用于多功能应用的带肋粘弹性 CNT-PDMS 薄膜的动态行为

IF 4.2 3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY
Matthew Phillips, Muh-Jang Chen, Jong Ryu, Mohammed Zikry
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引用次数: 0

摘要

通过在聚合物 PDMS 薄膜中添加碳纳米管(CNT)夹杂物,在大规模轧制过程中获得了定制的肋状结构,从而显著改善了系统在动态压缩应变速率下的机械行为。该研究采用非线性显式动态三维有限元(FE)方案来了解和预测制造的肋状薄膜结构在承受动态面内压缩载荷时的热机械响应。肋状薄膜的代表性体积元素 (RVE) FE 模型在横向和平行肋状方向上都承受了高达 104 s-1 的应变率。根据实验观察结果,对微观结构参数进行拉丁超立方采样,得到基于微观结构的 RVE。此外,还采用了内部点优化程序,对根据 FE 预测训练的回归模型进行优化,该模型可用于设计多功能应用的带肋材料。该模型验证了在动态压缩加载条件下,通过控制肋状微结构特征(如薄膜厚度、肋状振幅和波长),可以减轻 CNT-PDMS 系统的损坏。这种方法为设计材料提供了一个框架,这些材料可用于需要高应变率损伤耐受性、减少阻力、防污和超疏水的应用领域。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Dynamic Behavior of Ribbed Viscoelastic CNT-PDMS Thin-Films for Multifunctional Applications

Dynamic Behavior of Ribbed Viscoelastic CNT-PDMS Thin-Films for Multifunctional Applications

Tailored ribbing structures are obtained by large-scale rolling in polymer PDMS thin-films by adding carbon nanotubes (CNT) inclusions, which significantly improved the mechanical behavior of systems subjected to dynamic compressive strain rates. A nonlinear explicit dynamic three-dimensional finite-element (FE) scheme is used to understand and predict the thermomechanical response of the manufactured ribbed thin-film structures subjected to dynamic in-plane compressive loading. Representative volume element (RVE) FE models of the ribbed thin-films are subjected to strain rates as high as 104 s−1 in both the transverse and parallel ribbing directions. Latin Hypercube Sampling of the microstructural parameters, as informed from experimental observations, provide the microstructurally based RVEs. An interior-point optimization routine is also employed on a regression model trained from the FE predictions that can be used to design ribbed materials for multifunctional applications. The model verifies that damage can be mitigated in CNT-PDMS systems subjected to dynamic compressive loading conditions by controlling the ribbing microstructural characteristics, such as the film thickness and the ribbing amplitude and wavelength. This approach provides a framework for designing materials that can be utilized for applications that require high strain rate damage tolerance, drag reduction, antifouling, and superhydrophobicity.

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来源期刊
Macromolecular Materials and Engineering
Macromolecular Materials and Engineering 工程技术-材料科学:综合
CiteScore
7.30
自引率
5.10%
发文量
328
审稿时长
1.6 months
期刊介绍: Macromolecular Materials and Engineering is the high-quality polymer science journal dedicated to the design, modification, characterization, processing and application of advanced polymeric materials, including membranes, sensors, sustainability, composites, fibers, foams, 3D printing, actuators as well as energy and electronic applications. Macromolecular Materials and Engineering is among the top journals publishing original research in polymer science. The journal presents strictly peer-reviewed Research Articles, Reviews, Perspectives and Comments. ISSN: 1438-7492 (print). 1439-2054 (online). Readership:Polymer scientists, chemists, physicists, materials scientists, engineers Abstracting and Indexing Information: CAS: Chemical Abstracts Service (ACS) CCR Database (Clarivate Analytics) Chemical Abstracts Service/SciFinder (ACS) Chemistry Server Reaction Center (Clarivate Analytics) ChemWeb (ChemIndustry.com) Chimica Database (Elsevier) COMPENDEX (Elsevier) Current Contents: Physical, Chemical & Earth Sciences (Clarivate Analytics) Directory of Open Access Journals (DOAJ) INSPEC (IET) Journal Citation Reports/Science Edition (Clarivate Analytics) Materials Science & Engineering Database (ProQuest) PASCAL Database (INIST/CNRS) Polymer Library (iSmithers RAPRA) Reaction Citation Index (Clarivate Analytics) Science Citation Index (Clarivate Analytics) Science Citation Index Expanded (Clarivate Analytics) SciTech Premium Collection (ProQuest) SCOPUS (Elsevier) Technology Collection (ProQuest) Web of Science (Clarivate Analytics)
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