土壤性质的垂直变化对 137Cs 沉积的 H*(10)模拟的影响

IF 1.9 3区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES
Xibo Ma, Hikaru Kobayashi
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引用次数: 0

摘要

在评估和估算福岛核电站事故后 137Cs 在土壤中沉积所产生的环境剂量当量率 H*(10)时,基于蒙特卡罗方法的光子传输模拟发挥了至关重要的作用。然而,目前尚未对土壤性质的垂直变化对模拟结果的影响进行全面研究。忽略土壤性质的垂直分布不仅会导致土壤层屏蔽响应的潜在误差,还会导致放射源清单的确定,尤其是在使用以 Bq/kg 为单位的浓度数据时。这些疏忽降低了模拟结果的可靠性。本研究探讨了可能影响模拟结果的几种土壤性质因素,包括含水量引起的化学成分变化、容重分布和估计库存分布,所有这些都通过一个经过检验的模拟模型进行了评估。结果表明,不适当地分配土壤密度剖面会导致 H*(10)模拟结果出现相当大的误差。此外,还分析了 H*(10)对土壤垂直密度变化的敏感性,结果表明 H*(10)对顶部 0-5 厘米土壤层容重的变化高度敏感。这些结果有助于制定适当的模拟策略,并支持对过去的模拟结果进行重新评估。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Impacts of vertical variations in soil properties on H*(10) simulations for 137Cs deposition

Photon transport simulations based on the Monte Carlo method have played a crucial role in assessing and estimating the ambient dose equivalent rates H*(10), resulting from the deposition of 137Cs in soil following the nuclear power plant accident in Fukushima. However, a comprehensive examination of the effect of vertical variations in soil properties on the simulation outcomes has not yet been performed. Disregarding the vertical distribution of soil properties not only leads to potential inaccuracies in the shielding responses of soil layers but also in the determination of the radioactive source inventory, particularly when using the concentration data in Bq/kg. These oversights diminish the reliability of the simulation results. This study addresses several soil property factors that could potentially influence the simulation results, including variations in chemical composition induced by water content, bulk density profile, and estimated inventory profile, all evaluated through an examined simulation model. The results show that inappropriate assignment of the soil density profile can cause considerable errors in the H*(10) simulation outcomes. Furthermore, the sensitivity of H*(10) to variations in soil vertical density is analyzed, with the results indicating that H*(10) can be highly sensitive to changes in the bulk density of the top 0–5 cm soil layers. These results should facilitate the establishment of appropriate simulation strategies and support the reassessment of past simulation results.

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来源期刊
Journal of environmental radioactivity
Journal of environmental radioactivity 环境科学-环境科学
CiteScore
4.70
自引率
13.00%
发文量
209
审稿时长
73 days
期刊介绍: The Journal of Environmental Radioactivity provides a coherent international forum for publication of original research or review papers on any aspect of the occurrence of radioactivity in natural systems. Relevant subject areas range from applications of environmental radionuclides as mechanistic or timescale tracers of natural processes to assessments of the radioecological or radiological effects of ambient radioactivity. Papers deal with naturally occurring nuclides or with those created and released by man through nuclear weapons manufacture and testing, energy production, fuel-cycle technology, etc. Reports on radioactivity in the oceans, sediments, rivers, lakes, groundwaters, soils, atmosphere and all divisions of the biosphere are welcomed, but these should not simply be of a monitoring nature unless the data are particularly innovative.
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