Anna Zawadzka , Agnieszka Marjanowska , Amina Laouid , Krzysztof Wisniewski , Youssef El Kouari , Youssef El Hani , Przemysław Płóciennik
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Then, using spectroscopic techniques, the characteristics of the layers' optical and electrical properties were determined. The obtained results allowed the design of the complete structure of a thin-film perovskite cell, which was made using only the vacuum sublimation process. Simulations using the SCAPS-1D program and experimental results showed high agreement and allowed for obtaining an efficiency of approximately 18.5 % in the interested temperature range. Perovskite solar cell stability tests over six months confirmed the positive impact of the proposed technique for depositing the complete cell structure on its temporal stability. 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Perovskite solar cell stability tests over six months confirmed the positive impact of the proposed technique for depositing the complete cell structure on its temporal stability. 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引用次数: 0
摘要
本出版物中讨论的研究旨在开发一种适合在低温低压条件下工作、厚度小于 1 μm 的过氧化物太阳能电池。该研究提出了物理气相共沉积技术,并成功地将其用于制造以混合包晶石薄层作为能量收集材料的太阳能电池结构。为实施该项目,对甲基碘化铅铵盐在 10 K 至 320 K 宽温度范围内的行为进行了全面分析。初始阶段包括评估过氧化物晶材料层在冷却到液氦温度后的降解情况,然后再将其重新加热到室温。然后,利用光谱技术确定了材料层的光学和电学特性。根据所获得的结果,设计出了仅使用真空升华工艺制作的薄膜过氧化物电池的完整结构。使用 SCAPS-1D 程序进行的模拟与实验结果显示出高度一致,在相关温度范围内可获得约 18.5 % 的效率。历时六个月的 Perovskite 太阳能电池稳定性测试证实,所提出的沉积完整电池结构的技术对其时间稳定性产生了积极影响。这些研究成果为在太空中应用包晶石电池提供了乐观的前景。
Low-temperature influence on the properties and efficiency of thin-film perovskite solar cells fabricated by the PVco-D technique
The study discussed in this publication aimed to develop a perovskite solar cell adapted to operating conditions at reduced temperature and pressure and less than 1 μm thick. The physical vapor co-deposition technique was proposed and successfully used to create a solar cell structure with a thin layer of hybrid perovskite as an energy-collecting material. A comprehensive analysis of methylammonium lead iodide behavior in a wide temperature range from 10 K to 320 K was carried out to implement this project. The initial phase included assessing the degradation of the perovskite material layer after cooling to the temperature of liquid helium and then re-heating it to room temperature. Then, using spectroscopic techniques, the characteristics of the layers' optical and electrical properties were determined. The obtained results allowed the design of the complete structure of a thin-film perovskite cell, which was made using only the vacuum sublimation process. Simulations using the SCAPS-1D program and experimental results showed high agreement and allowed for obtaining an efficiency of approximately 18.5 % in the interested temperature range. Perovskite solar cell stability tests over six months confirmed the positive impact of the proposed technique for depositing the complete cell structure on its temporal stability. The research results are optimistic for the applications of perovskite cells in space.
期刊介绍:
Solar Energy Materials & Solar Cells is intended as a vehicle for the dissemination of research results on materials science and technology related to photovoltaic, photothermal and photoelectrochemical solar energy conversion. Materials science is taken in the broadest possible sense and encompasses physics, chemistry, optics, materials fabrication and analysis for all types of materials.