{"title":"石墨烯、硅和硅基材料的合成与结构设计,包括加入石墨烯作为阳极以提高锂离子电池的电化学性能","authors":"Jawad Reslan, Mohamed Saadaoui, Thierry Djenizian","doi":"10.1002/admi.202301062","DOIUrl":null,"url":null,"abstract":"<p>Silicon emerges as a candidate for advancing lithium ion batteries with important roles in various applications ranging from portable electronics to electric vehicles. However, despite its theoretical capacities silicon faces challenges such as unstable cycling and limited rate performance. This thorough review examines developments in improving the electrochemical performance of silicon and graphene within the context of lithium ion batteries. The focus lies on strategies for designing and synthesizing composite materials that incorporate silicon particularly when combined with graphene. Structural aspects like particle size, morphology and porosity are carefully optimized to harness the potential of silicon based anodes and graphene. The review highlights the effects resulting from these tailored design approaches, including key factors such as capacity retention, cycling stability and rate capability of the resulting anode materials. By exploring these design paradigms this review offers a comprehensive perspective on the transformative capabilities of silicon, graphene and silicon/graphene composites. It does not highlights recent advancements but also outlines future directions for innovation and practical applications. This compilation of progress contributes to the understanding of how silicon based anodes, in lithium ion batteries have evolved from small-scale implementations to catalyzing advancements in energy utilization.</p>","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":null,"pages":null},"PeriodicalIF":4.3000,"publicationDate":"2024-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202301062","citationCount":"0","resultStr":"{\"title\":\"Synthesis and Structural Design of Graphene, Silicon and Silicon-Based Materials Including Incorporation of Graphene as Anode to Improve Electrochemical Performance in Lithium-Ion Batteries\",\"authors\":\"Jawad Reslan, Mohamed Saadaoui, Thierry Djenizian\",\"doi\":\"10.1002/admi.202301062\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Silicon emerges as a candidate for advancing lithium ion batteries with important roles in various applications ranging from portable electronics to electric vehicles. However, despite its theoretical capacities silicon faces challenges such as unstable cycling and limited rate performance. This thorough review examines developments in improving the electrochemical performance of silicon and graphene within the context of lithium ion batteries. The focus lies on strategies for designing and synthesizing composite materials that incorporate silicon particularly when combined with graphene. Structural aspects like particle size, morphology and porosity are carefully optimized to harness the potential of silicon based anodes and graphene. The review highlights the effects resulting from these tailored design approaches, including key factors such as capacity retention, cycling stability and rate capability of the resulting anode materials. By exploring these design paradigms this review offers a comprehensive perspective on the transformative capabilities of silicon, graphene and silicon/graphene composites. It does not highlights recent advancements but also outlines future directions for innovation and practical applications. This compilation of progress contributes to the understanding of how silicon based anodes, in lithium ion batteries have evolved from small-scale implementations to catalyzing advancements in energy utilization.</p>\",\"PeriodicalId\":115,\"journal\":{\"name\":\"Advanced Materials Interfaces\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":4.3000,\"publicationDate\":\"2024-06-03\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202301062\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advanced Materials Interfaces\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://onlinelibrary.wiley.com/doi/10.1002/admi.202301062\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Materials Interfaces","FirstCategoryId":"88","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/admi.202301062","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Synthesis and Structural Design of Graphene, Silicon and Silicon-Based Materials Including Incorporation of Graphene as Anode to Improve Electrochemical Performance in Lithium-Ion Batteries
Silicon emerges as a candidate for advancing lithium ion batteries with important roles in various applications ranging from portable electronics to electric vehicles. However, despite its theoretical capacities silicon faces challenges such as unstable cycling and limited rate performance. This thorough review examines developments in improving the electrochemical performance of silicon and graphene within the context of lithium ion batteries. The focus lies on strategies for designing and synthesizing composite materials that incorporate silicon particularly when combined with graphene. Structural aspects like particle size, morphology and porosity are carefully optimized to harness the potential of silicon based anodes and graphene. The review highlights the effects resulting from these tailored design approaches, including key factors such as capacity retention, cycling stability and rate capability of the resulting anode materials. By exploring these design paradigms this review offers a comprehensive perspective on the transformative capabilities of silicon, graphene and silicon/graphene composites. It does not highlights recent advancements but also outlines future directions for innovation and practical applications. This compilation of progress contributes to the understanding of how silicon based anodes, in lithium ion batteries have evolved from small-scale implementations to catalyzing advancements in energy utilization.
期刊介绍:
Advanced Materials Interfaces publishes top-level research on interface technologies and effects. Considering any interface formed between solids, liquids, and gases, the journal ensures an interdisciplinary blend of physics, chemistry, materials science, and life sciences. Advanced Materials Interfaces was launched in 2014 and received an Impact Factor of 4.834 in 2018.
The scope of Advanced Materials Interfaces is dedicated to interfaces and surfaces that play an essential role in virtually all materials and devices. Physics, chemistry, materials science and life sciences blend to encourage new, cross-pollinating ideas, which will drive forward our understanding of the processes at the interface.
Advanced Materials Interfaces covers all topics in interface-related research:
Oil / water separation,
Applications of nanostructured materials,
2D materials and heterostructures,
Surfaces and interfaces in organic electronic devices,
Catalysis and membranes,
Self-assembly and nanopatterned surfaces,
Composite and coating materials,
Biointerfaces for technical and medical applications.
Advanced Materials Interfaces provides a forum for topics on surface and interface science with a wide choice of formats: Reviews, Full Papers, and Communications, as well as Progress Reports and Research News.