用于氧反应还原的铂基电催化剂应变工程学

IF 3.1 4区 工程技术 Q3 ENERGY & FUELS
Zeyu Wang, Yanru Liu, Shun Chen, Yun Zheng, Xiaogang Fu, Yan Zhang, Wanglei Wang
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引用次数: 0

摘要

质子交换膜燃料电池(PEMFC)在未来可持续能源系统的建设中发挥着不可替代的作用。然而,基于铂(Pt)的氧还原反应(ORR)电催化剂性能不足,阻碍了 PEMFCs 的整体效率。催化剂表面应变工程被认为是调整其电子结构从而优化催化行为的有效方法。本文将详细阐述应变工程在改善铂基催化剂的 ORR 方面的应用。首先,全面讨论了在理解应变对 ORR 催化剂的影响方面的最新进展。然后,全面讨论了调整铂基催化剂的应变工程方法。最后,进一步介绍了铂基催化剂应变调节所面临的各种挑战和潜在前景。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Strain engineering of Pt-based electrocatalysts for oxygen reaction reduction

Proton exchange membrane fuel cells (PEMFCs) are playing irreplaceable roles in the construction of the future sustainable energy system. However, the insufficient performance of platinum (Pt)-based electrocatalysts for oxygen reduction reaction (ORR) hinders the overall efficiency of PEMFCs. Engineering the surface strain of catalysts is considered an effective way to tune their electronic structures and therefore optimize catalytic behavior. In this paper, insights into strain engineering for improving Pt-based catalysts toward ORR are elaborated in detail. First, recent advances in understanding the strain effects on ORR catalysts are comprehensively discussed. Then, strain engineering methodologies for adjusting Pt-based catalysts are comprehensively discussed. Finally, further information on the various challenges and potential prospects for strain modulation of Pt-based catalysts is provided.

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来源期刊
Frontiers in Energy
Frontiers in Energy Energy-Energy Engineering and Power Technology
CiteScore
5.90
自引率
6.90%
发文量
708
期刊介绍: Frontiers in Energy, an interdisciplinary and peer-reviewed international journal launched in January 2007, seeks to provide a rapid and unique platform for reporting the most advanced research on energy technology and strategic thinking in order to promote timely communication between researchers, scientists, engineers, and policy makers in the field of energy. Frontiers in Energy aims to be a leading peer-reviewed platform and an authoritative source of information for analyses, reviews and evaluations in energy engineering and research, with a strong focus on energy analysis, energy modelling and prediction, integrated energy systems, energy conversion and conservation, energy planning and energy on economic and policy issues. Frontiers in Energy publishes state-of-the-art review articles, original research papers and short communications by individual researchers or research groups. It is strictly peer-reviewed and accepts only original submissions in English. The scope of the journal is broad and covers all latest focus in current energy research. High-quality papers are solicited in, but are not limited to the following areas: -Fundamental energy science -Energy technology, including energy generation, conversion, storage, renewables, transport, urban design and building efficiency -Energy and the environment, including pollution control, energy efficiency and climate change -Energy economics, strategy and policy -Emerging energy issue
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