Samantha Smith, Lewis Gaston, Jeffery Beasley, Jim Wang, Josh Padilla, Wenguang Sun
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引用次数: 0
摘要
渗流中磷的流失可能会导致下游水体富营养化。本研究考察了在可渗透反应屏障(PRB)中使用生铁岩和未经处理的赤泥(铝土矿提炼残渣)作为磷吸附剂以减少磷流失的可能性。研究了铁石和红泥对 P 的吸附(批量)、传输(柱)、饱和水力传导性(KS)和普通百慕大草(Cynodon dactylon;温室)生长的影响。两种材料的最大吸附量都在 30 mmol P kg-1 以下,约为富含 P 的沙质土壤的五倍;但随着 pH 值的降低,红泥的吸附量大大增加。与土壤 + 沙土相比,通过铁石柱和赤泥(用无反应沙稀释)传输 P 的速度相似且较慢。然而,当赤泥与土壤混合时,pH 值较低时吸附力增加,与铁石+土壤(76% 对 13%)相比,赤泥的钾保留率更高。虽然在土壤中加入 20% 的铁石不会降低 KS,但加入 5% 的红泥也会降低 KS。用赤泥改良土壤可增加百慕大草的生长和对钾的吸收。考虑到赤泥在酸性土壤中的长期中和作用以及对钾的吸附作用,如果赤泥的添加量较低,并且/或者与较粗的材料共同添加,那么赤泥可能适合在PRB中使用。
Ironstone and red mud barriers to reduce subsurface movement of soil phosphorus
Loss of phosphorus in seepage may contribute to eutrophication of downstream water bodies. This study examined the potential use of pedogenic ironstone and untreated red mud (bauxite refining residue) as P sorbents in a permeable reactive barrier (PRB) to mitigate such loss. Effects of ironstone and red mud on P sorption (batch), transport (columns), saturated hydraulic conductivity (KS), and growth of common bermudagrass (Cynodon dactylon; greenhouse) were examined. Both materials had sorption maxima of ∼30 mmol P kg−1 or about five times that of a P-enriched sandy soil; however, sorption by red mud greatly increased with decreasing pH. Transport of P through columns of ironstone and red mud (diluted with nonreactive sand) was similar and slower compared to soil + sand. However, when red mud was mixed with soil, increased sorption at lower pH resulted in greater P retention compared to ironstone + soil (76% vs. 13%). Although addition of ironstone to soil up to 20% did not reduce KS, red mud at even 5% did. Soil amendment with red mud increased bermudagrass growth and P uptake. Given long-term neutralization of red mud in an acidic soil and increased P sorption, it may be suitable in a PRB if incorporated at a low rate and/or co-incorporated with a coarser material.
期刊介绍:
Articles in JEQ cover various aspects of anthropogenic impacts on the environment, including agricultural, terrestrial, atmospheric, and aquatic systems, with emphasis on the understanding of underlying processes. To be acceptable for consideration in JEQ, a manuscript must make a significant contribution to the advancement of knowledge or toward a better understanding of existing concepts. The study should define principles of broad applicability, be related to problems over a sizable geographic area, or be of potential interest to a representative number of scientists. Emphasis is given to the understanding of underlying processes rather than to monitoring.
Contributions are accepted from all disciplines for consideration by the editorial board. Manuscripts may be volunteered, invited, or coordinated as a special section or symposium.