一种新型燃煤锅炉氮氧化物排放混合预测方法,结合了 CEEMDAN 和 LSTM 改进的自注意方法

IF 1.4 4区 工程技术 Q3 ENGINEERING, CHEMICAL
Hua Yan, Yunchi Chen, Bin Yang, Yang Yang, Hu Ni, Ying Wang
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引用次数: 0

摘要

燃煤锅炉中氮氧化物生成浓度的精确预测是选择性催化还原脱硝(SCR)系统明智优化和控制的基础。由于选择性催化还原脱硝过程的复杂性,根据选择性催化还原入口处氮氧化物浓度的监测数据调节氨喷射率存在时间延迟。这种延迟会导致氨泄漏,进而阻塞空气预热器。有鉴于此,我们提出了一种预测模型 CEEMDAN-LSTM-SA,它将数据分解与深度学习网络中的 LSTM(长短期记忆)融合自注意机制相结合,用于预测燃煤机组 SCR 入口处的氮氧化物排放浓度。为减少数据异常值对模型训练效果的影响,最初采用聚类方法结合统计测试策略,首先对数据集进行细化。利用 CEEMDAN 数据分解技术对数据进行分解,减轻数据的非平稳性和复杂性。随后,通过频谱分析,对分解后的成分进行分组和聚合,形成新的数据元素,再由构建的 LSTM-SA 深度学习网络进行预测。通过融合过程得出最终的氮氧化物排放浓度预测值。通过仔细研究和比较使用燃煤电厂数据的各种模型得出的预测值,可以明显看出 CEEMDAN-LSTM-SA 预测的性能指标为:平均绝对误差 7.425、平均绝对百分比误差 2.415%、均方根误差 9.715、R 平方 (R2) 值 0.789、平均绝对相对误差 2.109%、Theil 信息准则 0.016。与其他模型(包括传统的自我注意网络、LSTM 和 LSTM-SA 组合网络)相比,本研究提出的 CEEMDAN-LSTM-SA 模型具有更高的预测准确性和更强的泛化能力。因此,该预测模型有望为火电机组的 SCR 注氨策略提供一个有效的框架。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
A novel hybrid forecasting approach for NOx emission of coal-fired boiler combined with CEEMDAN and self-attention improved by LSTM

The precise prediction of NOx generation concentration in coal-fired boilers serves as the foundational cornerstone for the judicious optimization and control of selective catalytic reduction denitrification (SCR) systems. Owing to the intricate nature of the denitrification process within SCR, there exists a temporal delay in regulating the ammonia injection rate based on the monitored data of NOx concentration at the SCR inlet. Such delays can give rise to ammonia leakage and subsequent obstruction of the air preheater. In light of this, a predictive model, CEEMDAN-LSTM-SA, is proposed as an amalgamation of data decomposition and the LSTM (long short-term memory) fusion self-attention mechanism within a deep learning network, which is introduced to forecast the NOx emission concentration at the SCR inlet of coal-fired units. To mitigate the impact of data outliers on the training effectiveness of the model, a clustering method coupled with a statistical testing strategy is initially applied to refine the dataset first. CEEMDAN data decomposition technology is leveraged to facilitate the breakdown of data, alleviating its non-stationary and intricate characteristics. Subsequently, through spectral analysis, the decomposed components are grouped and aggregated to form novel data elements, which are then subjected to prediction by the constructed LSTM-SA deep learning network. The ultimate NOx emission concentration prediction value is derived through a process of fusion. Upon scrutinizing and comparing the predictions derived from various models using coal-fired power plant data, it is evident that the performance metrics of CEEMDAN-LSTM-SA predictions exhibit a mean absolute error of 7.425, mean absolute percentage error of 2.415%, root mean square error of 9.715, R-squared (R2) value of .789, mean absolute relative error of 2.109%, and a Theil's information criterion of .016. In contrast to other models, including traditional self-attention networks, LSTM, and LSTM-SA combination networks, CEEMDAN-LSTM-SA proposed in this study demonstrates superior prediction accuracy and enhanced generalization capabilities. Consequently, this predictive model stands poised to furnish an efficacious framework for the SCR ammonia injection strategy within thermal power units.

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来源期刊
自引率
11.10%
发文量
111
期刊介绍: Asia-Pacific Journal of Chemical Engineering is aimed at capturing current developments and initiatives in chemical engineering related and specialised areas. Publishing six issues each year, the journal showcases innovative technological developments, providing an opportunity for technology transfer and collaboration. Asia-Pacific Journal of Chemical Engineering will focus particular attention on the key areas of: Process Application (separation, polymer, catalysis, nanotechnology, electrochemistry, nuclear technology); Energy and Environmental Technology (materials for energy storage and conversion, coal gasification, gas liquefaction, air pollution control, water treatment, waste utilization and management, nuclear waste remediation); and Biochemical Engineering (including targeted drug delivery applications).
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