{"title":"光催化 H2O2 生成的演变：从纯水到自然系统及其他","authors":"Yuyang Tang, Wuming Wang, Jiaqi Ran, Cheng Peng, Zuxin Xu and Wenhai Chu","doi":"10.1039/D4EE02505A","DOIUrl":null,"url":null,"abstract":"<p >Photocatalytic hydrogen peroxide (PHP) production represents a sustainable approach that mimics photosynthesis using sunlight to generate H<small><sub>2</sub></small>O<small><sub>2</sub></small> from water and oxygen. This review explores the intricate mechanisms of PHP and provides a critical assessment on the development of PHP in different systems, including pure water, natural water, microdroplets, and coupling systems. Furthermore, their potential applications in environmental remediation, biomedicine and the production of high-value chemicals are discussed. Moreover, the current limitations of PHP efficiency and stability, particularly in the pure water system, are summarized, and possible solutions to overcome these challenges are proposed as well. The objective of this paper is to present perspectives on improving the PHP efficiency and to advance the sustainable development of PHP technology.</p>","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":" 18","pages":" 6482-6498"},"PeriodicalIF":30.8000,"publicationDate":"2024-08-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.rsc.org/en/content/articlepdf/2024/ee/d4ee02505a?page=search","citationCount":"0","resultStr":"{\"title\":\"The evolution of photocatalytic H2O2 generation: from pure water to natural systems and beyond\",\"authors\":\"Yuyang Tang, Wuming Wang, Jiaqi Ran, Cheng Peng, Zuxin Xu and Wenhai Chu\",\"doi\":\"10.1039/D4EE02505A\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Photocatalytic hydrogen peroxide (PHP) production represents a sustainable approach that mimics photosynthesis using sunlight to generate H<small><sub>2</sub></small>O<small><sub>2</sub></small> from water and oxygen. This review explores the intricate mechanisms of PHP and provides a critical assessment on the development of PHP in different systems, including pure water, natural water, microdroplets, and coupling systems. Furthermore, their potential applications in environmental remediation, biomedicine and the production of high-value chemicals are discussed. Moreover, the current limitations of PHP efficiency and stability, particularly in the pure water system, are summarized, and possible solutions to overcome these challenges are proposed as well. The objective of this paper is to present perspectives on improving the PHP efficiency and to advance the sustainable development of PHP technology.</p>\",\"PeriodicalId\":72,\"journal\":{\"name\":\"Energy & Environmental Science\",\"volume\":\" 18\",\"pages\":\" 6482-6498\"},\"PeriodicalIF\":30.8000,\"publicationDate\":\"2024-08-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://pubs.rsc.org/en/content/articlepdf/2024/ee/d4ee02505a?page=search\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Energy & Environmental Science\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://pubs.rsc.org/en/content/articlelanding/2024/ee/d4ee02505a\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Energy & Environmental Science","FirstCategoryId":"88","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2024/ee/d4ee02505a","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
The evolution of photocatalytic H2O2 generation: from pure water to natural systems and beyond
Photocatalytic hydrogen peroxide (PHP) production represents a sustainable approach that mimics photosynthesis using sunlight to generate H2O2 from water and oxygen. This review explores the intricate mechanisms of PHP and provides a critical assessment on the development of PHP in different systems, including pure water, natural water, microdroplets, and coupling systems. Furthermore, their potential applications in environmental remediation, biomedicine and the production of high-value chemicals are discussed. Moreover, the current limitations of PHP efficiency and stability, particularly in the pure water system, are summarized, and possible solutions to overcome these challenges are proposed as well. The objective of this paper is to present perspectives on improving the PHP efficiency and to advance the sustainable development of PHP technology.
期刊介绍：
Energy & Environmental Science, a peer-reviewed scientific journal, publishes original research and review articles covering interdisciplinary topics in the (bio)chemical and (bio)physical sciences, as well as chemical engineering disciplines. Published monthly by the Royal Society of Chemistry (RSC), a not-for-profit publisher, Energy & Environmental Science is recognized as a leading journal. It boasts an impressive impact factor of 8.500 as of 2009, ranking 8th among 140 journals in the category "Chemistry, Multidisciplinary," second among 71 journals in "Energy & Fuels," second among 128 journals in "Engineering, Chemical," and first among 181 scientific journals in "Environmental Sciences."
Energy & Environmental Science publishes various types of articles, including Research Papers (original scientific work), Review Articles, Perspectives, and Minireviews (feature review-type articles of broad interest), Communications (original scientific work of an urgent nature), Opinions (personal, often speculative viewpoints or hypotheses on current topics), and Analysis Articles (in-depth examination of energy-related issues).
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