N. S. Pokryshkin, I. O. Sobina, A. A. Knysh, A. S. Eremina, A. V. Syuy, V. G. Yakunin, V. Yu. Timoshenko
{"title":"近共振激光激发下具有有效反斯托克斯光致发光的过氧化物纳米晶体光诱导加热的特殊性","authors":"N. S. Pokryshkin, I. O. Sobina, A. A. Knysh, A. S. Eremina, A. V. Syuy, V. G. Yakunin, V. Yu. Timoshenko","doi":"10.1134/s1063782624020131","DOIUrl":null,"url":null,"abstract":"<h3 data-test=\"abstract-sub-heading\">Abstract</h3><p>The optical properties of a photoluminescent material based on CsPbBr<sub>3</sub> perovskite nanocrystals were studied in this work. The laser heating of the obtained samples was studied under three different regimes of laser excitation: the photoluminescence band appears in the Stokes region, in the anti-Stokes region, and coincides with the excitation line. It was found that under laser excitation of a certain wavelength, this material is able to demonstrate predominantly anti-Stokes (upconversion) photoluminescence. A method is proposed for estimating the PL quantum yield from data on absorption, photoheating, and the position of the photoluminescence band of a sample at two different wavelengths. The external photoluminescence quantum yield of CsPbBr<sub>3</sub> nanocrystals was experimentally determined to be 91 ± 4%. The results of this work can be useful for the development of optical cooling technology and can be used in the development of laser devices based on perovskite materials.</p>","PeriodicalId":21760,"journal":{"name":"Semiconductors","volume":null,"pages":null},"PeriodicalIF":0.6000,"publicationDate":"2024-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Peculiarities of Photoinduced Heating of Perovskite Nanocrystals with Effective Anti-Stokes Photoluminescence under Near-Resonant Laser Excitation\",\"authors\":\"N. S. Pokryshkin, I. O. Sobina, A. A. Knysh, A. S. Eremina, A. V. Syuy, V. G. Yakunin, V. Yu. Timoshenko\",\"doi\":\"10.1134/s1063782624020131\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<h3 data-test=\\\"abstract-sub-heading\\\">Abstract</h3><p>The optical properties of a photoluminescent material based on CsPbBr<sub>3</sub> perovskite nanocrystals were studied in this work. The laser heating of the obtained samples was studied under three different regimes of laser excitation: the photoluminescence band appears in the Stokes region, in the anti-Stokes region, and coincides with the excitation line. It was found that under laser excitation of a certain wavelength, this material is able to demonstrate predominantly anti-Stokes (upconversion) photoluminescence. A method is proposed for estimating the PL quantum yield from data on absorption, photoheating, and the position of the photoluminescence band of a sample at two different wavelengths. The external photoluminescence quantum yield of CsPbBr<sub>3</sub> nanocrystals was experimentally determined to be 91 ± 4%. The results of this work can be useful for the development of optical cooling technology and can be used in the development of laser devices based on perovskite materials.</p>\",\"PeriodicalId\":21760,\"journal\":{\"name\":\"Semiconductors\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":0.6000,\"publicationDate\":\"2024-09-02\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Semiconductors\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://doi.org/10.1134/s1063782624020131\",\"RegionNum\":4,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q4\",\"JCRName\":\"PHYSICS, CONDENSED MATTER\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Semiconductors","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1134/s1063782624020131","RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q4","JCRName":"PHYSICS, CONDENSED MATTER","Score":null,"Total":0}
Peculiarities of Photoinduced Heating of Perovskite Nanocrystals with Effective Anti-Stokes Photoluminescence under Near-Resonant Laser Excitation
Abstract
The optical properties of a photoluminescent material based on CsPbBr3 perovskite nanocrystals were studied in this work. The laser heating of the obtained samples was studied under three different regimes of laser excitation: the photoluminescence band appears in the Stokes region, in the anti-Stokes region, and coincides with the excitation line. It was found that under laser excitation of a certain wavelength, this material is able to demonstrate predominantly anti-Stokes (upconversion) photoluminescence. A method is proposed for estimating the PL quantum yield from data on absorption, photoheating, and the position of the photoluminescence band of a sample at two different wavelengths. The external photoluminescence quantum yield of CsPbBr3 nanocrystals was experimentally determined to be 91 ± 4%. The results of this work can be useful for the development of optical cooling technology and can be used in the development of laser devices based on perovskite materials.
期刊介绍：
Publishes the most important work in semiconductor research in the countries of the former Soviet Union. Covers semiconductor theory, transport phenomena in semiconductors, optics, magnetooptics, and electrooptics of semiconductors, semiconductor lasers and semiconductor surface physics. The journal features an extensive book review section.
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