V. Yu. Osipov, K. V. Bogdanov, A. Rampersaud, K. Takai, Y. Ishiguro, A. V. Baranov
{"title":"光学自旋极化条件下合成荧光钻石微晶中 NV（-）中心的电子自旋共振","authors":"V. Yu. Osipov, K. V. Bogdanov, A. Rampersaud, K. Takai, Y. Ishiguro, A. V. Baranov","doi":"10.1134/S0030400X23040148","DOIUrl":null,"url":null,"abstract":"<p>Electron paramagnetic resonance (EPR) spectra of synthetic diamond microcrystals with NV<sup>(‒)</sup>‑centers have been studied. It is shown that under the conditions of irradiation of the material with the light of a xenon lamp at low temperatures ~100 K, the intensities of the EPR signals corresponding to the “forbidden” (Δ<i>m</i><sub><i>s</i></sub> = 2) and low field allowed (Δ<i>m</i><sub><i>s</i></sub> = 1) transitions are amplified several times, while the EPR signals from paramagnetic nitrogen and impurity nickel in the charge state –1 practically do not change. This is due to a change in the population of levels of the ground triplet state of the NV<sup>(–)</sup>-center and the optical polarization of spins in the state <i>m</i><sub><i>s</i></sub> = 0 of the triplet level.</p>","PeriodicalId":723,"journal":{"name":"Optics and Spectroscopy","volume":"131 2","pages":"111 - 118"},"PeriodicalIF":0.8000,"publicationDate":"2024-03-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Electron Spin Resonance of NV(–)-Centers in Synthetic Fluorescent Diamond Microcrystals under Conditions of Optical Spin Polarization\",\"authors\":\"V. Yu. Osipov, K. V. Bogdanov, A. Rampersaud, K. Takai, Y. Ishiguro, A. V. Baranov\",\"doi\":\"10.1134/S0030400X23040148\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Electron paramagnetic resonance (EPR) spectra of synthetic diamond microcrystals with NV<sup>(‒)</sup>‑centers have been studied. It is shown that under the conditions of irradiation of the material with the light of a xenon lamp at low temperatures ~100 K, the intensities of the EPR signals corresponding to the “forbidden” (Δ<i>m</i><sub><i>s</i></sub> = 2) and low field allowed (Δ<i>m</i><sub><i>s</i></sub> = 1) transitions are amplified several times, while the EPR signals from paramagnetic nitrogen and impurity nickel in the charge state –1 practically do not change. This is due to a change in the population of levels of the ground triplet state of the NV<sup>(–)</sup>-center and the optical polarization of spins in the state <i>m</i><sub><i>s</i></sub> = 0 of the triplet level.</p>\",\"PeriodicalId\":723,\"journal\":{\"name\":\"Optics and Spectroscopy\",\"volume\":\"131 2\",\"pages\":\"111 - 118\"},\"PeriodicalIF\":0.8000,\"publicationDate\":\"2024-03-14\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Optics and Spectroscopy\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://link.springer.com/article/10.1134/S0030400X23040148\",\"RegionNum\":4,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q4\",\"JCRName\":\"OPTICS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Optics and Spectroscopy","FirstCategoryId":"101","ListUrlMain":"https://link.springer.com/article/10.1134/S0030400X23040148","RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q4","JCRName":"OPTICS","Score":null,"Total":0}
Electron Spin Resonance of NV(–)-Centers in Synthetic Fluorescent Diamond Microcrystals under Conditions of Optical Spin Polarization
Electron paramagnetic resonance (EPR) spectra of synthetic diamond microcrystals with NV(‒)‑centers have been studied. It is shown that under the conditions of irradiation of the material with the light of a xenon lamp at low temperatures ~100 K, the intensities of the EPR signals corresponding to the “forbidden” (Δms = 2) and low field allowed (Δms = 1) transitions are amplified several times, while the EPR signals from paramagnetic nitrogen and impurity nickel in the charge state –1 practically do not change. This is due to a change in the population of levels of the ground triplet state of the NV(–)-center and the optical polarization of spins in the state ms = 0 of the triplet level.
期刊介绍：
Optics and Spectroscopy (Optika i spektroskopiya), founded in 1956, presents original and review papers in various fields of modern optics and spectroscopy in the entire wavelength range from radio waves to X-rays. Topics covered include problems of theoretical and experimental spectroscopy of atoms, molecules, and condensed state, lasers and the interaction of laser radiation with matter, physical and geometrical optics, holography, and physical principles of optical instrument making.
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