Rui Liu , Chaojun Zhang , Rijia Liu , Yuan Sun , Binqiao Ren , Yuhang Tong , Yu Tao
{"title":"推进抗生素检测和降解:氮化石墨碳(g-C3N4)应用的最新创新","authors":"Rui Liu , Chaojun Zhang , Rijia Liu , Yuan Sun , Binqiao Ren , Yuhang Tong , Yu Tao","doi":"10.1016/j.jes.2024.03.033","DOIUrl":null,"url":null,"abstract":"<div><p>The uncontrolled release of antibiotics into the environment would be extremely harmful to human health and ecosystems. Therefore, it is in urgent need to monitor the environment and promote the detection and degradation of antibiotics to the relatively harmless by-products to a feasible extent. Graphitic carbon nitride (g-C<sub>3</sub>N<sub>4</sub>) is a non-metallic n-type semiconductor that can be used for the antibiotic detection and degradation due to its easy synthesis process, excellent chemical stability and unique optical properties. Unfortunately, the utilization of visible light, electron-hole recombination and electron conductivity have hindered its potential applications in the fields of photocatalytic degradation and electrochemical detection. Although previous publications have highlighted the diverse modification methods for the g-C<sub>3</sub>N<sub>4</sub>-based materials, the underlying structure-performance relationships of g-C<sub>3</sub>N<sub>4</sub>, especially for the detection and degradation of antibiotics, remains to be further explored. In view of this, the current review centered on the recent progress in the modification techniques of g-C<sub>3</sub>N<sub>4</sub>, the detection and degradation of antibiotics using the g-C<sub>3</sub>N<sub>4</sub>-based materials, as well as the potential antibiotic degradation mechanisms of the g-C<sub>3</sub>N<sub>4</sub>-based materials. Additionally, the underlying applications of the g-C<sub>3</sub>N<sub>4</sub>-based materials for antibiotic detection and degradation were also prospected. This review would provide a valuable research foundation and the up-to-date information for the g-C<sub>3</sub>N<sub>4</sub>-based materials to combat antibiotic pollution in the environment.</p></div>","PeriodicalId":15788,"journal":{"name":"Journal of Environmental Sciences-china","volume":"150 ","pages":"Pages 657-675"},"PeriodicalIF":5.9000,"publicationDate":"2024-04-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Advancing antibiotic detection and degradation: recent innovations in graphitic carbon nitride (g-C3N4) applications\",\"authors\":\"Rui Liu , Chaojun Zhang , Rijia Liu , Yuan Sun , Binqiao Ren , Yuhang Tong , Yu Tao\",\"doi\":\"10.1016/j.jes.2024.03.033\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>The uncontrolled release of antibiotics into the environment would be extremely harmful to human health and ecosystems. Therefore, it is in urgent need to monitor the environment and promote the detection and degradation of antibiotics to the relatively harmless by-products to a feasible extent. Graphitic carbon nitride (g-C<sub>3</sub>N<sub>4</sub>) is a non-metallic n-type semiconductor that can be used for the antibiotic detection and degradation due to its easy synthesis process, excellent chemical stability and unique optical properties. Unfortunately, the utilization of visible light, electron-hole recombination and electron conductivity have hindered its potential applications in the fields of photocatalytic degradation and electrochemical detection. Although previous publications have highlighted the diverse modification methods for the g-C<sub>3</sub>N<sub>4</sub>-based materials, the underlying structure-performance relationships of g-C<sub>3</sub>N<sub>4</sub>, especially for the detection and degradation of antibiotics, remains to be further explored. In view of this, the current review centered on the recent progress in the modification techniques of g-C<sub>3</sub>N<sub>4</sub>, the detection and degradation of antibiotics using the g-C<sub>3</sub>N<sub>4</sub>-based materials, as well as the potential antibiotic degradation mechanisms of the g-C<sub>3</sub>N<sub>4</sub>-based materials. Additionally, the underlying applications of the g-C<sub>3</sub>N<sub>4</sub>-based materials for antibiotic detection and degradation were also prospected. This review would provide a valuable research foundation and the up-to-date information for the g-C<sub>3</sub>N<sub>4</sub>-based materials to combat antibiotic pollution in the environment.</p></div>\",\"PeriodicalId\":15788,\"journal\":{\"name\":\"Journal of Environmental Sciences-china\",\"volume\":\"150 \",\"pages\":\"Pages 657-675\"},\"PeriodicalIF\":5.9000,\"publicationDate\":\"2024-04-03\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Environmental Sciences-china\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1001074224001499\",\"RegionNum\":2,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENVIRONMENTAL SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Environmental Sciences-china","FirstCategoryId":"93","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1001074224001499","RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
Advancing antibiotic detection and degradation: recent innovations in graphitic carbon nitride (g-C3N4) applications
The uncontrolled release of antibiotics into the environment would be extremely harmful to human health and ecosystems. Therefore, it is in urgent need to monitor the environment and promote the detection and degradation of antibiotics to the relatively harmless by-products to a feasible extent. Graphitic carbon nitride (g-C3N4) is a non-metallic n-type semiconductor that can be used for the antibiotic detection and degradation due to its easy synthesis process, excellent chemical stability and unique optical properties. Unfortunately, the utilization of visible light, electron-hole recombination and electron conductivity have hindered its potential applications in the fields of photocatalytic degradation and electrochemical detection. Although previous publications have highlighted the diverse modification methods for the g-C3N4-based materials, the underlying structure-performance relationships of g-C3N4, especially for the detection and degradation of antibiotics, remains to be further explored. In view of this, the current review centered on the recent progress in the modification techniques of g-C3N4, the detection and degradation of antibiotics using the g-C3N4-based materials, as well as the potential antibiotic degradation mechanisms of the g-C3N4-based materials. Additionally, the underlying applications of the g-C3N4-based materials for antibiotic detection and degradation were also prospected. This review would provide a valuable research foundation and the up-to-date information for the g-C3N4-based materials to combat antibiotic pollution in the environment.
期刊介绍:
The Journal of Environmental Sciences is an international journal started in 1989. The journal is devoted to publish original, peer-reviewed research papers on main aspects of environmental sciences, such as environmental chemistry, environmental biology, ecology, geosciences and environmental physics. Appropriate subjects include basic and applied research on atmospheric, terrestrial and aquatic environments, pollution control and abatement technology, conservation of natural resources, environmental health and toxicology. Announcements of international environmental science meetings and other recent information are also included.