{"title":"微通道陶瓷甲醇转化器的设计与性能实验研究","authors":"Haoming Sun, Dong Tang, Ruixiao Tian, Jinyan Tang","doi":"10.1007/s11581-024-05726-8","DOIUrl":null,"url":null,"abstract":"<div><p>Hydrogen possesses high energy density and emits zero carbon, making it a promising alternative fuel. However, the current storage and transportation of hydrogen pose significant safety risks. The on-site hydrogen production technology through methanol reforming offers a fundamental solution to the challenges of hydrogen storage and transportation. This study presents the design of a microchannel methanol reformer fabricated using cordierite honeycomb ceramics and evaluates its operational performance through multi-parameter experiments. The results show that optimal reforming performance is achieved at a reaction temperature of 553 K, a water-to-methanol ratio of 1.25, and a feed volume of 0.4 ml/min. Under these conditions, methanol conversion reaches 84.99%, hydrogen production amounts to 361.69 ml/min, and the carbon monoxide concentration is 0.6232%, demonstrating good stability during prolonged operation. This study provides valuable insights for the industrialization of methanol reformers and the utilization of hydrogen energy.</p></div>","PeriodicalId":599,"journal":{"name":"Ionics","volume":"30 10","pages":"6279 - 6291"},"PeriodicalIF":2.4000,"publicationDate":"2024-07-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Design and performance experimental study of microchannel ceramic methanol reformer\",\"authors\":\"Haoming Sun, Dong Tang, Ruixiao Tian, Jinyan Tang\",\"doi\":\"10.1007/s11581-024-05726-8\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Hydrogen possesses high energy density and emits zero carbon, making it a promising alternative fuel. However, the current storage and transportation of hydrogen pose significant safety risks. The on-site hydrogen production technology through methanol reforming offers a fundamental solution to the challenges of hydrogen storage and transportation. This study presents the design of a microchannel methanol reformer fabricated using cordierite honeycomb ceramics and evaluates its operational performance through multi-parameter experiments. The results show that optimal reforming performance is achieved at a reaction temperature of 553 K, a water-to-methanol ratio of 1.25, and a feed volume of 0.4 ml/min. Under these conditions, methanol conversion reaches 84.99%, hydrogen production amounts to 361.69 ml/min, and the carbon monoxide concentration is 0.6232%, demonstrating good stability during prolonged operation. This study provides valuable insights for the industrialization of methanol reformers and the utilization of hydrogen energy.</p></div>\",\"PeriodicalId\":599,\"journal\":{\"name\":\"Ionics\",\"volume\":\"30 10\",\"pages\":\"6279 - 6291\"},\"PeriodicalIF\":2.4000,\"publicationDate\":\"2024-07-23\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Ionics\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s11581-024-05726-8\",\"RegionNum\":4,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Ionics","FirstCategoryId":"92","ListUrlMain":"https://link.springer.com/article/10.1007/s11581-024-05726-8","RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Design and performance experimental study of microchannel ceramic methanol reformer
Hydrogen possesses high energy density and emits zero carbon, making it a promising alternative fuel. However, the current storage and transportation of hydrogen pose significant safety risks. The on-site hydrogen production technology through methanol reforming offers a fundamental solution to the challenges of hydrogen storage and transportation. This study presents the design of a microchannel methanol reformer fabricated using cordierite honeycomb ceramics and evaluates its operational performance through multi-parameter experiments. The results show that optimal reforming performance is achieved at a reaction temperature of 553 K, a water-to-methanol ratio of 1.25, and a feed volume of 0.4 ml/min. Under these conditions, methanol conversion reaches 84.99%, hydrogen production amounts to 361.69 ml/min, and the carbon monoxide concentration is 0.6232%, demonstrating good stability during prolonged operation. This study provides valuable insights for the industrialization of methanol reformers and the utilization of hydrogen energy.
期刊介绍:
Ionics is publishing original results in the fields of science and technology of ionic motion. This includes theoretical, experimental and practical work on electrolytes, electrode, ionic/electronic interfaces, ionic transport aspects of corrosion, galvanic cells, e.g. for thermodynamic and kinetic studies, batteries, fuel cells, sensors and electrochromics. Fast solid ionic conductors are presently providing new opportunities in view of several advantages, in addition to conventional liquid electrolytes.