Neha Chaurasia , Rajesh K. Yadav , Shaifali Mishra , Rehana Shahin , Satyam Singh , Navneet K. Gupta , S.K. Pandey , Mantesh Kumari Yadav , Jin-OoK Baeg , Ahmad J. Obaidullah , Krishna Kumar Yadav
{"title":"熠熠生辉：掺杂 B@S 的氮化石墨碳纳米棒在可见光下催化 C-N 键形成的能力得到增强","authors":"Neha Chaurasia , Rajesh K. Yadav , Shaifali Mishra , Rehana Shahin , Satyam Singh , Navneet K. Gupta , S.K. Pandey , Mantesh Kumari Yadav , Jin-OoK Baeg , Ahmad J. Obaidullah , Krishna Kumar Yadav","doi":"10.1016/j.flatc.2024.100669","DOIUrl":null,"url":null,"abstract":"<div><p>Graphitic carbon nitride as a photocatalyst seeking attention nowadays, due to its thermal stability, band structure, and chemical properties. Herein, we reported a boron sulfur co-doped graphitic carbon nitride (B@S-g-C<sub>3</sub>N<sub>4</sub>) photocatalyst synthesized by a one-pot thermal polycondensation mechanism. However, it was observed that due to co-doping in native carbon nitride structure the photocatalytic behavior and the band structure enhanced which was capable of fascinating the demand of organic transformations i.e. photocatalytic and charge transfer capability. The synthesized B@S-g-C<sub>3</sub>N<sub>4</sub> photocatalyst was characterized by UV–vis DRS, FT-IR, XRD, SEM, EDX, HR-TEM, XPS and electrochemical properties. In addition, the synthesized B@S-g-C<sub>3</sub>N<sub>4</sub> photocatalyst is a metal-free carbon nitride photocatalyst proven to be highly effective in performing organic transformations (conversion yield 98 %) like C-N bond formation under visible light source.</p></div>","PeriodicalId":316,"journal":{"name":"FlatChem","volume":"46 ","pages":"Article 100669"},"PeriodicalIF":5.9000,"publicationDate":"2024-05-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Shining bright: B@S-codoped graphitic carbon nitride nanorods illuminate enhanced catalytic C-N bond formation under visible-light\",\"authors\":\"Neha Chaurasia , Rajesh K. Yadav , Shaifali Mishra , Rehana Shahin , Satyam Singh , Navneet K. Gupta , S.K. Pandey , Mantesh Kumari Yadav , Jin-OoK Baeg , Ahmad J. Obaidullah , Krishna Kumar Yadav\",\"doi\":\"10.1016/j.flatc.2024.100669\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Graphitic carbon nitride as a photocatalyst seeking attention nowadays, due to its thermal stability, band structure, and chemical properties. Herein, we reported a boron sulfur co-doped graphitic carbon nitride (B@S-g-C<sub>3</sub>N<sub>4</sub>) photocatalyst synthesized by a one-pot thermal polycondensation mechanism. However, it was observed that due to co-doping in native carbon nitride structure the photocatalytic behavior and the band structure enhanced which was capable of fascinating the demand of organic transformations i.e. photocatalytic and charge transfer capability. The synthesized B@S-g-C<sub>3</sub>N<sub>4</sub> photocatalyst was characterized by UV–vis DRS, FT-IR, XRD, SEM, EDX, HR-TEM, XPS and electrochemical properties. In addition, the synthesized B@S-g-C<sub>3</sub>N<sub>4</sub> photocatalyst is a metal-free carbon nitride photocatalyst proven to be highly effective in performing organic transformations (conversion yield 98 %) like C-N bond formation under visible light source.</p></div>\",\"PeriodicalId\":316,\"journal\":{\"name\":\"FlatChem\",\"volume\":\"46 \",\"pages\":\"Article 100669\"},\"PeriodicalIF\":5.9000,\"publicationDate\":\"2024-05-07\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"FlatChem\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2452262724000631\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"FlatChem","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2452262724000631","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Shining bright: B@S-codoped graphitic carbon nitride nanorods illuminate enhanced catalytic C-N bond formation under visible-light
Graphitic carbon nitride as a photocatalyst seeking attention nowadays, due to its thermal stability, band structure, and chemical properties. Herein, we reported a boron sulfur co-doped graphitic carbon nitride (B@S-g-C3N4) photocatalyst synthesized by a one-pot thermal polycondensation mechanism. However, it was observed that due to co-doping in native carbon nitride structure the photocatalytic behavior and the band structure enhanced which was capable of fascinating the demand of organic transformations i.e. photocatalytic and charge transfer capability. The synthesized B@S-g-C3N4 photocatalyst was characterized by UV–vis DRS, FT-IR, XRD, SEM, EDX, HR-TEM, XPS and electrochemical properties. In addition, the synthesized B@S-g-C3N4 photocatalyst is a metal-free carbon nitride photocatalyst proven to be highly effective in performing organic transformations (conversion yield 98 %) like C-N bond formation under visible light source.
期刊介绍：
FlatChem - Chemistry of Flat Materials, a new voice in the community, publishes original and significant, cutting-edge research related to the chemistry of graphene and related 2D & layered materials. The overall aim of the journal is to combine the chemistry and applications of these materials, where the submission of communications, full papers, and concepts should contain chemistry in a materials context, which can be both experimental and/or theoretical. In addition to original research articles, FlatChem also offers reviews, minireviews, highlights and perspectives on the future of this research area with the scientific leaders in fields related to Flat Materials. Topics of interest include, but are not limited to, the following: -Design, synthesis, applications and investigation of graphene, graphene related materials and other 2D & layered materials (for example Silicene, Germanene, Phosphorene, MXenes, Boron nitride, Transition metal dichalcogenides) -Characterization of these materials using all forms of spectroscopy and microscopy techniques -Chemical modification or functionalization and dispersion of these materials, as well as interactions with other materials -Exploring the surface chemistry of these materials for applications in: Sensors or detectors in electrochemical/Lab on a Chip devices, Composite materials, Membranes, Environment technology, Catalysis for energy storage and conversion (for example fuel cells, supercapacitors, batteries, hydrogen storage), Biomedical technology (drug delivery, biosensing, bioimaging)
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