{"title":"利用计算流体动力学 (CFD) 建立流化床光反应器 (FBP) 的理论流体动力学模型:固定在海滩沙粒上的 TiO2-CuO 的流化条件","authors":"R. Solano, M. Mueses, Adriana Herrera","doi":"10.1155/2024/8637773","DOIUrl":null,"url":null,"abstract":"The flow regime is essential in the photoreactor’s performance in pollutant degradation in the aqueous medium, especially in fluidized systems. Therefore, this study is focused on determining the fluidization conditions of a granular catalyst based on TiO2-CuO nanoparticles (1 wt.% CuO) immobilized on beach sand granules using an FBP photoreactor. COMSOL Multiphysics 6.0 was employed for inlet velocities between 0.1 m/s and 1.0 m/s, mainly from the Reynolds averaged Navier–Stokes (RANS) turbulence model and the Stokes drag law. The results indicated that the average velocities in the annular section are much higher (4.11ut and 5.42ut) than the required particle terminal velocity. Moreover, the pressure contour lines revealed that these flow velocities do not represent excessive pressures in the concentric cylinders, with maximum gauge pressures of 740.52 Pa and 1310 Pa for inlet velocities Uo=0.75 and 1.0 m/s, respectively. Finally, it was determined that the Reynolds number adjusted (Repf) values lower than or equal to 1.37×10−3 allow high fluidization after 2 seconds. This information makes it possible to adapt and assemble the FBP equipment for future photocatalytic evaluation.","PeriodicalId":45541,"journal":{"name":"Modelling and Simulation in Engineering","volume":null,"pages":null},"PeriodicalIF":0.8000,"publicationDate":"2024-03-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Theoretical Hydrodynamic Modeling of the Fluidized Bed Photoreactor (FBP) Using Computational Fluid Dynamics (CFD): Fluidization Conditions for TiO2-CuO Immobilized on Beach Sand Granules\",\"authors\":\"R. Solano, M. Mueses, Adriana Herrera\",\"doi\":\"10.1155/2024/8637773\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The flow regime is essential in the photoreactor’s performance in pollutant degradation in the aqueous medium, especially in fluidized systems. Therefore, this study is focused on determining the fluidization conditions of a granular catalyst based on TiO2-CuO nanoparticles (1 wt.% CuO) immobilized on beach sand granules using an FBP photoreactor. COMSOL Multiphysics 6.0 was employed for inlet velocities between 0.1 m/s and 1.0 m/s, mainly from the Reynolds averaged Navier–Stokes (RANS) turbulence model and the Stokes drag law. The results indicated that the average velocities in the annular section are much higher (4.11ut and 5.42ut) than the required particle terminal velocity. Moreover, the pressure contour lines revealed that these flow velocities do not represent excessive pressures in the concentric cylinders, with maximum gauge pressures of 740.52 Pa and 1310 Pa for inlet velocities Uo=0.75 and 1.0 m/s, respectively. Finally, it was determined that the Reynolds number adjusted (Repf) values lower than or equal to 1.37×10−3 allow high fluidization after 2 seconds. This information makes it possible to adapt and assemble the FBP equipment for future photocatalytic evaluation.\",\"PeriodicalId\":45541,\"journal\":{\"name\":\"Modelling and Simulation in Engineering\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":0.8000,\"publicationDate\":\"2024-03-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Modelling and Simulation in Engineering\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.1155/2024/8637773\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ENGINEERING, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Modelling and Simulation in Engineering","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.1155/2024/8637773","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENGINEERING, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
摘要
光反应器在水介质中降解污染物时,尤其是在流化系统中,流态对其性能至关重要。因此,本研究的重点是利用 FBP 光反应器确定固定在海滩沙粒上的基于 TiO2-CuO 纳米颗粒(1 wt.% CuO)的颗粒催化剂的流化条件。COMSOL Multiphysics 6.0 采用雷诺平均纳维-斯托克斯(RANS)湍流模型和斯托克斯阻力定律,入口速度介于 0.1 m/s 和 1.0 m/s 之间。结果表明,环形部分的平均速度(4.11ut 和 5.42ut)远高于所需的颗粒末端速度。此外,压力等值线显示,这些流速并不代表同心圆筒中的压力过大,入口速度 Uo=0.75 和 1.0 m/s 时的最大表压分别为 740.52 Pa 和 1310 Pa。最后确定,雷诺数调整值(Repf)小于或等于 1.37×10-3 时,2 秒后流化程度较高。有了这些信息,就可以调整和组装 FBP 设备,以便将来进行光催化评估。
Theoretical Hydrodynamic Modeling of the Fluidized Bed Photoreactor (FBP) Using Computational Fluid Dynamics (CFD): Fluidization Conditions for TiO2-CuO Immobilized on Beach Sand Granules
The flow regime is essential in the photoreactor’s performance in pollutant degradation in the aqueous medium, especially in fluidized systems. Therefore, this study is focused on determining the fluidization conditions of a granular catalyst based on TiO2-CuO nanoparticles (1 wt.% CuO) immobilized on beach sand granules using an FBP photoreactor. COMSOL Multiphysics 6.0 was employed for inlet velocities between 0.1 m/s and 1.0 m/s, mainly from the Reynolds averaged Navier–Stokes (RANS) turbulence model and the Stokes drag law. The results indicated that the average velocities in the annular section are much higher (4.11ut and 5.42ut) than the required particle terminal velocity. Moreover, the pressure contour lines revealed that these flow velocities do not represent excessive pressures in the concentric cylinders, with maximum gauge pressures of 740.52 Pa and 1310 Pa for inlet velocities Uo=0.75 and 1.0 m/s, respectively. Finally, it was determined that the Reynolds number adjusted (Repf) values lower than or equal to 1.37×10−3 allow high fluidization after 2 seconds. This information makes it possible to adapt and assemble the FBP equipment for future photocatalytic evaluation.
期刊介绍:
Modelling and Simulation in Engineering aims at providing a forum for the discussion of formalisms, methodologies and simulation tools that are intended to support the new, broader interpretation of Engineering. Competitive pressures of Global Economy have had a profound effect on the manufacturing in Europe, Japan and the USA with much of the production being outsourced. In this context the traditional interpretation of engineering profession linked to the actual manufacturing needs to be broadened to include the integration of outsourced components and the consideration of logistic, economical and human factors in the design of engineering products and services.