{"title":"利用坚固稳定的金属有机框架进行二氧化碳光催化还原：综述","authors":"Ryohei Mori","doi":"10.1007/s40243-023-00252-5","DOIUrl":null,"url":null,"abstract":"<p>Climate change and global warming problem are becoming the serious issue and some action is necessary in order to mitigate the rising temperature. CO<sub>2</sub> increase is one of the reason for temperature rise, and the technology to convert CO<sub>2</sub> to beneficial energy or chemical substance could be one of the key solution (CO<sub>2</sub> photocatalytic reduction). Metal–organic frameworks (MOFs) have gained much attention owing to their extremely large surface areas, tunable fine structures, and potential applications in many areas. Recently, MOFs have been demonstrated to be promising materials for CO<sub>2</sub> photocatalytic reduction. This review summarized recent research progresses in photocatalytic reduction using MOFs. MOFs were classified mainly by the type of metal center, and the feature and tendency against their functions towards CO<sub>2</sub> photocatalytic activity will be explained.</p>","PeriodicalId":692,"journal":{"name":"Materials for Renewable and Sustainable Energy","volume":null,"pages":null},"PeriodicalIF":3.6000,"publicationDate":"2024-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"CO2 photocatalytic reduction with robust and stable metal–organic framework: a review\",\"authors\":\"Ryohei Mori\",\"doi\":\"10.1007/s40243-023-00252-5\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Climate change and global warming problem are becoming the serious issue and some action is necessary in order to mitigate the rising temperature. CO<sub>2</sub> increase is one of the reason for temperature rise, and the technology to convert CO<sub>2</sub> to beneficial energy or chemical substance could be one of the key solution (CO<sub>2</sub> photocatalytic reduction). Metal–organic frameworks (MOFs) have gained much attention owing to their extremely large surface areas, tunable fine structures, and potential applications in many areas. Recently, MOFs have been demonstrated to be promising materials for CO<sub>2</sub> photocatalytic reduction. This review summarized recent research progresses in photocatalytic reduction using MOFs. MOFs were classified mainly by the type of metal center, and the feature and tendency against their functions towards CO<sub>2</sub> photocatalytic activity will be explained.</p>\",\"PeriodicalId\":692,\"journal\":{\"name\":\"Materials for Renewable and Sustainable Energy\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":3.6000,\"publicationDate\":\"2024-03-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Materials for Renewable and Sustainable Energy\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.1007/s40243-023-00252-5\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Materials for Renewable and Sustainable Energy","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.1007/s40243-023-00252-5","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
摘要
气候变化和全球变暖问题日益严重，有必要采取一些行动来减缓气温的上升。二氧化碳增加是气温上升的原因之一，而将二氧化碳转化为有益的能源或化学物质的技术可能是关键的解决方案之一（二氧化碳光催化还原）。金属有机框架（MOFs）因其超大的表面积、可调的精细结构以及在许多领域的潜在应用而备受关注。最近，MOFs 被证明是一种很有前途的二氧化碳光催化还原材料。本综述总结了利用 MOFs 进行光催化还原的最新研究进展。主要根据金属中心的类型对 MOFs 进行分类，并阐述其在 CO2 光催化活性方面的功能特点和发展趋势。
CO2 photocatalytic reduction with robust and stable metal–organic framework: a review
Climate change and global warming problem are becoming the serious issue and some action is necessary in order to mitigate the rising temperature. CO2 increase is one of the reason for temperature rise, and the technology to convert CO2 to beneficial energy or chemical substance could be one of the key solution (CO2 photocatalytic reduction). Metal–organic frameworks (MOFs) have gained much attention owing to their extremely large surface areas, tunable fine structures, and potential applications in many areas. Recently, MOFs have been demonstrated to be promising materials for CO2 photocatalytic reduction. This review summarized recent research progresses in photocatalytic reduction using MOFs. MOFs were classified mainly by the type of metal center, and the feature and tendency against their functions towards CO2 photocatalytic activity will be explained.
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Energy is the single most valuable resource for human activity and the basis for all human progress. Materials play a key role in enabling technologies that can offer promising solutions to achieve renewable and sustainable energy pathways for the future.
Materials for Renewable and Sustainable Energy has been established to be the world''s foremost interdisciplinary forum for publication of research on all aspects of the study of materials for the deployment of renewable and sustainable energy technologies. The journal covers experimental and theoretical aspects of materials and prototype devices for sustainable energy conversion, storage, and saving, together with materials needed for renewable fuel production. It publishes reviews, original research articles, rapid communications, and perspectives. All manuscripts are peer-reviewed for scientific quality.
Topics include:
1. MATERIALS for renewable energy storage and conversion: Batteries, Supercapacitors, Fuel cells, Hydrogen storage, and Photovoltaics and solar cells.
2. MATERIALS for renewable and sustainable fuel production: Hydrogen production and fuel generation from renewables (catalysis), Solar-driven reactions to hydrogen and fuels from renewables (photocatalysis), Biofuels, and Carbon dioxide sequestration and conversion.
3. MATERIALS for energy saving: Thermoelectrics, Novel illumination sources for efficient lighting, and Energy saving in buildings.
4. MATERIALS modeling and theoretical aspects.
5. Advanced characterization techniques of MATERIALS
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