{"title":"强场电离非相对论强度下的相对论动力学和自旋轨道动力学","authors":"Andrew S. Maxwell, Lars Bojer Madsen","doi":"10.1103/physreva.110.033108","DOIUrl":null,"url":null,"abstract":"Spin-orbit dynamics and relativistic corrections to the kinetic energy in strong-field dynamics have long been ignored for near- and mid-infrared fields with intensities <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><msup><mn>10</mn><mn>13</mn></msup><mtext>–</mtext><msup><mn>10</mn><mn>14</mn></msup><mspace width=\"0.28em\"></mspace><mi mathvariant=\"normal\">W</mi><mo>/</mo><msup><mrow><mi>cm</mi></mrow><mn>2</mn></msup></mrow></math>, as the final photoelectron energies are considered too low for these effects to play a role. However, using a precise and flexible path-integral formalism, we include all correction terms from the fine-structure, Breit-Pauli Hamiltonian. This enables a treatment of spin, through coherent spin states, which is the first model to use this approach in strong-field physics. We are able to show that the most energetically rescattered wave packets are effected by relativistic kinetic energy corrections during rescattering. We probe these effects and show that they yield notable differences for a 1600-nm wavelength laser field on the dynamics and the photoelectron spectra. Furthermore, we find that the dynamical spin-orbit coupling is strongly overestimated if relativistic corrections to kinetic energy are not considered. Finally, we derive a new condition that demonstrates that relativistic effects begin to play a role at intensities many orders of magnitude lower than expected for the case of rescatterering. Our findings may have important implications for imaging processes such as laser-induced electron diffraction, which includes high-energy photoelectron recollisions.","PeriodicalId":20146,"journal":{"name":"Physical Review A","volume":"27 1","pages":""},"PeriodicalIF":2.9000,"publicationDate":"2024-09-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Relativistic and spin-orbit dynamics at nonrelativistic intensities in strong-field ionization\",\"authors\":\"Andrew S. Maxwell, Lars Bojer Madsen\",\"doi\":\"10.1103/physreva.110.033108\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Spin-orbit dynamics and relativistic corrections to the kinetic energy in strong-field dynamics have long been ignored for near- and mid-infrared fields with intensities <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mrow><msup><mn>10</mn><mn>13</mn></msup><mtext>–</mtext><msup><mn>10</mn><mn>14</mn></msup><mspace width=\\\"0.28em\\\"></mspace><mi mathvariant=\\\"normal\\\">W</mi><mo>/</mo><msup><mrow><mi>cm</mi></mrow><mn>2</mn></msup></mrow></math>, as the final photoelectron energies are considered too low for these effects to play a role. However, using a precise and flexible path-integral formalism, we include all correction terms from the fine-structure, Breit-Pauli Hamiltonian. This enables a treatment of spin, through coherent spin states, which is the first model to use this approach in strong-field physics. We are able to show that the most energetically rescattered wave packets are effected by relativistic kinetic energy corrections during rescattering. We probe these effects and show that they yield notable differences for a 1600-nm wavelength laser field on the dynamics and the photoelectron spectra. Furthermore, we find that the dynamical spin-orbit coupling is strongly overestimated if relativistic corrections to kinetic energy are not considered. Finally, we derive a new condition that demonstrates that relativistic effects begin to play a role at intensities many orders of magnitude lower than expected for the case of rescatterering. Our findings may have important implications for imaging processes such as laser-induced electron diffraction, which includes high-energy photoelectron recollisions.\",\"PeriodicalId\":20146,\"journal\":{\"name\":\"Physical Review A\",\"volume\":\"27 1\",\"pages\":\"\"},\"PeriodicalIF\":2.9000,\"publicationDate\":\"2024-09-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Physical Review A\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://doi.org/10.1103/physreva.110.033108\",\"RegionNum\":2,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"Physics and Astronomy\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Physical Review A","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1103/physreva.110.033108","RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"Physics and Astronomy","Score":null,"Total":0}
Relativistic and spin-orbit dynamics at nonrelativistic intensities in strong-field ionization
Spin-orbit dynamics and relativistic corrections to the kinetic energy in strong-field dynamics have long been ignored for near- and mid-infrared fields with intensities , as the final photoelectron energies are considered too low for these effects to play a role. However, using a precise and flexible path-integral formalism, we include all correction terms from the fine-structure, Breit-Pauli Hamiltonian. This enables a treatment of spin, through coherent spin states, which is the first model to use this approach in strong-field physics. We are able to show that the most energetically rescattered wave packets are effected by relativistic kinetic energy corrections during rescattering. We probe these effects and show that they yield notable differences for a 1600-nm wavelength laser field on the dynamics and the photoelectron spectra. Furthermore, we find that the dynamical spin-orbit coupling is strongly overestimated if relativistic corrections to kinetic energy are not considered. Finally, we derive a new condition that demonstrates that relativistic effects begin to play a role at intensities many orders of magnitude lower than expected for the case of rescatterering. Our findings may have important implications for imaging processes such as laser-induced electron diffraction, which includes high-energy photoelectron recollisions.
期刊介绍:
Physical Review A (PRA) publishes important developments in the rapidly evolving areas of atomic, molecular, and optical (AMO) physics, quantum information, and related fundamental concepts.
PRA covers atomic, molecular, and optical physics, foundations of quantum mechanics, and quantum information, including:
-Fundamental concepts
-Quantum information
-Atomic and molecular structure and dynamics; high-precision measurement
-Atomic and molecular collisions and interactions
-Atomic and molecular processes in external fields, including interactions with strong fields and short pulses
-Matter waves and collective properties of cold atoms and molecules
-Quantum optics, physics of lasers, nonlinear optics, and classical optics