与等离子拓扑边缘态强耦合介导的长程分子能量转移

IF 6.5 2区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Álvaro Buendía, José A. Sánchez-Gil, Vincenzo Giannini, William L. Barnes, Marie S. Rider
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引用次数: 0

摘要

光与分子物质之间的强耦合目前在化学和物理学中都引起了人们的兴趣,在分子偏振光学领域发展迅速。质子表面电场的近场增强效应及其高度可调性使金属纳米粒子阵列成为实现和控制强耦合的有趣平台。二维质子阵列每个单元有多个纳米粒子,具有晶体对称性,可以承载拓扑边角态。在此,我们利用耦合偶极子框架(包括长程相互作用)探索分子材料与这些边缘态的耦合。我们研究了弱耦合和强耦合两种情况,并证明拓扑边缘态耦合可用于增强分子间的高定向长程能量转移。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Long-range molecular energy transfer mediated by strong coupling to plasmonic topological edge states
Strong coupling between light and molecular matter is currently attracting interest both in chemistry and physics, in the fast-growing field of molecular polaritonics. The large near-field enhancement of the electric field of plasmonic surfaces and their high tunability make arrays of metallic nanoparticles an interesting platform to achieve and control strong coupling. Two dimensional plasmonic arrays with several nanoparticles per unit cell and crystalline symmetries can host topological edge and corner states. Here we explore the coupling of molecular materials to these edge states using a coupled-dipole framework including long-range interactions. We study both the weak and strong coupling regimes and demonstrate that coupling to topological edge states can be employed to enhance highly-directional long-range energy transfer between molecules.
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来源期刊
Nanophotonics
Nanophotonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
13.50
自引率
6.70%
发文量
358
审稿时长
7 weeks
期刊介绍: Nanophotonics, published in collaboration with Sciencewise, is a prestigious journal that showcases recent international research results, notable advancements in the field, and innovative applications. It is regarded as one of the leading publications in the realm of nanophotonics and encompasses a range of article types including research articles, selectively invited reviews, letters, and perspectives. The journal specifically delves into the study of photon interaction with nano-structures, such as carbon nano-tubes, nano metal particles, nano crystals, semiconductor nano dots, photonic crystals, tissue, and DNA. It offers comprehensive coverage of the most up-to-date discoveries, making it an essential resource for physicists, engineers, and material scientists.
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