Yang Cao, Liming Qing, Junru Yao, Yan Wang, Ning Gu, Qiang Fu, Youyi Sun
{"title":"用于固态超级电容器的集成电极分离器-电解质水凝胶的简易合成","authors":"Yang Cao, Liming Qing, Junru Yao, Yan Wang, Ning Gu, Qiang Fu, Youyi Sun","doi":"10.1007/s10008-024-06013-2","DOIUrl":null,"url":null,"abstract":"<div><p>A new integrated electrode-separator-electrolyte hydrogel is designed and prepared, which is composed of organic liquid crystal, polyvinyl alcohol (PVA), polyaniline (PANI), and reduced graphene oxide (rGO). The organic liquid crystal is introduced into PVA hydrogel, effectively improving compatibility between active materials and hydrogel matrix. The PANI active material is in situ polymerized in hydrogel to prepare PANI-double-network hydrogel. It simultaneously acts as electrode, separator, and electrolyte for assembling flexible solid-state supercapacitor. It obtains an area-specific capacitance of 160.2 mF/cm<sup>2</sup> and a power density of 101.5 μW/cm<sup>2</sup> with an energy density of 21.0 μWh/cm<sup>2</sup>. This work provides a new method to reduce interfacial resistance of electrode, separator, and electrolyte of flexible solid-state supercapacitor, further improving its electrochemical performance.</p></div>","PeriodicalId":665,"journal":{"name":"Journal of Solid State Electrochemistry","volume":"28 11","pages":"4067 - 4075"},"PeriodicalIF":2.6000,"publicationDate":"2024-07-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Facile synthesis of integrated electrode-separator-electrolyte hydrogel for solid-state supercapacitor\",\"authors\":\"Yang Cao, Liming Qing, Junru Yao, Yan Wang, Ning Gu, Qiang Fu, Youyi Sun\",\"doi\":\"10.1007/s10008-024-06013-2\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>A new integrated electrode-separator-electrolyte hydrogel is designed and prepared, which is composed of organic liquid crystal, polyvinyl alcohol (PVA), polyaniline (PANI), and reduced graphene oxide (rGO). The organic liquid crystal is introduced into PVA hydrogel, effectively improving compatibility between active materials and hydrogel matrix. The PANI active material is in situ polymerized in hydrogel to prepare PANI-double-network hydrogel. It simultaneously acts as electrode, separator, and electrolyte for assembling flexible solid-state supercapacitor. It obtains an area-specific capacitance of 160.2 mF/cm<sup>2</sup> and a power density of 101.5 μW/cm<sup>2</sup> with an energy density of 21.0 μWh/cm<sup>2</sup>. This work provides a new method to reduce interfacial resistance of electrode, separator, and electrolyte of flexible solid-state supercapacitor, further improving its electrochemical performance.</p></div>\",\"PeriodicalId\":665,\"journal\":{\"name\":\"Journal of Solid State Electrochemistry\",\"volume\":\"28 11\",\"pages\":\"4067 - 4075\"},\"PeriodicalIF\":2.6000,\"publicationDate\":\"2024-07-16\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Solid State Electrochemistry\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s10008-024-06013-2\",\"RegionNum\":4,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ELECTROCHEMISTRY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Solid State Electrochemistry","FirstCategoryId":"5","ListUrlMain":"https://link.springer.com/article/10.1007/s10008-024-06013-2","RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ELECTROCHEMISTRY","Score":null,"Total":0}
Facile synthesis of integrated electrode-separator-electrolyte hydrogel for solid-state supercapacitor
A new integrated electrode-separator-electrolyte hydrogel is designed and prepared, which is composed of organic liquid crystal, polyvinyl alcohol (PVA), polyaniline (PANI), and reduced graphene oxide (rGO). The organic liquid crystal is introduced into PVA hydrogel, effectively improving compatibility between active materials and hydrogel matrix. The PANI active material is in situ polymerized in hydrogel to prepare PANI-double-network hydrogel. It simultaneously acts as electrode, separator, and electrolyte for assembling flexible solid-state supercapacitor. It obtains an area-specific capacitance of 160.2 mF/cm2 and a power density of 101.5 μW/cm2 with an energy density of 21.0 μWh/cm2. This work provides a new method to reduce interfacial resistance of electrode, separator, and electrolyte of flexible solid-state supercapacitor, further improving its electrochemical performance.
期刊介绍：
The Journal of Solid State Electrochemistry is devoted to all aspects of solid-state chemistry and solid-state physics in electrochemistry.
The Journal of Solid State Electrochemistry publishes papers on all aspects of electrochemistry of solid compounds, including experimental and theoretical, basic and applied work. It equally publishes papers on the thermodynamics and kinetics of electrochemical reactions if at least one actively participating phase is solid. Also of interest are articles on the transport of ions and electrons in solids whenever these processes are relevant to electrochemical reactions and on the use of solid-state electrochemical reactions in the analysis of solids and their surfaces.
The journal covers solid-state electrochemistry and focusses on the following fields: mechanisms of solid-state electrochemical reactions, semiconductor electrochemistry, electrochemical batteries, accumulators and fuel cells, electrochemical mineral leaching, galvanic metal plating, electrochemical potential memory devices, solid-state electrochemical sensors, ion and electron transport in solid materials and polymers, electrocatalysis, photoelectrochemistry, corrosion of solid materials, solid-state electroanalysis, electrochemical machining of materials, electrochromism and electrochromic devices, new electrochemical solid-state synthesis.
The Journal of Solid State Electrochemistry makes the professional in research and industry aware of this swift progress and its importance for future developments and success in the above-mentioned fields.
求助内容：
应助结果提醒方式：
京公网安备 11010802042870号
