{"title":"MOF 衍生的 LDHs:揭示其在氧气进化反应中的潜力","authors":"Mohammad Etesami , Shiva Rezaei Motlagh , Ramin Khezri , Mohan Gopalakrishnan , Jayaraman Theerthagiri , Myong Yong Choi , Kasidit Nootong , Anongnat Somwangthanaroj , Soorathep Kheawhom","doi":"10.1016/j.enchem.2024.100128","DOIUrl":null,"url":null,"abstract":"<div><p>This review explores the potential of metal-organic frameworks (MOFs) to drive sustainable clean energy solutions and their crucial role in transitioning towards a decarbonized global economy. The paper underscores the remarkable versatility and modifiability of MOFs. Central to this discourse is the conversion of MOFs into layered double hydroxides (LDHs), with a detailed exposition of the synthesis methodologies and their consequential effects on catalytic efficacy. A meticulous evaluation of MOF-derived LDHs is presented, particularly in the context of the oxygen evolution reaction (OER), encapsulating cutting-edge progress and probing the feasibility of integrating these materials into next-generation energy technologies. Diverging from existing literature, this research provides an in-depth exploration of MOF-to-LDH conversion, a promising area in OER catalysis. In addition, structural engineering techniques to optimize the performance of MOF-derived LDHs in electrochemical devices are explored, highlighting the potential of MOFs as future electrocatalysts and guiding future research directions.</p></div>","PeriodicalId":307,"journal":{"name":"EnergyChem","volume":"6 4","pages":"Article 100128"},"PeriodicalIF":22.2000,"publicationDate":"2024-05-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"MOF-derived LDHs: Unveiling their potential in oxygen evolution reaction\",\"authors\":\"Mohammad Etesami , Shiva Rezaei Motlagh , Ramin Khezri , Mohan Gopalakrishnan , Jayaraman Theerthagiri , Myong Yong Choi , Kasidit Nootong , Anongnat Somwangthanaroj , Soorathep Kheawhom\",\"doi\":\"10.1016/j.enchem.2024.100128\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>This review explores the potential of metal-organic frameworks (MOFs) to drive sustainable clean energy solutions and their crucial role in transitioning towards a decarbonized global economy. The paper underscores the remarkable versatility and modifiability of MOFs. Central to this discourse is the conversion of MOFs into layered double hydroxides (LDHs), with a detailed exposition of the synthesis methodologies and their consequential effects on catalytic efficacy. A meticulous evaluation of MOF-derived LDHs is presented, particularly in the context of the oxygen evolution reaction (OER), encapsulating cutting-edge progress and probing the feasibility of integrating these materials into next-generation energy technologies. Diverging from existing literature, this research provides an in-depth exploration of MOF-to-LDH conversion, a promising area in OER catalysis. In addition, structural engineering techniques to optimize the performance of MOF-derived LDHs in electrochemical devices are explored, highlighting the potential of MOFs as future electrocatalysts and guiding future research directions.</p></div>\",\"PeriodicalId\":307,\"journal\":{\"name\":\"EnergyChem\",\"volume\":\"6 4\",\"pages\":\"Article 100128\"},\"PeriodicalIF\":22.2000,\"publicationDate\":\"2024-05-31\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"EnergyChem\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2589778024000125\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"EnergyChem","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2589778024000125","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
MOF-derived LDHs: Unveiling their potential in oxygen evolution reaction
This review explores the potential of metal-organic frameworks (MOFs) to drive sustainable clean energy solutions and their crucial role in transitioning towards a decarbonized global economy. The paper underscores the remarkable versatility and modifiability of MOFs. Central to this discourse is the conversion of MOFs into layered double hydroxides (LDHs), with a detailed exposition of the synthesis methodologies and their consequential effects on catalytic efficacy. A meticulous evaluation of MOF-derived LDHs is presented, particularly in the context of the oxygen evolution reaction (OER), encapsulating cutting-edge progress and probing the feasibility of integrating these materials into next-generation energy technologies. Diverging from existing literature, this research provides an in-depth exploration of MOF-to-LDH conversion, a promising area in OER catalysis. In addition, structural engineering techniques to optimize the performance of MOF-derived LDHs in electrochemical devices are explored, highlighting the potential of MOFs as future electrocatalysts and guiding future research directions.
期刊介绍:
EnergyChem, a reputable journal, focuses on publishing high-quality research and review articles within the realm of chemistry, chemical engineering, and materials science with a specific emphasis on energy applications. The priority areas covered by the journal include:Solar energy,Energy harvesting devices,Fuel cells,Hydrogen energy,Bioenergy and biofuels,Batteries,Supercapacitors,Electrocatalysis and photocatalysis,Energy storage and energy conversion,Carbon capture and storage