{"title":"显示法布里-佩罗激光的柔性防水竹节状包覆过氧化物聚合物纳米/微纤维","authors":"Hsin-Ming Cheng, You-Jia Pang, Chia-Kai Lin, Sheng‐Chan Wu, Bo-Zhu You, Jung‐Yao Chen, Hsu-Cheng Hsu","doi":"10.1063/5.0200465","DOIUrl":null,"url":null,"abstract":"Methylammonium lead bromide perovskite (MAPbBr3)-embedded nano- and micro-fibers are successfully fabricated by using the uniaxial electrospinning technique. Through the study of solidification and coordination between perovskite with hybrid polymers, polymethyl methacrylate, and polyacrylonitrile, the bamboo-like perovskite-embedded polymer nano/microfibers are unpredictably formed. Encapsulated in polymer, the passive perovskite-embedded polymer fibers exhibit a long-term fluorescence performance when simultaneously exposed to both water immersion and short-wavelength laser irradiation. Notably, due to the efficient gain media, the perovskite-rich region of the electrospun fiber can act as an optical microcavity. Multi-mode and single-mode lasing behaviors can be achieved via different cavity lengths. The mechanism of a microlaser within this perovskite fiber is confirmed through a Fabry–Pérot cavity, which provides an opportunity for optical components in lasers.","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":"71 4","pages":""},"PeriodicalIF":8.3000,"publicationDate":"2024-06-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Flexible water-resistant bamboo-like perovskite-embedded polymer nano/microfibers exhibiting Fabry–Pérot lasing\",\"authors\":\"Hsin-Ming Cheng, You-Jia Pang, Chia-Kai Lin, Sheng‐Chan Wu, Bo-Zhu You, Jung‐Yao Chen, Hsu-Cheng Hsu\",\"doi\":\"10.1063/5.0200465\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Methylammonium lead bromide perovskite (MAPbBr3)-embedded nano- and micro-fibers are successfully fabricated by using the uniaxial electrospinning technique. Through the study of solidification and coordination between perovskite with hybrid polymers, polymethyl methacrylate, and polyacrylonitrile, the bamboo-like perovskite-embedded polymer nano/microfibers are unpredictably formed. Encapsulated in polymer, the passive perovskite-embedded polymer fibers exhibit a long-term fluorescence performance when simultaneously exposed to both water immersion and short-wavelength laser irradiation. Notably, due to the efficient gain media, the perovskite-rich region of the electrospun fiber can act as an optical microcavity. Multi-mode and single-mode lasing behaviors can be achieved via different cavity lengths. The mechanism of a microlaser within this perovskite fiber is confirmed through a Fabry–Pérot cavity, which provides an opportunity for optical components in lasers.\",\"PeriodicalId\":5,\"journal\":{\"name\":\"ACS Applied Materials & Interfaces\",\"volume\":\"71 4\",\"pages\":\"\"},\"PeriodicalIF\":8.3000,\"publicationDate\":\"2024-06-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Materials & Interfaces\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1063/5.0200465\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Materials & Interfaces","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1063/5.0200465","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Methylammonium lead bromide perovskite (MAPbBr3)-embedded nano- and micro-fibers are successfully fabricated by using the uniaxial electrospinning technique. Through the study of solidification and coordination between perovskite with hybrid polymers, polymethyl methacrylate, and polyacrylonitrile, the bamboo-like perovskite-embedded polymer nano/microfibers are unpredictably formed. Encapsulated in polymer, the passive perovskite-embedded polymer fibers exhibit a long-term fluorescence performance when simultaneously exposed to both water immersion and short-wavelength laser irradiation. Notably, due to the efficient gain media, the perovskite-rich region of the electrospun fiber can act as an optical microcavity. Multi-mode and single-mode lasing behaviors can be achieved via different cavity lengths. The mechanism of a microlaser within this perovskite fiber is confirmed through a Fabry–Pérot cavity, which provides an opportunity for optical components in lasers.
期刊介绍:
ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.