{"title":"多功能柔性大米淀粉-氧化石墨烯生物纳米复合材料","authors":"Prathmesh Bhadane and Abhijit Mishra","doi":"10.1039/D4EW00419A","DOIUrl":null,"url":null,"abstract":"<p >In light of the pressing challenge of global plastic and water pollution, this study seeks a single solution by exploring the remarkable potential of rice starch (RS)–graphene oxide (GO) bio-nanocomposite films. RS–GO composite films were prepared with varying GO concentrations. As the GO weight percentage was increased from 0 wt% to 1 wt% of starch, the ultimate tensile strength of the composite was seen to increase by 438%, whereas a marginal decrease of 29% in elongation was observed. Reinforcement of GO into the starch film also helped to enhance the melting temperature because of the strong hydrogen bond formation between RS and GO sheets. Apart from the enhanced mechanical and thermal stability of the prepared composite films, they also exhibited antibacterial properties against both Gram-positive and Gram-negative bacterial strains, encouraging their use in food packaging and storage industries. In addition, the use of RS–GO biocomposites as adsorbent materials for lead removal from wastewater was also explored. As the GO concentration was increased in the composite film, the Pb(<small>II</small>) ion removal efficiency (RE) also increased, with a maximum RE of 99% observed for 5 wt% GO film from 10 ppm Pb(<small>II</small>) water solution. In conclusion, the ability of RS–GO bio-nanocomposites to address plastic and water pollution adds to their value as eco-friendly materials.</p>","PeriodicalId":3,"journal":{"name":"ACS Applied Electronic Materials","volume":null,"pages":null},"PeriodicalIF":4.3000,"publicationDate":"2024-07-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Versatile, flexible rice starch–graphene oxide bio-nanocomposites†\",\"authors\":\"Prathmesh Bhadane and Abhijit Mishra\",\"doi\":\"10.1039/D4EW00419A\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >In light of the pressing challenge of global plastic and water pollution, this study seeks a single solution by exploring the remarkable potential of rice starch (RS)–graphene oxide (GO) bio-nanocomposite films. RS–GO composite films were prepared with varying GO concentrations. As the GO weight percentage was increased from 0 wt% to 1 wt% of starch, the ultimate tensile strength of the composite was seen to increase by 438%, whereas a marginal decrease of 29% in elongation was observed. Reinforcement of GO into the starch film also helped to enhance the melting temperature because of the strong hydrogen bond formation between RS and GO sheets. Apart from the enhanced mechanical and thermal stability of the prepared composite films, they also exhibited antibacterial properties against both Gram-positive and Gram-negative bacterial strains, encouraging their use in food packaging and storage industries. In addition, the use of RS–GO biocomposites as adsorbent materials for lead removal from wastewater was also explored. As the GO concentration was increased in the composite film, the Pb(<small>II</small>) ion removal efficiency (RE) also increased, with a maximum RE of 99% observed for 5 wt% GO film from 10 ppm Pb(<small>II</small>) water solution. In conclusion, the ability of RS–GO bio-nanocomposites to address plastic and water pollution adds to their value as eco-friendly materials.</p>\",\"PeriodicalId\":3,\"journal\":{\"name\":\"ACS Applied Electronic Materials\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":4.3000,\"publicationDate\":\"2024-07-10\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Electronic Materials\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://pubs.rsc.org/en/content/articlelanding/2024/ew/d4ew00419a\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, ELECTRICAL & ELECTRONIC\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Electronic Materials","FirstCategoryId":"93","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2024/ew/d4ew00419a","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ELECTRICAL & ELECTRONIC","Score":null,"Total":0}
引用次数: 0
摘要
鉴于全球塑料和水污染的紧迫挑战,本研究通过探索大米淀粉(RS)-氧化石墨烯(GO)生物纳米复合薄膜的巨大潜力,寻求一种独特的解决方案。研究人员使用不同浓度的 GO 制备了 RS-GO 复合薄膜。随着 GO 在淀粉中的重量百分比从 0 wt.% 增加到 1 wt.%,复合材料的极限拉伸强度增加了 438%,而伸长率则略微下降了 29%。在淀粉膜中添加 GO 还有助于提高熔化温度,因为 RS 和 GO 片之间形成了牢固的氢键。所制备的复合薄膜除了具有更高的机械稳定性和热稳定性外,还对革兰氏阳性和革兰氏阴性细菌菌株具有抗菌性能,因此可用于食品包装和储存行业。此外,还探索了 RS-GO 生物复合材料作为吸附材料用于去除废水中的铅。随着复合薄膜中 GO 浓度的增加,Pb(II) 离子的去除率(RE)也随之增加,从 10 ppm Pb(II) 水溶液中去除 5 wt.% GO 薄膜的 RE 最高可达 99%。总之,RS-GO 生物纳米复合材料解决塑料和水污染问题的能力增加了其作为生态友好材料的价值。
In light of the pressing challenge of global plastic and water pollution, this study seeks a single solution by exploring the remarkable potential of rice starch (RS)–graphene oxide (GO) bio-nanocomposite films. RS–GO composite films were prepared with varying GO concentrations. As the GO weight percentage was increased from 0 wt% to 1 wt% of starch, the ultimate tensile strength of the composite was seen to increase by 438%, whereas a marginal decrease of 29% in elongation was observed. Reinforcement of GO into the starch film also helped to enhance the melting temperature because of the strong hydrogen bond formation between RS and GO sheets. Apart from the enhanced mechanical and thermal stability of the prepared composite films, they also exhibited antibacterial properties against both Gram-positive and Gram-negative bacterial strains, encouraging their use in food packaging and storage industries. In addition, the use of RS–GO biocomposites as adsorbent materials for lead removal from wastewater was also explored. As the GO concentration was increased in the composite film, the Pb(II) ion removal efficiency (RE) also increased, with a maximum RE of 99% observed for 5 wt% GO film from 10 ppm Pb(II) water solution. In conclusion, the ability of RS–GO bio-nanocomposites to address plastic and water pollution adds to their value as eco-friendly materials.