{"title":"太阳能/微波驱动复合膜蒸发及其在海水淡化中的应用","authors":"","doi":"10.1016/j.diamond.2024.111541","DOIUrl":null,"url":null,"abstract":"<div><p>Increased economic growth and population expansion has heightened the demand for water resources, leading to escalating levels of water scarcity. Sustainable seawater desalination methods, powered by renewable energy, offer promising solutions to the long-standing global water shortage. This study presents a method for seawater desalination that employs eco-friendly materials. The approach involves utilizing metakaolin-based porous geopolymer (GP) as the base material, and depositing graphene oxide (GO) to create a graphene oxide geopolymer (GOGP) composite membrane. The membrane undergoes in-situ self-reduction to obtain reduced graphene oxide geopolymer (rGOGP). The study examines the composition, microstructure, and water evaporation performance of the composite membrane under both solar/microwave-driven. The results show that, under microwave conditions with a frequency of 2450 MHz and power of 400 W, the evaporation rate can reach up to 4.13 kg·m<sup>−2</sup>·h<sup>−1</sup>, doubling the evaporation rate achieved through solar-driven evaporation at an equivalent efficiency level. Furthermore, the evaporation rate of the composite membrane remains consistent when exposed to high-concentration saltwater of 15 wt%. Notably, the removal rates of Na<sup>+</sup>, K<sup>+</sup>, Ca<sup>2+</sup>, and Mg<sup>2+</sup> all exceed 99 %, meeting the drinking water requirements established by the World Health Organization. This study provides a novel approach to seawater desalination utilizing environmentally friendly materials and clean energy sources.</p></div>","PeriodicalId":11266,"journal":{"name":"Diamond and Related Materials","volume":null,"pages":null},"PeriodicalIF":4.3000,"publicationDate":"2024-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Solar/microwave-driven composite membrane evaporation and its application in seawater desalination\",\"authors\":\"\",\"doi\":\"10.1016/j.diamond.2024.111541\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Increased economic growth and population expansion has heightened the demand for water resources, leading to escalating levels of water scarcity. Sustainable seawater desalination methods, powered by renewable energy, offer promising solutions to the long-standing global water shortage. This study presents a method for seawater desalination that employs eco-friendly materials. The approach involves utilizing metakaolin-based porous geopolymer (GP) as the base material, and depositing graphene oxide (GO) to create a graphene oxide geopolymer (GOGP) composite membrane. The membrane undergoes in-situ self-reduction to obtain reduced graphene oxide geopolymer (rGOGP). The study examines the composition, microstructure, and water evaporation performance of the composite membrane under both solar/microwave-driven. The results show that, under microwave conditions with a frequency of 2450 MHz and power of 400 W, the evaporation rate can reach up to 4.13 kg·m<sup>−2</sup>·h<sup>−1</sup>, doubling the evaporation rate achieved through solar-driven evaporation at an equivalent efficiency level. Furthermore, the evaporation rate of the composite membrane remains consistent when exposed to high-concentration saltwater of 15 wt%. Notably, the removal rates of Na<sup>+</sup>, K<sup>+</sup>, Ca<sup>2+</sup>, and Mg<sup>2+</sup> all exceed 99 %, meeting the drinking water requirements established by the World Health Organization. This study provides a novel approach to seawater desalination utilizing environmentally friendly materials and clean energy sources.</p></div>\",\"PeriodicalId\":11266,\"journal\":{\"name\":\"Diamond and Related Materials\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":4.3000,\"publicationDate\":\"2024-09-02\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Diamond and Related Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0925963524007544\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MATERIALS SCIENCE, COATINGS & FILMS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Diamond and Related Materials","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0925963524007544","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, COATINGS & FILMS","Score":null,"Total":0}
Solar/microwave-driven composite membrane evaporation and its application in seawater desalination
Increased economic growth and population expansion has heightened the demand for water resources, leading to escalating levels of water scarcity. Sustainable seawater desalination methods, powered by renewable energy, offer promising solutions to the long-standing global water shortage. This study presents a method for seawater desalination that employs eco-friendly materials. The approach involves utilizing metakaolin-based porous geopolymer (GP) as the base material, and depositing graphene oxide (GO) to create a graphene oxide geopolymer (GOGP) composite membrane. The membrane undergoes in-situ self-reduction to obtain reduced graphene oxide geopolymer (rGOGP). The study examines the composition, microstructure, and water evaporation performance of the composite membrane under both solar/microwave-driven. The results show that, under microwave conditions with a frequency of 2450 MHz and power of 400 W, the evaporation rate can reach up to 4.13 kg·m−2·h−1, doubling the evaporation rate achieved through solar-driven evaporation at an equivalent efficiency level. Furthermore, the evaporation rate of the composite membrane remains consistent when exposed to high-concentration saltwater of 15 wt%. Notably, the removal rates of Na+, K+, Ca2+, and Mg2+ all exceed 99 %, meeting the drinking water requirements established by the World Health Organization. This study provides a novel approach to seawater desalination utilizing environmentally friendly materials and clean energy sources.
期刊介绍:
DRM is a leading international journal that publishes new fundamental and applied research on all forms of diamond, the integration of diamond with other advanced materials and development of technologies exploiting diamond. The synthesis, characterization and processing of single crystal diamond, polycrystalline films, nanodiamond powders and heterostructures with other advanced materials are encouraged topics for technical and review articles. In addition to diamond, the journal publishes manuscripts on the synthesis, characterization and application of other related materials including diamond-like carbons, carbon nanotubes, graphene, and boron and carbon nitrides. Articles are sought on the chemical functionalization of diamond and related materials as well as their use in electrochemistry, energy storage and conversion, chemical and biological sensing, imaging, thermal management, photonic and quantum applications, electron emission and electronic devices.
The International Conference on Diamond and Carbon Materials has evolved into the largest and most well attended forum in the field of diamond, providing a forum to showcase the latest results in the science and technology of diamond and other carbon materials such as carbon nanotubes, graphene, and diamond-like carbon. Run annually in association with Diamond and Related Materials the conference provides junior and established researchers the opportunity to exchange the latest results ranging from fundamental physical and chemical concepts to applied research focusing on the next generation carbon-based devices.