利用石英晶体微天平探索金属电镀储能技术:综述

Viktor Vanoppen, Diethelm Johannsmann, Xu Hou, Jens Sjölund, Peter Broqvist, Erik J. Berg
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引用次数: 0

摘要

本文回顾了电化学石英晶体微天平 (EQCM) 传感在研究金属电镀(尤其是用于储能目的)方面的发展和应用。探讨了 EQCM 在描述电极/电解质界面动力学方面的作用,例如电双层堆积、离子/分子吸附、金属成核和生长。介绍了 QCM 传感器的建模,并强调了其重要性。综述了使用金属电极所面临的挑战,包括副反应和枝晶的形成及其缓解策略。讨论了影响电镀过程的众多因素,如电解液成分、添加剂、温度和电流密度,以及它们对电镀金属的质量、结构和机械特性的影响。展望未来,我们强调有必要加深对电镀金属纳米结构所产生的 QCM 信号响应的基本理解并推进模拟。进一步开发和整合创新的 EQCM 策略将为从根本上理解和优化金属电镀的能量存储和应用提供独特的未来手段。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Exploring Metal Electroplating for Energy Storage by Quartz Crystal Microbalance: A Review

Exploring Metal Electroplating for Energy Storage by Quartz Crystal Microbalance: A Review

The development and application of Electrochemical Quartz Crystal Microbalance (EQCM) sensing to study metal electroplating, especially for energy storage purposes, are reviewed. The roles of EQCM in describing electrode/electrolyte interface dynamics, such as the electric double-layer build-up, ionic/molecular adsorption, metal nucleation, and growth, are addressed. Modeling of the QCM sensor is introduced and its importance is emphasized. Challenges of metal electrode use, including side reactions and dendrite formation, along with their mitigation strategies are reviewed. Numerous factors affecting the electroplating processes, such as electrolyte composition, additives, temperature, and current density, and their influence on the electroplated metals’ mass, structural, and mechanical characteristics are discussed. Looking forward, the need for deeper fundamental understanding and advancing simulations of the QCM signal response as a result of electroplating metal nanostructures is stressed. Further development and integration of innovative EQCM-strategies will provide unique future means to fundamentally understand and optimize metal electroplating for energy storage and application alike.

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