{"title":"基于过渡金属的高效硝酸盐还原电催化剂的最新进展与展望","authors":"Jun Zhou, Sanshuang Gao and Guangzhi Hu*, ","doi":"10.1021/acs.energyfuels.4c00415","DOIUrl":null,"url":null,"abstract":"<p >Electrochemical nitrate reduction is the process of converting nitrate into ammonia or nitrogen using electric energy. This saves energy, protects the environment, and is an important technology for nitrogen resource recovery and water purification. This paper examines recent advances in electrochemical nitrate reduction technology research and analyzes the reaction mechanism and path of electrochemical nitrate reduction as well as the influence of various factors on the reaction path through thermodynamic and kinetic principles. Second, the catalytic performances of transition metal electrocatalysts in the form of single metals, alloys, oxides, and composites in electrochemical nitrate reduction are analyzed in detail, which lays the foundation for the rational development of new, efficient, and stable electrocatalysts. Finally, future development directions and prospects for electrochemical nitrate reduction technology are envisioned.</p>","PeriodicalId":35,"journal":{"name":"Energy & Fuels","volume":"38 8","pages":"6701–6722"},"PeriodicalIF":5.3000,"publicationDate":"2024-04-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Recent Progress and Perspectives on Transition Metal-Based Electrocatalysts for Efficient Nitrate Reduction\",\"authors\":\"Jun Zhou, Sanshuang Gao and Guangzhi Hu*, \",\"doi\":\"10.1021/acs.energyfuels.4c00415\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Electrochemical nitrate reduction is the process of converting nitrate into ammonia or nitrogen using electric energy. This saves energy, protects the environment, and is an important technology for nitrogen resource recovery and water purification. This paper examines recent advances in electrochemical nitrate reduction technology research and analyzes the reaction mechanism and path of electrochemical nitrate reduction as well as the influence of various factors on the reaction path through thermodynamic and kinetic principles. Second, the catalytic performances of transition metal electrocatalysts in the form of single metals, alloys, oxides, and composites in electrochemical nitrate reduction are analyzed in detail, which lays the foundation for the rational development of new, efficient, and stable electrocatalysts. Finally, future development directions and prospects for electrochemical nitrate reduction technology are envisioned.</p>\",\"PeriodicalId\":35,\"journal\":{\"name\":\"Energy & Fuels\",\"volume\":\"38 8\",\"pages\":\"6701–6722\"},\"PeriodicalIF\":5.3000,\"publicationDate\":\"2024-04-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Energy & Fuels\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acs.energyfuels.4c00415\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENERGY & FUELS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Energy & Fuels","FirstCategoryId":"5","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.energyfuels.4c00415","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
Recent Progress and Perspectives on Transition Metal-Based Electrocatalysts for Efficient Nitrate Reduction
Electrochemical nitrate reduction is the process of converting nitrate into ammonia or nitrogen using electric energy. This saves energy, protects the environment, and is an important technology for nitrogen resource recovery and water purification. This paper examines recent advances in electrochemical nitrate reduction technology research and analyzes the reaction mechanism and path of electrochemical nitrate reduction as well as the influence of various factors on the reaction path through thermodynamic and kinetic principles. Second, the catalytic performances of transition metal electrocatalysts in the form of single metals, alloys, oxides, and composites in electrochemical nitrate reduction are analyzed in detail, which lays the foundation for the rational development of new, efficient, and stable electrocatalysts. Finally, future development directions and prospects for electrochemical nitrate reduction technology are envisioned.
期刊介绍:
Energy & Fuels publishes reports of research in the technical area defined by the intersection of the disciplines of chemistry and chemical engineering and the application domain of non-nuclear energy and fuels. This includes research directed at the formation of, exploration for, and production of fossil fuels and biomass; the properties and structure or molecular composition of both raw fuels and refined products; the chemistry involved in the processing and utilization of fuels; fuel cells and their applications; and the analytical and instrumental techniques used in investigations of the foregoing areas.