碳量子点光催化技术的最新进展

IF 2.8 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Dan Xu, Cailian Yu, Xianlong Peng, Hong Yan, Yuanbo Zhang
{"title":"碳量子点光催化技术的最新进展","authors":"Dan Xu,&nbsp;Cailian Yu,&nbsp;Xianlong Peng,&nbsp;Hong Yan,&nbsp;Yuanbo Zhang","doi":"10.1007/s11164-024-05389-0","DOIUrl":null,"url":null,"abstract":"<div><p>Carbon quantum dots (CQDs), as a novel type of carbon nanomaterial, are widely used in fields such as drug delivery, biosensing, fluorescent probes, and photocatalysis, benefiting from their excellent photostability, water solubility, biocompatibility, fluorescence, low-cost, and green non-toxicity. Meanwhile, due to the conjugated π structure of CQDs and surface defects generated by sp<sup>2</sup> hybridization, they possess unique optoelectronic properties, including tunable fluorescence, good upconversion photoluminescence, and efficient photoelectron transfer. These properties are key to the role of CQDs in the field of photocatalysis. This review summarises CQDs’ research progress and reaction mechanisms in photocatalysis, including their optical properties and synthesis strategies. Emphasis was placed on the application of CQDs in the field of photocatalysis, including photocatalytic CO<sub>2</sub> conversion, degradation of organic and heavy metal pollutants, hydrogen production, and nitrogen fixation. In addition, the challenges and prospects of CQDs in the field of photocatalysis are discussed, providing new ideas for studying CQDs photocatalytic materials.</p><h3>Graphical abstract</h3>\n<div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":753,"journal":{"name":"Research on Chemical Intermediates","volume":"50 10","pages":"4597 - 4617"},"PeriodicalIF":2.8000,"publicationDate":"2024-08-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Recent advances in carbon quantum dot photocatalysis\",\"authors\":\"Dan Xu,&nbsp;Cailian Yu,&nbsp;Xianlong Peng,&nbsp;Hong Yan,&nbsp;Yuanbo Zhang\",\"doi\":\"10.1007/s11164-024-05389-0\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Carbon quantum dots (CQDs), as a novel type of carbon nanomaterial, are widely used in fields such as drug delivery, biosensing, fluorescent probes, and photocatalysis, benefiting from their excellent photostability, water solubility, biocompatibility, fluorescence, low-cost, and green non-toxicity. Meanwhile, due to the conjugated π structure of CQDs and surface defects generated by sp<sup>2</sup> hybridization, they possess unique optoelectronic properties, including tunable fluorescence, good upconversion photoluminescence, and efficient photoelectron transfer. These properties are key to the role of CQDs in the field of photocatalysis. This review summarises CQDs’ research progress and reaction mechanisms in photocatalysis, including their optical properties and synthesis strategies. Emphasis was placed on the application of CQDs in the field of photocatalysis, including photocatalytic CO<sub>2</sub> conversion, degradation of organic and heavy metal pollutants, hydrogen production, and nitrogen fixation. In addition, the challenges and prospects of CQDs in the field of photocatalysis are discussed, providing new ideas for studying CQDs photocatalytic materials.</p><h3>Graphical abstract</h3>\\n<div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>\",\"PeriodicalId\":753,\"journal\":{\"name\":\"Research on Chemical Intermediates\",\"volume\":\"50 10\",\"pages\":\"4597 - 4617\"},\"PeriodicalIF\":2.8000,\"publicationDate\":\"2024-08-28\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Research on Chemical Intermediates\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s11164-024-05389-0\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Research on Chemical Intermediates","FirstCategoryId":"92","ListUrlMain":"https://link.springer.com/article/10.1007/s11164-024-05389-0","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

碳量子点(CQDs)作为一种新型的碳纳米材料,具有优异的光稳定性、水溶性、生物相容性、荧光性、低成本和绿色无毒等特点,被广泛应用于药物传输、生物传感、荧光探针和光催化等领域。同时,由于 CQDs 的共轭 π 结构和 sp2 杂化产生的表面缺陷,它们具有独特的光电特性,包括可调荧光、良好的上转换光致发光和高效的光电子转移。这些特性是 CQDs 在光催化领域发挥作用的关键。本综述总结了 CQDs 在光催化领域的研究进展和反应机制,包括其光学特性和合成策略。重点介绍了 CQDs 在光催化领域的应用,包括光催化 CO2 转化、有机和重金属污染物降解、制氢和固氮。此外,还讨论了 CQDs 在光催化领域的挑战和前景,为研究 CQDs 光催化材料提供了新思路。图文摘要
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Recent advances in carbon quantum dot photocatalysis

Recent advances in carbon quantum dot photocatalysis

Carbon quantum dots (CQDs), as a novel type of carbon nanomaterial, are widely used in fields such as drug delivery, biosensing, fluorescent probes, and photocatalysis, benefiting from their excellent photostability, water solubility, biocompatibility, fluorescence, low-cost, and green non-toxicity. Meanwhile, due to the conjugated π structure of CQDs and surface defects generated by sp2 hybridization, they possess unique optoelectronic properties, including tunable fluorescence, good upconversion photoluminescence, and efficient photoelectron transfer. These properties are key to the role of CQDs in the field of photocatalysis. This review summarises CQDs’ research progress and reaction mechanisms in photocatalysis, including their optical properties and synthesis strategies. Emphasis was placed on the application of CQDs in the field of photocatalysis, including photocatalytic CO2 conversion, degradation of organic and heavy metal pollutants, hydrogen production, and nitrogen fixation. In addition, the challenges and prospects of CQDs in the field of photocatalysis are discussed, providing new ideas for studying CQDs photocatalytic materials.

Graphical abstract

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
CiteScore
5.70
自引率
18.20%
发文量
229
审稿时长
2.6 months
期刊介绍: Research on Chemical Intermediates publishes current research articles and concise dynamic reviews on the properties, structures and reactivities of intermediate species in all the various domains of chemistry. The journal also contains articles in related disciplines such as spectroscopy, molecular biology and biochemistry, atmospheric and environmental sciences, catalysis, photochemistry and photophysics. In addition, special issues dedicated to specific topics in the field are regularly published.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信