{"title":"外延生长氮化镓表面液态镓有序化的温度依赖性","authors":"Takuo Sasaki, Takuya Iwata, Kanya Sugitani, Takahiro Kawamura, Toru Akiyama and Masamitu Takahasi","doi":"10.35848/1882-0786/ad237b","DOIUrl":null,"url":null,"abstract":"The three-dimensional ordering of the gallium (Ga) adlayers on GaN(0001) and (000 ) surfaces was probed using in situ X-ray scattering under MBE conditions. An ordered bilayer of Ga forms on GaN(0001) but the ordering decreases at substrate temperatures of <450 °C, consistent with the mechanism of non-equilibrium epitaxial growth. Monolayer Ga that forms on GaN(000 ) is laterally disordered and has no temperature dependence, along with droplets of excess Ga. The vertical and lateral B-factors for each Ga layer were confirmed using first-principles molecular dynamics calculations.","PeriodicalId":8093,"journal":{"name":"Applied Physics Express","volume":"66 1","pages":""},"PeriodicalIF":2.3000,"publicationDate":"2024-02-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Temperature dependence of liquid-gallium ordering on the surface of epitaxially grown GaN\",\"authors\":\"Takuo Sasaki, Takuya Iwata, Kanya Sugitani, Takahiro Kawamura, Toru Akiyama and Masamitu Takahasi\",\"doi\":\"10.35848/1882-0786/ad237b\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The three-dimensional ordering of the gallium (Ga) adlayers on GaN(0001) and (000 ) surfaces was probed using in situ X-ray scattering under MBE conditions. An ordered bilayer of Ga forms on GaN(0001) but the ordering decreases at substrate temperatures of <450 °C, consistent with the mechanism of non-equilibrium epitaxial growth. Monolayer Ga that forms on GaN(000 ) is laterally disordered and has no temperature dependence, along with droplets of excess Ga. The vertical and lateral B-factors for each Ga layer were confirmed using first-principles molecular dynamics calculations.\",\"PeriodicalId\":8093,\"journal\":{\"name\":\"Applied Physics Express\",\"volume\":\"66 1\",\"pages\":\"\"},\"PeriodicalIF\":2.3000,\"publicationDate\":\"2024-02-20\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Applied Physics Express\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://doi.org/10.35848/1882-0786/ad237b\",\"RegionNum\":4,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"PHYSICS, APPLIED\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Applied Physics Express","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.35848/1882-0786/ad237b","RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"PHYSICS, APPLIED","Score":null,"Total":0}
引用次数: 0
摘要
在 MBE 条件下,利用原位 X 射线散射探测了 GaN(0001)和(000 )表面镓(Ga)叠层的三维有序性。在氮化镓(0001)上形成了有序的双层镓,但在衬底温度<450 ℃时有序性降低,这与非平衡外延生长的机制一致。在氮化镓(000 )上形成的单层镓是横向无序的,并且与温度无关,同时还有过量的镓滴。第一原理分子动力学计算证实了每个镓层的垂直和横向 B 因子。
Temperature dependence of liquid-gallium ordering on the surface of epitaxially grown GaN
The three-dimensional ordering of the gallium (Ga) adlayers on GaN(0001) and (000 ) surfaces was probed using in situ X-ray scattering under MBE conditions. An ordered bilayer of Ga forms on GaN(0001) but the ordering decreases at substrate temperatures of <450 °C, consistent with the mechanism of non-equilibrium epitaxial growth. Monolayer Ga that forms on GaN(000 ) is laterally disordered and has no temperature dependence, along with droplets of excess Ga. The vertical and lateral B-factors for each Ga layer were confirmed using first-principles molecular dynamics calculations.
期刊介绍:
Applied Physics Express (APEX) is a letters journal devoted solely to rapid dissemination of up-to-date and concise reports on new findings in applied physics. The motto of APEX is high scientific quality and prompt publication. APEX is a sister journal of the Japanese Journal of Applied Physics (JJAP) and is published by IOP Publishing Ltd on behalf of the Japan Society of Applied Physics (JSAP).