光催化应用 g-C3N4-MXene 纳米复合材料的最新进展综述。

IF 2.9 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY
N Subha, Lakshmana Reddy Nagappagari, A Ravi Sankar
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引用次数: 0

摘要

环境修复和可再生能源发电解决方案加强了对高效光催化材料的探索。最近,g-C3N4 和 MXene 的复合材料因其在光催化领域的潜在应用而备受关注。在 g-C3N4-MXene 复合材料中,g-C3N4 具有独特的物理、化学和光学特性,可增加对可见光的吸收。同时,MXene 还能改善导电性、反应分子或活性位点的吸附性以及电荷转移特性。结合 MXene 和 g-C3N4 的独特物理化学特性,所得到的复合材料表现出卓越的光响应特性,在光催化反应中至关重要。此外,g-C3N4-MXene 复合材料还具有稳定性和可回收性,因此有望成为环境修复领域可持续、可扩展的光催化材料。本综述通过不同的合成过程深入分析了 g-C3N4-MXene 复合材料的开发和设计,并全面分析了其在二氧化碳(CO2)还原、光催化降解、水分裂过程(主要是氢(H2)生成、H2O2 生成、N2 固定和氮氧化物去除)中的应用。此外,还讨论了 g-C3N4-MXene 复合材料在光催化应用中的电荷转移机制。这篇综述深入探讨了 g-C3N4-MXene 复合材料的光催化能力,显示了它们在应对当前环境挑战和为可持续能源转换技术奠定坚实基础方面的潜力。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
A review on recent advances in g-C3N4-MXene nanocomposites for photocatalytic applications.

The solutions for environmental remediation and renewable energy generation have intensified the exploration of efficient photocatalytic materials. Recently, the composites of g-C3N4and MXene have gained considerable interest for their potential applications in photocatalysis. In the g-C3N4-MXene composite, the g-C3N4possesses unique physical, chemical, and optical properties to increase visible light absorption. At the same time, MXene improves conductivity, adsorption of reactant molecules or the active sites, and charge transfer properties. Combining the unique physico-chemical properties of MXene and g-C3N4, the resulting composite exhibits superior photo-responsive behavior and is critical in photocatalytic reactions. Furthermore, the g-C3N4-MXene composite exhibits stability and recyclability, making it a promising candidate for sustainable and scalable photocatalytic material in environmental remediation. This review offers an in-depth analysis of the development and design of g-C3N4-MXene composites through diverse synthesis procedures and a comprehensive analysis of their application in carbon dioxide (CO2) reduction, photocatalytic degradation, water splitting processes, mainly hydrogen (H2) generation, H2O2production, N2fixation, and NOxremoval. The charge transfer mechanism of g-C3N4-MXene composite for photocatalytic application has also been discussed. This review provides insights into the photocatalytic capabilities of g-C3N4-MXene composites, showing their potential to address current environmental challenges and establish a robust foundation for sustainable energy conversion technologies.

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来源期刊
Nanotechnology
Nanotechnology 工程技术-材料科学:综合
CiteScore
7.10
自引率
5.70%
发文量
820
审稿时长
2.5 months
期刊介绍: The journal aims to publish papers at the forefront of nanoscale science and technology and especially those of an interdisciplinary nature. Here, nanotechnology is taken to include the ability to individually address, control, and modify structures, materials and devices with nanometre precision, and the synthesis of such structures into systems of micro- and macroscopic dimensions such as MEMS based devices. It encompasses the understanding of the fundamental physics, chemistry, biology and technology of nanometre-scale objects and how such objects can be used in the areas of computation, sensors, nanostructured materials and nano-biotechnology.
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