磁场增强型电催化水分离透视

IF 3.5 2区物理与天体物理 Q2 PHYSICS, APPLIED

Applied Physics Letters Pub Date : 2024-09-10 DOI:10.1063/5.0229187

Yuanyuan Zhang, Mengxin Chen, Ji Chen, Mingyi Zhang, Ping Xu

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引用次数: 0

摘要

磁场效应能够在多个尺度上增强水分离过程，因此受到广泛关注。然而，人们对磁效应的来源和磁催化剂的磁调制还缺乏系统全面的了解。本视角侧重于利用外部磁场改善电催化水分离的最新进展，并提出了未来的研究方向。首先，详细阐述了几种磁效应的机理及其对水分离的影响，包括磁流体动力学效应、磁热效应、自旋极化效应和磁阻效应。然后，总结了磁效应催化剂的分类和构建策略，主要分为单一金属/合金催化剂、基于金属氧化物的催化剂和其他磁性催化剂。最后，讨论了磁场增强水分离的挑战和潜在前景，包括机理研究、原位表征和多场协同效应。

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A perspective on magnetic field-enhanced electrocatalytic water splitting

Magnetic field effects have received widespread attention due to their ability to enhance the process of water splitting at multiple scales. However, a systematic and comprehensive understanding of the source of the magnetic effect and the magnetic modulation of magnetic catalysts is lacking. This perspective focuses on recent advancements in harnessing external magnetic field to improve electrocatalytic water splitting and suggests future directions. First, the mechanism of several magnetic effects and their effects on water splitting are elaborated in detail, including the magnetohydrodynamic effect, magnetothermal effect, spin polarization effect, and magnetoresistance effect. Then, the classification and construction strategies of magnetic effect catalysts are summarized, primarily divided into single metal/alloy catalysts, metal oxide-based catalysts, and other magnetic catalysts. Finally, the challenges and potential perspective of magnetic field-enhanced water splitting are discussed, including mechanism study, in situ characterization, and multi-field synergy effects.

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来源期刊

Applied Physics Letters 物理-物理：应用

CiteScore

6.40

自引率

10.00%

发文量

1821

审稿时长

1.6 months

期刊介绍： Applied Physics Letters (APL) features concise, up-to-date reports on significant new findings in applied physics. Emphasizing rapid dissemination of key data and new physical insights, APL offers prompt publication of new experimental and theoretical papers reporting applications of physics phenomena to all branches of science, engineering, and modern technology. In addition to regular articles, the journal also publishes invited Fast Track, Perspectives, and in-depth Editorials which report on cutting-edge areas in applied physics. APL Perspectives are forward-looking invited letters which highlight recent developments or discoveries. Emphasis is placed on very recent developments, potentially disruptive technologies, open questions and possible solutions. They also include a mini-roadmap detailing where the community should direct efforts in order for the phenomena to be viable for application and the challenges associated with meeting that performance threshold. Perspectives are characterized by personal viewpoints and opinions of recognized experts in the field. Fast Track articles are invited original research articles that report results that are particularly novel and important or provide a significant advancement in an emerging field. Because of the urgency and scientific importance of the work, the peer review process is accelerated. If, during the review process, it becomes apparent that the paper does not meet the Fast Track criterion, it is returned to a normal track.