Mayur Mehta, N. L. Singh, Ratankumar Singh, R. Makwana, P. V. Subhash, Rakesh Chauhan, S. V. Suryanarayana, K. Katovsky
{"title":"带有不确定性传播和协方差分析的 85Rb(n,2n)84mRb 和 85Rb(n,p)85mKr 反应的活化截面","authors":"Mayur Mehta, N. L. Singh, Ratankumar Singh, R. Makwana, P. V. Subhash, Rakesh Chauhan, S. V. Suryanarayana, K. Katovsky","doi":"10.1007/s10967-024-09682-5","DOIUrl":null,"url":null,"abstract":"<p>The cross section of <sup>85</sup>Rb(n,2n)<sup>84m</sup>Rb and <sup>85</sup>Rb(n,p)<sup>85m</sup>Kr reactions were measured at neutron energy range 12–20 MeV using activation analysis followed by off-line γ-ray spectroscopic technique. The quasi mono-energetic neutrons were produced through <sup>7</sup>Li(p,n)<sup>7</sup>Be reaction. The measurements were done relative to <sup>27</sup>Al(n,α)<sup>24</sup>Na reference monitor reaction cross section. The detailed uncertainty propagation from the attributes present in measurements was performed using covariance analysis. The γ-ray self-attenuation and background low neutron energy corrections were performed in the measurement studies. Theoretical calculations were performed by TALYS-1.96 nuclear code. The comparison of measured values with the available data in EXFOR database and evaluated data from JENDL-5 and EAF-2010 shows the measured cross section values of <sup>85</sup>Rb(n,p)<sup>85m</sup>Kr reaction were slightly higher than the published values, evaluated data and theoretical data while for <sup>85</sup>Rb(n,2n)<sup>84m</sup>Rb, the measured values were consistent with the published data.</p>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":null,"pages":null},"PeriodicalIF":1.5000,"publicationDate":"2024-09-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Activation cross section for 85Rb(n,2n)84mRb and 85Rb(n,p)85mKr reactions with uncertainty propagation and covariance analysis\",\"authors\":\"Mayur Mehta, N. L. Singh, Ratankumar Singh, R. Makwana, P. V. Subhash, Rakesh Chauhan, S. V. Suryanarayana, K. Katovsky\",\"doi\":\"10.1007/s10967-024-09682-5\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>The cross section of <sup>85</sup>Rb(n,2n)<sup>84m</sup>Rb and <sup>85</sup>Rb(n,p)<sup>85m</sup>Kr reactions were measured at neutron energy range 12–20 MeV using activation analysis followed by off-line γ-ray spectroscopic technique. The quasi mono-energetic neutrons were produced through <sup>7</sup>Li(p,n)<sup>7</sup>Be reaction. The measurements were done relative to <sup>27</sup>Al(n,α)<sup>24</sup>Na reference monitor reaction cross section. The detailed uncertainty propagation from the attributes present in measurements was performed using covariance analysis. The γ-ray self-attenuation and background low neutron energy corrections were performed in the measurement studies. Theoretical calculations were performed by TALYS-1.96 nuclear code. The comparison of measured values with the available data in EXFOR database and evaluated data from JENDL-5 and EAF-2010 shows the measured cross section values of <sup>85</sup>Rb(n,p)<sup>85m</sup>Kr reaction were slightly higher than the published values, evaluated data and theoretical data while for <sup>85</sup>Rb(n,2n)<sup>84m</sup>Rb, the measured values were consistent with the published data.</p>\",\"PeriodicalId\":661,\"journal\":{\"name\":\"Journal of Radioanalytical and Nuclear Chemistry\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":1.5000,\"publicationDate\":\"2024-09-05\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Radioanalytical and Nuclear Chemistry\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://doi.org/10.1007/s10967-024-09682-5\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, ANALYTICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Radioanalytical and Nuclear Chemistry","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1007/s10967-024-09682-5","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, ANALYTICAL","Score":null,"Total":0}
Activation cross section for 85Rb(n,2n)84mRb and 85Rb(n,p)85mKr reactions with uncertainty propagation and covariance analysis
The cross section of 85Rb(n,2n)84mRb and 85Rb(n,p)85mKr reactions were measured at neutron energy range 12–20 MeV using activation analysis followed by off-line γ-ray spectroscopic technique. The quasi mono-energetic neutrons were produced through 7Li(p,n)7Be reaction. The measurements were done relative to 27Al(n,α)24Na reference monitor reaction cross section. The detailed uncertainty propagation from the attributes present in measurements was performed using covariance analysis. The γ-ray self-attenuation and background low neutron energy corrections were performed in the measurement studies. Theoretical calculations were performed by TALYS-1.96 nuclear code. The comparison of measured values with the available data in EXFOR database and evaluated data from JENDL-5 and EAF-2010 shows the measured cross section values of 85Rb(n,p)85mKr reaction were slightly higher than the published values, evaluated data and theoretical data while for 85Rb(n,2n)84mRb, the measured values were consistent with the published data.
期刊介绍:
An international periodical publishing original papers, letters, review papers and short communications on nuclear chemistry. The subjects covered include: Nuclear chemistry, Radiochemistry, Radiation chemistry, Radiobiological chemistry, Environmental radiochemistry, Production and control of radioisotopes and labelled compounds, Nuclear power plant chemistry, Nuclear fuel chemistry, Radioanalytical chemistry, Radiation detection and measurement, Nuclear instrumentation and automation, etc.