F. Pizzi , M. Rahmani , C. Romera-Castillo , F. Peters , J. Grau , F. Capuano , L. Jofre
{"title":"凝结特性对上层海洋湍流中微塑料聚集的影响","authors":"F. Pizzi , M. Rahmani , C. Romera-Castillo , F. Peters , J. Grau , F. Capuano , L. Jofre","doi":"10.1016/j.advwatres.2024.104798","DOIUrl":null,"url":null,"abstract":"<div><p>The dynamics and aggregation of microplastics in marine environments are investigated through high-fidelity direct numerical simulations with Lagrangian point-particle tracking. The properties of microplastics and biogenic particles, including size, density, and concentration, align with scenarios typical of seawater systems. The stickiness nature of microplastics, induced by biofilm formation (biofouling), is modeled through coagulation efficiency (stickiness parameter), which represents the probability of aggregation following a collision event. Two main aspects are at the core of the present work: analyzing the mechanisms of collision and coalescence between microplastics and biogenic particles, along with their spatial distribution, and characterizing the emerging aggregates. The results indicate that particles stickiness, concentration and (especially) size impact on the collision and coalescence rates. Furthermore, microplastics exhibit a strong tendency to accumulate near biogenic particles, leading to the creation of hetero-aggregates whose tendency to sink supports the general hypothesis of “missing microplastics”. Particularly, in cases where microplastics and biogenic particles are evenly concentrated, microplastics primarily contribute to the formation of aggregates. The stickiness mainly determines the most complex and large aggregates, which are less than 1% of the total.</p></div>","PeriodicalId":7614,"journal":{"name":"Advances in Water Resources","volume":"193 ","pages":"Article 104798"},"PeriodicalIF":4.0000,"publicationDate":"2024-08-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S0309170824001854/pdfft?md5=fc4f45b46f9fa9d8b4ba89f62b60412c&pid=1-s2.0-S0309170824001854-main.pdf","citationCount":"0","resultStr":"{\"title\":\"Impact of coagulation characteristics on the aggregation of microplastics in upper-ocean turbulence\",\"authors\":\"F. Pizzi , M. Rahmani , C. Romera-Castillo , F. Peters , J. Grau , F. Capuano , L. Jofre\",\"doi\":\"10.1016/j.advwatres.2024.104798\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>The dynamics and aggregation of microplastics in marine environments are investigated through high-fidelity direct numerical simulations with Lagrangian point-particle tracking. The properties of microplastics and biogenic particles, including size, density, and concentration, align with scenarios typical of seawater systems. The stickiness nature of microplastics, induced by biofilm formation (biofouling), is modeled through coagulation efficiency (stickiness parameter), which represents the probability of aggregation following a collision event. Two main aspects are at the core of the present work: analyzing the mechanisms of collision and coalescence between microplastics and biogenic particles, along with their spatial distribution, and characterizing the emerging aggregates. The results indicate that particles stickiness, concentration and (especially) size impact on the collision and coalescence rates. Furthermore, microplastics exhibit a strong tendency to accumulate near biogenic particles, leading to the creation of hetero-aggregates whose tendency to sink supports the general hypothesis of “missing microplastics”. Particularly, in cases where microplastics and biogenic particles are evenly concentrated, microplastics primarily contribute to the formation of aggregates. The stickiness mainly determines the most complex and large aggregates, which are less than 1% of the total.</p></div>\",\"PeriodicalId\":7614,\"journal\":{\"name\":\"Advances in Water Resources\",\"volume\":\"193 \",\"pages\":\"Article 104798\"},\"PeriodicalIF\":4.0000,\"publicationDate\":\"2024-08-30\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.sciencedirect.com/science/article/pii/S0309170824001854/pdfft?md5=fc4f45b46f9fa9d8b4ba89f62b60412c&pid=1-s2.0-S0309170824001854-main.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advances in Water Resources\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0309170824001854\",\"RegionNum\":2,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"WATER RESOURCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advances in Water Resources","FirstCategoryId":"93","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0309170824001854","RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"WATER RESOURCES","Score":null,"Total":0}
Impact of coagulation characteristics on the aggregation of microplastics in upper-ocean turbulence
The dynamics and aggregation of microplastics in marine environments are investigated through high-fidelity direct numerical simulations with Lagrangian point-particle tracking. The properties of microplastics and biogenic particles, including size, density, and concentration, align with scenarios typical of seawater systems. The stickiness nature of microplastics, induced by biofilm formation (biofouling), is modeled through coagulation efficiency (stickiness parameter), which represents the probability of aggregation following a collision event. Two main aspects are at the core of the present work: analyzing the mechanisms of collision and coalescence between microplastics and biogenic particles, along with their spatial distribution, and characterizing the emerging aggregates. The results indicate that particles stickiness, concentration and (especially) size impact on the collision and coalescence rates. Furthermore, microplastics exhibit a strong tendency to accumulate near biogenic particles, leading to the creation of hetero-aggregates whose tendency to sink supports the general hypothesis of “missing microplastics”. Particularly, in cases where microplastics and biogenic particles are evenly concentrated, microplastics primarily contribute to the formation of aggregates. The stickiness mainly determines the most complex and large aggregates, which are less than 1% of the total.
期刊介绍:
Advances in Water Resources provides a forum for the presentation of fundamental scientific advances in the understanding of water resources systems. The scope of Advances in Water Resources includes any combination of theoretical, computational, and experimental approaches used to advance fundamental understanding of surface or subsurface water resources systems or the interaction of these systems with the atmosphere, geosphere, biosphere, and human societies. Manuscripts involving case studies that do not attempt to reach broader conclusions, research on engineering design, applied hydraulics, or water quality and treatment, as well as applications of existing knowledge that do not advance fundamental understanding of hydrological processes, are not appropriate for Advances in Water Resources.
Examples of appropriate topical areas that will be considered include the following:
• Surface and subsurface hydrology
• Hydrometeorology
• Environmental fluid dynamics
• Ecohydrology and ecohydrodynamics
• Multiphase transport phenomena in porous media
• Fluid flow and species transport and reaction processes