Goutam Choudhury, Karoline Block, Mahnoosh Haghighatnasab, Johannes Quaas, Tom Goren, Matthias Tesche
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Comparisons with existing literature demonstrate that these datasets effectively bound the regionally observed CCN concentrations, with CALIOP typically representing the upper bound and CAMS the lower bound. Monthly and annual variations in CCN concentrations obtained from the two datasets largely agree over the Northern Hemisphere and align with previously reported variations. However, inconsistencies emerge over pristine oceans, particularly in the Southern Hemisphere, where the datasets show not only opposing seasonal changes but also contrasting annual trends. A closure study of trends in CCN and cloud droplet concentrations suggests that dust-influenced and pristine-maritime environments primarily limit our current understanding of CCN-cloud-droplet relationships. Long-term CCN observations in these regions are crucial for improving global datasets and advancing our understanding of aerosol-cloud interactions.","PeriodicalId":8611,"journal":{"name":"Atmospheric Chemistry and Physics","volume":"692 1","pages":""},"PeriodicalIF":5.2000,"publicationDate":"2024-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Pristine oceans control the uncertainty in aerosol–cloud interactions\",\"authors\":\"Goutam Choudhury, Karoline Block, Mahnoosh Haghighatnasab, Johannes Quaas, Tom Goren, Matthias Tesche\",\"doi\":\"10.5194/egusphere-2024-1863\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<strong>Abstract.</strong> Quantifying global cloud condensation nuclei (CCN) concentrations is crucial for reducing uncertainties in radiative forcing resulting from aerosol-cloud interactions. This study analyzes two novel, independent, open-source global CCN datasets derived from spaceborne Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP) measurements and Copernicus Atmosphere Monitoring Service (CAMS) reanalysis and examines the spatio-temporal variability of CCN concentrations pertinent to liquid clouds. The results reveal consistent large-scale patterns in both CALIOP and CAMS datasets, although CALIOP values are approximately 79 % higher than those from CAMS. Comparisons with existing literature demonstrate that these datasets effectively bound the regionally observed CCN concentrations, with CALIOP typically representing the upper bound and CAMS the lower bound. Monthly and annual variations in CCN concentrations obtained from the two datasets largely agree over the Northern Hemisphere and align with previously reported variations. However, inconsistencies emerge over pristine oceans, particularly in the Southern Hemisphere, where the datasets show not only opposing seasonal changes but also contrasting annual trends. A closure study of trends in CCN and cloud droplet concentrations suggests that dust-influenced and pristine-maritime environments primarily limit our current understanding of CCN-cloud-droplet relationships. 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Pristine oceans control the uncertainty in aerosol–cloud interactions
Abstract. Quantifying global cloud condensation nuclei (CCN) concentrations is crucial for reducing uncertainties in radiative forcing resulting from aerosol-cloud interactions. This study analyzes two novel, independent, open-source global CCN datasets derived from spaceborne Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP) measurements and Copernicus Atmosphere Monitoring Service (CAMS) reanalysis and examines the spatio-temporal variability of CCN concentrations pertinent to liquid clouds. The results reveal consistent large-scale patterns in both CALIOP and CAMS datasets, although CALIOP values are approximately 79 % higher than those from CAMS. Comparisons with existing literature demonstrate that these datasets effectively bound the regionally observed CCN concentrations, with CALIOP typically representing the upper bound and CAMS the lower bound. Monthly and annual variations in CCN concentrations obtained from the two datasets largely agree over the Northern Hemisphere and align with previously reported variations. However, inconsistencies emerge over pristine oceans, particularly in the Southern Hemisphere, where the datasets show not only opposing seasonal changes but also contrasting annual trends. A closure study of trends in CCN and cloud droplet concentrations suggests that dust-influenced and pristine-maritime environments primarily limit our current understanding of CCN-cloud-droplet relationships. Long-term CCN observations in these regions are crucial for improving global datasets and advancing our understanding of aerosol-cloud interactions.
期刊介绍:
Atmospheric Chemistry and Physics (ACP) is a not-for-profit international scientific journal dedicated to the publication and public discussion of high-quality studies investigating the Earth''s atmosphere and the underlying chemical and physical processes. It covers the altitude range from the land and ocean surface up to the turbopause, including the troposphere, stratosphere, and mesosphere.
The main subject areas comprise atmospheric modelling, field measurements, remote sensing, and laboratory studies of gases, aerosols, clouds and precipitation, isotopes, radiation, dynamics, biosphere interactions, and hydrosphere interactions. The journal scope is focused on studies with general implications for atmospheric science rather than investigations that are primarily of local or technical interest.