具有高过滤效率和抗菌特性的木纤维三电材料及其在面罩中的呼吸监测功能

IF 4.3 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
ACS Omega Pub Date : 2024-07-25 DOI:10.1021/acsomega.4c01906
Xiaoping Sun, Juan Yuan, Qiuxiao Zhu, Yanfen Sun, Haoqiu Chen, Shuangli Liao, Jiaxuan Yan, Jiecheng Cai, Yuhe Wei, Lianxin Luo
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引用次数: 0

摘要

自供电的可穿戴电子产品在传感和健康监测领域发展迅速,这给三电材料带来了更大的挑战。木纤维有限的表面极性和结构缺陷限制了其作为石油基材料替代品的潜力。本研究以甘蔗渣纤维为原料,探索了多种方法,包括用多巴胺(PDA)对纤维素纳米纤维(CNFs)进行功能化处理、原位嵌入银颗粒、过滤和冷冻干燥。这些方法旨在提高木质纤维素材料的三电输出、抗菌性能和过滤性能。基于 Ag/PDA/CNF 的三电纳米发电机(TENG)的开路电压为 211 V,短路电流为 18.1 μA。通过冷冻干燥 Ag/PDA/CNF 材料制备的气凝胶与通过电纺丝制造的聚偏氟乙烯纳米纤维结构相结合,构成了 TENG 单元。利用这种组合制造出的自供电呼吸检测口罩,对 0.3 μm 微粒的过滤效率达到 94.23%,抗菌率超过 99%。此外,它还能有效响应呼吸缓慢、呼吸正常和呼吸急促的呼吸频率信号,输出的电信号与呼吸频率相关。这项研究极大地推动了木纤维三电材料在医疗应用的自供电可穿戴电子产品中作为石油衍生材料的替代品。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Wood Fiber-Based Triboelectric Material with High Filtration Efficiency and Antibacterial Properties and Its Respiratory Monitoring in Mask

Wood Fiber-Based Triboelectric Material with High Filtration Efficiency and Antibacterial Properties and Its Respiratory Monitoring in Mask
Self-powered wearable electronic products have rapidly advanced in the fields of sensing and health monitoring, presenting greater challenges for triboelectric materials. The limited surface polarity and structural defects in wood fibers restrict their potential as substitutes for petroleum-based materials. This study used bagasse fiber as the raw material and explored various methods, including functionalizing cellulose nanofibrils (CNFs) with polydopamine (PDA), in situ embedding of silver particles, filtration, and freeze-drying. These methods aimed to enhance the triboelectric output, antibacterial properties, and filtration properties of lignocellulosic materials. The Ag/PDA/CNF-based triboelectric nanogenerator (TENG) demonstrated an open-circuit voltage of 211 V and a short-circuit current of 18.1 μA. An aerogel prepared by freeze-drying the Ag/PDA/CNF material, combined with a polyvinylidene fluoride nanofiber structure fabricated by electrospinning, constitutes the TENG unit. A self-powered respiratory detection mask was created using this combination, achieving a filtration efficiency of 94.23% for 0.3 μm particles and an antibacterial rate exceeding 99%. In addition, it effectively responded to respiratory frequency signals of slow breathing, normal breathing, and shortness of breath, with the output electrical signal correlating with the respiratory frequency. This study considerably contributes to advancing wood fiber-based triboelectric materials as alternatives to petroleum-derived materials in self-powered wearable electronic products for medical applications.
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来源期刊
ACS Omega
ACS Omega Chemical Engineering-General Chemical Engineering
CiteScore
6.60
自引率
4.90%
发文量
3945
审稿时长
2.4 months
期刊介绍: ACS Omega is an open-access global publication for scientific articles that describe new findings in chemistry and interfacing areas of science, without any perceived evaluation of immediate impact.
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