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引用次数: 0
摘要
将二氧化碳转化为高价值的燃料和化学品已引起全世界的研究兴趣。二氧化碳的转化和利用已成为社会最紧迫的任务之一。在此背景下，利用太阳能将 CO2 转化为 CH4 和 CH3OH 等高价值燃料具有极高的潜在应用价值。本文综述了利用各种新型催化剂光催化还原二氧化碳的研究进展和成果。此外，还综述了提高光催化性能的策略。最后，通过对反应机理的全面探索，提出了改进催化剂催化机理和设计新型高活性、高稳定性催化剂的建议，以满足未来工业生产的要求。
Developments and challenges on enhancement of photocatalytic CO2 reduction through photocatalysis
The conversion of CO2 into high-value fuels and chemicals has garnered research interest worldwide. The conversion and utilization of CO2 has become one of the most urgent tasks for society. In this context, using solar energy to convert CO2 into high-value fuels such as CH4 and CH3OH has extremely high potential application value. Herein, the research progress and results of applying various photocatalysts in photocatalytic CO2 reduction with various novel catalysts were reviewed. Furthermore, strategies for improving photocatalytic performance were reviewed. Finally, improving the catalytic mechanism of catalysts and designing novel high-activity, high-stability catalysts through comprehensive exploration of the reaction mechanism were suggested to meet the future requirements of industrial production.
期刊介绍：
Carbon Resources Conversion (CRC) publishes fundamental studies and industrial developments regarding relevant technologies aiming for the clean, efficient, value-added, and low-carbon utilization of carbon-containing resources as fuel for energy and as feedstock for materials or chemicals from, for example, fossil fuels, biomass, syngas, CO2, hydrocarbons, and organic wastes via physical, thermal, chemical, biological, and other technical methods. CRC also publishes scientific and engineering studies on resource characterization and pretreatment, carbon material innovation and production, clean technologies related to carbon resource conversion and utilization, and various process-supporting technologies, including on-line or off-line measurement and monitoring, modeling, simulations focused on safe and efficient process operation and control, and process and equipment optimization.
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