Prof. S. A. T. Shanmugapriya, Anand Kumar, Mohd Afzal, Ratiram Gomaji Chaudhary, Kotesh Kumar Mandari, Aniruddha Mondal, Sudip Mondal
{"title":"制备高多孔片状 Fe3O4 碳纳米复合材料:电催化氧进化反应的多功能催化剂","authors":"Prof. S. A. T. Shanmugapriya, Anand Kumar, Mohd Afzal, Ratiram Gomaji Chaudhary, Kotesh Kumar Mandari, Aniruddha Mondal, Sudip Mondal","doi":"10.1002/slct.202304092","DOIUrl":null,"url":null,"abstract":"<p>Fuel cells and metal-air batteries are examples of renewable energy technologies that depend on having highly effective electrocatalysts for the oxygen evolution reaction (OER). In this study, a mesoporous nanostructure composed of Fe<sub>3</sub>O<sub>4</sub>-Carbon nanocomposites was synthesised using a simple and economically viable approach at a relatively low temperature. The observed catalytic activity of the prepared defected Fe<sub>3</sub>O<sub>4</sub>-Carbon nanocomposites mesoporous nanostructure was found to be remarkable. Additionally, the nanostructure exhibited a high tolerance to methanol and demonstrated durability towards the oxygen evolution reaction (OER) in alkaline media. In the course of the experiment, it was observed that the catalyst exhibited noteworthy activity in the Oxygen Evolution Reaction (OER) when compared to the commercially available RuO<sub>2</sub> catalyst. This was evident through a more overpotential value of 325 mV at current density of 10 mA/cm<sup>2</sup>. The catalyst‘s notable capacity for high oxygen reaction activity may potentially enhance the synergistic effect resulting from the combination of defect sites and the porous structure of Fe<sub>3</sub>O<sub>4</sub>-Carbon nanocomposites. The findings of this study indicate that the Fe<sub>3</sub>O<sub>4</sub>-Carbon nanocomposites nanostructures exhibit promising attributes as an electrocatalyst for the oxygen evolution reaction (OER) in real-world scenarios.</p>","PeriodicalId":146,"journal":{"name":"ChemistrySelect","volume":"9 15","pages":""},"PeriodicalIF":2.0000,"publicationDate":"2024-04-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Fabrication of Highly Porous and Sheet Like Fe3O4-Carbon Nanocomposites: A Versatile Catalyst for Electrocatalytic Oxygen Evolution Reactions\",\"authors\":\"Prof. S. A. T. Shanmugapriya, Anand Kumar, Mohd Afzal, Ratiram Gomaji Chaudhary, Kotesh Kumar Mandari, Aniruddha Mondal, Sudip Mondal\",\"doi\":\"10.1002/slct.202304092\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Fuel cells and metal-air batteries are examples of renewable energy technologies that depend on having highly effective electrocatalysts for the oxygen evolution reaction (OER). In this study, a mesoporous nanostructure composed of Fe<sub>3</sub>O<sub>4</sub>-Carbon nanocomposites was synthesised using a simple and economically viable approach at a relatively low temperature. The observed catalytic activity of the prepared defected Fe<sub>3</sub>O<sub>4</sub>-Carbon nanocomposites mesoporous nanostructure was found to be remarkable. Additionally, the nanostructure exhibited a high tolerance to methanol and demonstrated durability towards the oxygen evolution reaction (OER) in alkaline media. In the course of the experiment, it was observed that the catalyst exhibited noteworthy activity in the Oxygen Evolution Reaction (OER) when compared to the commercially available RuO<sub>2</sub> catalyst. This was evident through a more overpotential value of 325 mV at current density of 10 mA/cm<sup>2</sup>. The catalyst‘s notable capacity for high oxygen reaction activity may potentially enhance the synergistic effect resulting from the combination of defect sites and the porous structure of Fe<sub>3</sub>O<sub>4</sub>-Carbon nanocomposites. The findings of this study indicate that the Fe<sub>3</sub>O<sub>4</sub>-Carbon nanocomposites nanostructures exhibit promising attributes as an electrocatalyst for the oxygen evolution reaction (OER) in real-world scenarios.</p>\",\"PeriodicalId\":146,\"journal\":{\"name\":\"ChemistrySelect\",\"volume\":\"9 15\",\"pages\":\"\"},\"PeriodicalIF\":2.0000,\"publicationDate\":\"2024-04-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ChemistrySelect\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://onlinelibrary.wiley.com/doi/10.1002/slct.202304092\",\"RegionNum\":4,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ChemistrySelect","FirstCategoryId":"92","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/slct.202304092","RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Fabrication of Highly Porous and Sheet Like Fe3O4-Carbon Nanocomposites: A Versatile Catalyst for Electrocatalytic Oxygen Evolution Reactions
Fuel cells and metal-air batteries are examples of renewable energy technologies that depend on having highly effective electrocatalysts for the oxygen evolution reaction (OER). In this study, a mesoporous nanostructure composed of Fe3O4-Carbon nanocomposites was synthesised using a simple and economically viable approach at a relatively low temperature. The observed catalytic activity of the prepared defected Fe3O4-Carbon nanocomposites mesoporous nanostructure was found to be remarkable. Additionally, the nanostructure exhibited a high tolerance to methanol and demonstrated durability towards the oxygen evolution reaction (OER) in alkaline media. In the course of the experiment, it was observed that the catalyst exhibited noteworthy activity in the Oxygen Evolution Reaction (OER) when compared to the commercially available RuO2 catalyst. This was evident through a more overpotential value of 325 mV at current density of 10 mA/cm2. The catalyst‘s notable capacity for high oxygen reaction activity may potentially enhance the synergistic effect resulting from the combination of defect sites and the porous structure of Fe3O4-Carbon nanocomposites. The findings of this study indicate that the Fe3O4-Carbon nanocomposites nanostructures exhibit promising attributes as an electrocatalyst for the oxygen evolution reaction (OER) in real-world scenarios.
期刊介绍:
ChemistrySelect is the latest journal from ChemPubSoc Europe and Wiley-VCH. It offers researchers a quality society-owned journal in which to publish their work in all areas of chemistry. Manuscripts are evaluated by active researchers to ensure they add meaningfully to the scientific literature, and those accepted are processed quickly to ensure rapid online publication.