{"title":"基于二维扩散控制比色传感阵列的低成本点用传感设备,用于连续和多重空气污染监测","authors":"Jingjing Yu, Wei Ding, Francis Tsow, Chinmay Chandrakant Dixit, Vishal Varun Tipparaju, Erica Forzani, Xiaojun Xian","doi":"10.1021/acsestengg.4c00416","DOIUrl":null,"url":null,"abstract":"The development of a low-cost and point-of-use sensing device capable of continuously and simultaneously detecting various air pollutants is essential for enhancing air pollution monitoring in communities and workplaces. This technology would enable real-time monitoring, facilitating prompt interventions to mitigate the impact of air pollution on human health and the environment. Colorimetric gas sensors are often used to detect different air pollutants owing to their high selectivity and sensitivity, low cost, and compact size. Nevertheless, continuous and multiplexed detection of gas with a colorimetric sensor often requires lifetime-extension methods and an expensive, space-demanding, and power-hungry optical imaging system as the signal transducer. To address these challenges, we introduce a fully integrated portable gas sensing device that uses cheap, miniaturized, and power-efficient electronic and sensing components. This device enables continuous and multiplexed monitoring of air pollutants through a two-dimensional (2D) diffusion-controlled colorimetric sensor array. By selecting sensing probes with specific colorimetric chemical reactions for different gas analytes, the 2D sensor array ensures specificity across a range of analytes. The test results demonstrate that our 2D diffusion-based colorimetric sensing device can be used for sensitive, selective, and multiplexed monitoring of different air pollutants (ammonia, carbon monoxide, carbon dioxide, and nitrogen dioxide) in a continuous manner. This device has proven effective in monitoring pollutants released from car exhaust. Our innovative chemical sensing approach has facilitated the creation of a compact, cost-effective, and easily deployable sensing device. This device offers continuous and multiplexed sensing capabilities, making it ideal for air pollution monitoring in communities and workplaces to provide evidence-based environmental data for effective air pollution management strategies.","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"66 2 1","pages":""},"PeriodicalIF":7.4000,"publicationDate":"2024-08-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Low-Cost and Point-of-Use Sensing Device Based on 2D Diffusion-Controlled Colorimetric Sensing Array for Continuous and Multiplexed Air Pollution Monitoring\",\"authors\":\"Jingjing Yu, Wei Ding, Francis Tsow, Chinmay Chandrakant Dixit, Vishal Varun Tipparaju, Erica Forzani, Xiaojun Xian\",\"doi\":\"10.1021/acsestengg.4c00416\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The development of a low-cost and point-of-use sensing device capable of continuously and simultaneously detecting various air pollutants is essential for enhancing air pollution monitoring in communities and workplaces. This technology would enable real-time monitoring, facilitating prompt interventions to mitigate the impact of air pollution on human health and the environment. Colorimetric gas sensors are often used to detect different air pollutants owing to their high selectivity and sensitivity, low cost, and compact size. Nevertheless, continuous and multiplexed detection of gas with a colorimetric sensor often requires lifetime-extension methods and an expensive, space-demanding, and power-hungry optical imaging system as the signal transducer. To address these challenges, we introduce a fully integrated portable gas sensing device that uses cheap, miniaturized, and power-efficient electronic and sensing components. This device enables continuous and multiplexed monitoring of air pollutants through a two-dimensional (2D) diffusion-controlled colorimetric sensor array. By selecting sensing probes with specific colorimetric chemical reactions for different gas analytes, the 2D sensor array ensures specificity across a range of analytes. The test results demonstrate that our 2D diffusion-based colorimetric sensing device can be used for sensitive, selective, and multiplexed monitoring of different air pollutants (ammonia, carbon monoxide, carbon dioxide, and nitrogen dioxide) in a continuous manner. This device has proven effective in monitoring pollutants released from car exhaust. Our innovative chemical sensing approach has facilitated the creation of a compact, cost-effective, and easily deployable sensing device. This device offers continuous and multiplexed sensing capabilities, making it ideal for air pollution monitoring in communities and workplaces to provide evidence-based environmental data for effective air pollution management strategies.\",\"PeriodicalId\":7008,\"journal\":{\"name\":\"ACS ES&T engineering\",\"volume\":\"66 2 1\",\"pages\":\"\"},\"PeriodicalIF\":7.4000,\"publicationDate\":\"2024-08-27\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS ES&T engineering\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.1021/acsestengg.4c00416\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, ENVIRONMENTAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS ES&T engineering","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.1021/acsestengg.4c00416","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
Low-Cost and Point-of-Use Sensing Device Based on 2D Diffusion-Controlled Colorimetric Sensing Array for Continuous and Multiplexed Air Pollution Monitoring
The development of a low-cost and point-of-use sensing device capable of continuously and simultaneously detecting various air pollutants is essential for enhancing air pollution monitoring in communities and workplaces. This technology would enable real-time monitoring, facilitating prompt interventions to mitigate the impact of air pollution on human health and the environment. Colorimetric gas sensors are often used to detect different air pollutants owing to their high selectivity and sensitivity, low cost, and compact size. Nevertheless, continuous and multiplexed detection of gas with a colorimetric sensor often requires lifetime-extension methods and an expensive, space-demanding, and power-hungry optical imaging system as the signal transducer. To address these challenges, we introduce a fully integrated portable gas sensing device that uses cheap, miniaturized, and power-efficient electronic and sensing components. This device enables continuous and multiplexed monitoring of air pollutants through a two-dimensional (2D) diffusion-controlled colorimetric sensor array. By selecting sensing probes with specific colorimetric chemical reactions for different gas analytes, the 2D sensor array ensures specificity across a range of analytes. The test results demonstrate that our 2D diffusion-based colorimetric sensing device can be used for sensitive, selective, and multiplexed monitoring of different air pollutants (ammonia, carbon monoxide, carbon dioxide, and nitrogen dioxide) in a continuous manner. This device has proven effective in monitoring pollutants released from car exhaust. Our innovative chemical sensing approach has facilitated the creation of a compact, cost-effective, and easily deployable sensing device. This device offers continuous and multiplexed sensing capabilities, making it ideal for air pollution monitoring in communities and workplaces to provide evidence-based environmental data for effective air pollution management strategies.
期刊介绍:
ACS ES&T Engineering publishes impactful research and review articles across all realms of environmental technology and engineering, employing a rigorous peer-review process. As a specialized journal, it aims to provide an international platform for research and innovation, inviting contributions on materials technologies, processes, data analytics, and engineering systems that can effectively manage, protect, and remediate air, water, and soil quality, as well as treat wastes and recover resources.
The journal encourages research that supports informed decision-making within complex engineered systems and is grounded in mechanistic science and analytics, describing intricate environmental engineering systems. It considers papers presenting novel advancements, spanning from laboratory discovery to field-based application. However, case or demonstration studies lacking significant scientific advancements and technological innovations are not within its scope.
Contributions containing experimental and/or theoretical methods, rooted in engineering principles and integrated with knowledge from other disciplines, are welcomed.