. The review begins by discussing advanced synthesis techniques and surface engineering strategies for PQDs, highlighting recent developments in the field. Structural and optical characterization techniques are then examined, emphasizing the importance of understanding quantum confinement effects and emission mechanisms in PQDs. The review also includes a discussion on modelling and simulation, discussing computational methods for predicting and optimizing PQD properties. Experimental studies and device fabrication techniques are discussed in detail, showcasing the progress made in integrating PQDs into optoelectronic devices. Advanced applications of PQDs in light-emitting devices, solar cells, sensors, and photodetectors are explored, highlighting their potential for efficiency enhancements and novel functionalities. A detailed discussion on the emerging role of machine learning (ML) in PQD research, focusing on its applications in materials discovery and device optimization are also included. This review explores the potential of luminescent PQDs for quantum computing applications, focusing on their role as qubits, quantum gates, and quantum memory devices, emphasizing the latest advancements, challenges, and future prospects of integrating PQDs into quantum computing architectures. The review concludes with an overview of emerging trends and future directions in the field, emphasizing the need for continued research to unlock the full potential of PQDs in advanced photonic and electronic devices.</div></div>\",\"PeriodicalId\":16159,\"journal\":{\"name\":\"Journal of Luminescence\",\"volume\":\"277 \",\"pages\":\"Article 120906\"},\"PeriodicalIF\":3.3000,\"publicationDate\":\"2024-09-23\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Luminescence\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0022231324004708\",\"RegionNum\":3,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"OPTICS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Luminescence","FirstCategoryId":"101","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0022231324004708","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"OPTICS","Score":null,"Total":0}
Luminescent perovskite quantum dots: Progress in fabrication, modelling and machine learning approaches for advanced photonic and quantum computing applications
Luminescent metal halide quantum dots (QDs), particularly perovskite quantum dots (PQDs), garnered remarkable attention for unique optical properties as well as critical use for advanced photonic and electronic devices. This comprehensive review explores the synthesis, properties, and applications of PQDs, with a focus on their role in luminescent metal halide QD devices. The review begins by discussing advanced synthesis techniques and surface engineering strategies for PQDs, highlighting recent developments in the field. Structural and optical characterization techniques are then examined, emphasizing the importance of understanding quantum confinement effects and emission mechanisms in PQDs. The review also includes a discussion on modelling and simulation, discussing computational methods for predicting and optimizing PQD properties. Experimental studies and device fabrication techniques are discussed in detail, showcasing the progress made in integrating PQDs into optoelectronic devices. Advanced applications of PQDs in light-emitting devices, solar cells, sensors, and photodetectors are explored, highlighting their potential for efficiency enhancements and novel functionalities. A detailed discussion on the emerging role of machine learning (ML) in PQD research, focusing on its applications in materials discovery and device optimization are also included. This review explores the potential of luminescent PQDs for quantum computing applications, focusing on their role as qubits, quantum gates, and quantum memory devices, emphasizing the latest advancements, challenges, and future prospects of integrating PQDs into quantum computing architectures. The review concludes with an overview of emerging trends and future directions in the field, emphasizing the need for continued research to unlock the full potential of PQDs in advanced photonic and electronic devices.
期刊介绍:
The purpose of the Journal of Luminescence is to provide a means of communication between scientists in different disciplines who share a common interest in the electronic excited states of molecular, ionic and covalent systems, whether crystalline, amorphous, or liquid.
We invite original papers and reviews on such subjects as: exciton and polariton dynamics, dynamics of localized excited states, energy and charge transport in ordered and disordered systems, radiative and non-radiative recombination, relaxation processes, vibronic interactions in electronic excited states, photochemistry in condensed systems, excited state resonance, double resonance, spin dynamics, selective excitation spectroscopy, hole burning, coherent processes in excited states, (e.g. coherent optical transients, photon echoes, transient gratings), multiphoton processes, optical bistability, photochromism, and new techniques for the study of excited states. This list is not intended to be exhaustive. Papers in the traditional areas of optical spectroscopy (absorption, MCD, luminescence, Raman scattering) are welcome. Papers on applications (phosphors, scintillators, electro- and cathodo-luminescence, radiography, bioimaging, solar energy, energy conversion, etc.) are also welcome if they present results of scientific, rather than only technological interest. However, papers containing purely theoretical results, not related to phenomena in the excited states, as well as papers using luminescence spectroscopy to perform routine analytical chemistry or biochemistry procedures, are outside the scope of the journal. Some exceptions will be possible at the discretion of the editors.