{"title":"用于 Si3N4/1045 钢接触的三层薄膜的磁性处理,可持续减少摩擦和磨损","authors":"Xinrui Li, Xiaoqiang Fan, Yihan Zhang, Zhongpan Zhang, Minhao Zhu","doi":"10.1016/j.jclepro.2024.143766","DOIUrl":null,"url":null,"abstract":"<div><div>Conventional anti-wear approaches lead to energy inefficiency and excessive waste, posing significant challenges to sustainability and cleaner production. Herein, we investigate the influence of eco-friendly magnetic fields on the tribological behavior of interfaces, with an emphasis on the formation and characteristics of the protective tribofilm. The experimental design combined finite element analysis and friction tests to systematically reveal the relationship between magnetic field strength, oxidation of wear debris, and tribological properties. The results demonstrated that the introduction of a magnetic field led to a 22% reduction in the friction coefficient and a 28% decrease in wear volume. High-intensity magnetic fields refined the wear debris by up to 42.6% and also promoted the oxidation of wear debris, leading to a predominance of Fe<sub>3</sub>O<sub>4</sub> in the tribofilm. The structured arrangement and reorganization of Fe<sub>3</sub>O<sub>4</sub> particles within the tribofilm enhance its density and thickness (from 2 μm to 3 μm). Simultaneously, the rotational motion of Fe<sub>2</sub>O<sub>3</sub> particles at the interface modifies the friction contact state, thereby refining friction performance. The findings underscore the significance of considering magnetic fields in the design of tribological systems for enhanced performance and sustainability.</div></div>","PeriodicalId":9,"journal":{"name":"ACS Catalysis ","volume":null,"pages":null},"PeriodicalIF":11.3000,"publicationDate":"2024-09-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Magnetic-Manipulation of tribofilm for Si3N4/1045 steel contact toward sustainable reduction in friction and wear\",\"authors\":\"Xinrui Li, Xiaoqiang Fan, Yihan Zhang, Zhongpan Zhang, Minhao Zhu\",\"doi\":\"10.1016/j.jclepro.2024.143766\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Conventional anti-wear approaches lead to energy inefficiency and excessive waste, posing significant challenges to sustainability and cleaner production. Herein, we investigate the influence of eco-friendly magnetic fields on the tribological behavior of interfaces, with an emphasis on the formation and characteristics of the protective tribofilm. The experimental design combined finite element analysis and friction tests to systematically reveal the relationship between magnetic field strength, oxidation of wear debris, and tribological properties. The results demonstrated that the introduction of a magnetic field led to a 22% reduction in the friction coefficient and a 28% decrease in wear volume. High-intensity magnetic fields refined the wear debris by up to 42.6% and also promoted the oxidation of wear debris, leading to a predominance of Fe<sub>3</sub>O<sub>4</sub> in the tribofilm. The structured arrangement and reorganization of Fe<sub>3</sub>O<sub>4</sub> particles within the tribofilm enhance its density and thickness (from 2 μm to 3 μm). Simultaneously, the rotational motion of Fe<sub>2</sub>O<sub>3</sub> particles at the interface modifies the friction contact state, thereby refining friction performance. The findings underscore the significance of considering magnetic fields in the design of tribological systems for enhanced performance and sustainability.</div></div>\",\"PeriodicalId\":9,\"journal\":{\"name\":\"ACS Catalysis \",\"volume\":null,\"pages\":null},\"PeriodicalIF\":11.3000,\"publicationDate\":\"2024-09-22\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Catalysis \",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0959652624032153\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Catalysis ","FirstCategoryId":"93","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0959652624032153","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Magnetic-Manipulation of tribofilm for Si3N4/1045 steel contact toward sustainable reduction in friction and wear
Conventional anti-wear approaches lead to energy inefficiency and excessive waste, posing significant challenges to sustainability and cleaner production. Herein, we investigate the influence of eco-friendly magnetic fields on the tribological behavior of interfaces, with an emphasis on the formation and characteristics of the protective tribofilm. The experimental design combined finite element analysis and friction tests to systematically reveal the relationship between magnetic field strength, oxidation of wear debris, and tribological properties. The results demonstrated that the introduction of a magnetic field led to a 22% reduction in the friction coefficient and a 28% decrease in wear volume. High-intensity magnetic fields refined the wear debris by up to 42.6% and also promoted the oxidation of wear debris, leading to a predominance of Fe3O4 in the tribofilm. The structured arrangement and reorganization of Fe3O4 particles within the tribofilm enhance its density and thickness (from 2 μm to 3 μm). Simultaneously, the rotational motion of Fe2O3 particles at the interface modifies the friction contact state, thereby refining friction performance. The findings underscore the significance of considering magnetic fields in the design of tribological systems for enhanced performance and sustainability.
期刊介绍:
ACS Catalysis is an esteemed journal that publishes original research in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. It offers broad coverage across diverse areas such as life sciences, organometallics and synthesis, photochemistry and electrochemistry, drug discovery and synthesis, materials science, environmental protection, polymer discovery and synthesis, and energy and fuels.
The scope of the journal is to showcase innovative work in various aspects of catalysis. This includes new reactions and novel synthetic approaches utilizing known catalysts, the discovery or modification of new catalysts, elucidation of catalytic mechanisms through cutting-edge investigations, practical enhancements of existing processes, as well as conceptual advances in the field. Contributions to ACS Catalysis can encompass both experimental and theoretical research focused on catalytic molecules, macromolecules, and materials that exhibit catalytic turnover.