气固上升器和下降器反应器中高速射流的混合效应

IF 4.1 2区 材料科学 Q2 ENGINEERING, CHEMICAL
Zihan Yan, Dongdong Wang, Lining Wu, Chunxi Lu
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引用次数: 0

摘要

对于高温和短接触时间的气固反应过程,升流器和降流器被认为是合适的反应器。为了实现反应物与催化剂的密集和完全混合,原料总是以高速射流的形式引入。在本研究中,为了研究不同类型的高速射流在立管和沉降器中的混合效果,在高速进料射流中注入了可追踪的臭氧,使其与催化剂颗粒发生反应。通过检测臭氧的分解,分析了在同流喷射和逆流喷射的影响下,立管和下流器中的气固混合和反应情况。利用相对臭氧浓度来反映位置反应范围,并提出其径向不均匀性指数来比较立管和下管的结果。研究发现,下流器中的射流影响区为进料射流与催化剂的混合提供了相对较好的环境。在立管中,引入逆流喷射可改善进料与催化剂初始接触区域的气固混合均匀性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Mixing effects of high-speed jets in gas-solid riser and downer reactors

Mixing effects of high-speed jets in gas-solid riser and downer reactors

For the high-temperature and short-contact time gas-solid reaction process, riser and downer are considered appropriate reactors. To realize an intensive and complete mixing of reactants with catalysts, the feed raw is always introduced in the form of high-speed jets. In this study, in order to investigate the mixing effects of different types of high-speed jets in riser and downer, traceable ozone is injected with the high-speed feed jets to react with catalyst particles. By detecting the decomposition of ozone, the gas-solid mixing and reaction in riser and downer under the influence of both co-current and counter-current injections are analyzed. The relative ozone concentration is used to reflect the location reaction extent and its radial nonuniformity index is proposed to compare the results in riser and downer. It is found that the jet influence zone in downer provides a relatively better environment for the mixing of feed jets with catalysts. In the riser, introduction of counter-current injections could improve the uniformity of gas-solid mixing in the initial contact region of feed with catalysts.

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来源期刊
Particuology
Particuology 工程技术-材料科学:综合
CiteScore
6.70
自引率
2.90%
发文量
1730
审稿时长
32 days
期刊介绍: The word ‘particuology’ was coined to parallel the discipline for the science and technology of particles. Particuology is an interdisciplinary journal that publishes frontier research articles and critical reviews on the discovery, formulation and engineering of particulate materials, processes and systems. It especially welcomes contributions utilising advanced theoretical, modelling and measurement methods to enable the discovery and creation of new particulate materials, and the manufacturing of functional particulate-based products, such as sensors. Papers are handled by Thematic Editors who oversee contributions from specific subject fields. These fields are classified into: Particle Synthesis and Modification; Particle Characterization and Measurement; Granular Systems and Bulk Solids Technology; Fluidization and Particle-Fluid Systems; Aerosols; and Applications of Particle Technology. Key topics concerning the creation and processing of particulates include: -Modelling and simulation of particle formation, collective behaviour of particles and systems for particle production over a broad spectrum of length scales -Mining of experimental data for particle synthesis and surface properties to facilitate the creation of new materials and processes -Particle design and preparation including controlled response and sensing functionalities in formation, delivery systems and biological systems, etc. -Experimental and computational methods for visualization and analysis of particulate system. These topics are broadly relevant to the production of materials, pharmaceuticals and food, and to the conversion of energy resources to fuels and protection of the environment.
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