{"title":"掺杂钕⁺的 TeO₂-ZnO 波导中的金纳米粒子的等离子效应增强了光增益,这种波导是用基座结构制作的","authors":"","doi":"10.1016/j.jlumin.2024.120865","DOIUrl":null,"url":null,"abstract":"<div><p>Investigation of the signal enhancement of Nd<sup>3+</sup> codoped TeO<sub>2</sub>-ZnO pedestal waveguides, at 1064 nm, due to Au nanoparticles deposited over the core is presented for the first time. Nd<sup>3+</sup> doped TeO<sub>2</sub>-ZnO thin film was obtained by RF Magnetron Sputtering deposition. The resulting core with 500 nm height and widths in the 4–40 μm range, exhibited low roughness average in all area measured (0.48 ± 0.04) nm. Minimum propagation losses of 2.2 dB/cm were observed for waveguide width of 40 μm whereas an increase took place for smaller ones. Scanning electron microscopy (SEM) allowed the waveguide structure inspection and transmission electronic microscopy (TEM) the Au nanoparticles evaluation. The results showed that the Au nanoparticles contributed up to 75 % of relative gain enhancement, under 808 nm excitation. This increase was due to the local field growth in the proximity of the nanoparticles that enhances the density of excited Nd<sup>3+</sup>. The internal gain that considers the propagation losses reached positive values for larger core widths (above 8 μm).</p><p>The present study opens possibilities for optical amplifiers with low propagation losses based on different metal-dielectric composites, as well as other waveguide-based devices.</p></div>","PeriodicalId":16159,"journal":{"name":"Journal of Luminescence","volume":null,"pages":null},"PeriodicalIF":3.3000,"publicationDate":"2024-08-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Enhanced optical gain assisted by the plasmonic effects of Au nanoparticles in Nd³⁺ doped TeO₂-ZnO waveguides produced with the pedestal architecture\",\"authors\":\"\",\"doi\":\"10.1016/j.jlumin.2024.120865\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Investigation of the signal enhancement of Nd<sup>3+</sup> codoped TeO<sub>2</sub>-ZnO pedestal waveguides, at 1064 nm, due to Au nanoparticles deposited over the core is presented for the first time. Nd<sup>3+</sup> doped TeO<sub>2</sub>-ZnO thin film was obtained by RF Magnetron Sputtering deposition. The resulting core with 500 nm height and widths in the 4–40 μm range, exhibited low roughness average in all area measured (0.48 ± 0.04) nm. Minimum propagation losses of 2.2 dB/cm were observed for waveguide width of 40 μm whereas an increase took place for smaller ones. Scanning electron microscopy (SEM) allowed the waveguide structure inspection and transmission electronic microscopy (TEM) the Au nanoparticles evaluation. The results showed that the Au nanoparticles contributed up to 75 % of relative gain enhancement, under 808 nm excitation. This increase was due to the local field growth in the proximity of the nanoparticles that enhances the density of excited Nd<sup>3+</sup>. The internal gain that considers the propagation losses reached positive values for larger core widths (above 8 μm).</p><p>The present study opens possibilities for optical amplifiers with low propagation losses based on different metal-dielectric composites, as well as other waveguide-based devices.</p></div>\",\"PeriodicalId\":16159,\"journal\":{\"name\":\"Journal of Luminescence\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":3.3000,\"publicationDate\":\"2024-08-29\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Luminescence\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0022231324004290\",\"RegionNum\":3,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"OPTICS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Luminescence","FirstCategoryId":"101","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0022231324004290","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"OPTICS","Score":null,"Total":0}
Enhanced optical gain assisted by the plasmonic effects of Au nanoparticles in Nd³⁺ doped TeO₂-ZnO waveguides produced with the pedestal architecture
Investigation of the signal enhancement of Nd3+ codoped TeO2-ZnO pedestal waveguides, at 1064 nm, due to Au nanoparticles deposited over the core is presented for the first time. Nd3+ doped TeO2-ZnO thin film was obtained by RF Magnetron Sputtering deposition. The resulting core with 500 nm height and widths in the 4–40 μm range, exhibited low roughness average in all area measured (0.48 ± 0.04) nm. Minimum propagation losses of 2.2 dB/cm were observed for waveguide width of 40 μm whereas an increase took place for smaller ones. Scanning electron microscopy (SEM) allowed the waveguide structure inspection and transmission electronic microscopy (TEM) the Au nanoparticles evaluation. The results showed that the Au nanoparticles contributed up to 75 % of relative gain enhancement, under 808 nm excitation. This increase was due to the local field growth in the proximity of the nanoparticles that enhances the density of excited Nd3+. The internal gain that considers the propagation losses reached positive values for larger core widths (above 8 μm).
The present study opens possibilities for optical amplifiers with low propagation losses based on different metal-dielectric composites, as well as other waveguide-based devices.
期刊介绍:
The purpose of the Journal of Luminescence is to provide a means of communication between scientists in different disciplines who share a common interest in the electronic excited states of molecular, ionic and covalent systems, whether crystalline, amorphous, or liquid.
We invite original papers and reviews on such subjects as: exciton and polariton dynamics, dynamics of localized excited states, energy and charge transport in ordered and disordered systems, radiative and non-radiative recombination, relaxation processes, vibronic interactions in electronic excited states, photochemistry in condensed systems, excited state resonance, double resonance, spin dynamics, selective excitation spectroscopy, hole burning, coherent processes in excited states, (e.g. coherent optical transients, photon echoes, transient gratings), multiphoton processes, optical bistability, photochromism, and new techniques for the study of excited states. This list is not intended to be exhaustive. Papers in the traditional areas of optical spectroscopy (absorption, MCD, luminescence, Raman scattering) are welcome. Papers on applications (phosphors, scintillators, electro- and cathodo-luminescence, radiography, bioimaging, solar energy, energy conversion, etc.) are also welcome if they present results of scientific, rather than only technological interest. However, papers containing purely theoretical results, not related to phenomena in the excited states, as well as papers using luminescence spectroscopy to perform routine analytical chemistry or biochemistry procedures, are outside the scope of the journal. Some exceptions will be possible at the discretion of the editors.