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{"title":"珠江口盆地珠江地层二氧化碳长期封存机理及注入模式的影响","authors":"Tao Xuan, Xiaomin Cao, Qi Li, Fangfang Li, Liang Xu","doi":"10.1002/ghg.2261","DOIUrl":null,"url":null,"abstract":"<p>In this paper, the mechanisms of long-term CO<sub>2</sub> sequestration and the effects of injection modes (including injection temperature, injection rate and injection cycle) in Zhujiang Formation characterized by high porosity and permeability were investigated using the numerical simulation method. Simulation results showed that more than 88% of the injected CO<sub>2</sub> would exist in a supercritical state during the injection period and more than 79% of CO<sub>2</sub> would be sequestrated in the reservoir by mineral trapping after 5,000 years. Eventually, the distribution shape of SC-CO<sub>2</sub> was a quarter funnel near the injection well, while the distribution shapes of dissolved and mineralized CO<sub>2</sub> were both one quarter rotunda. During the long-term CO<sub>2</sub> sequestration in Zhujiang Formation, the dissolved minerals were anorthite, chlorite and smectite in turn, while the top three main precipitated minerals were calcite, dawsonite and albite. Moreover, higher injection temperature leads to a higher mineral tapping and more dissolved/precipitated minerals. While higher injection rate reduces the mineral tapping and total amount of dissolved/precipitated mineral. Compared to injection temperature and injection rate, the injection cycle has little effect on the CO<sub>2</sub> phase evolution and mineral dissolution/precipitation process. © 2024 Society of Chemical Industry and John Wiley & Sons, Ltd.</p>","PeriodicalId":12796,"journal":{"name":"Greenhouse Gases: Science and Technology","volume":"14 2","pages":"221-237"},"PeriodicalIF":2.7000,"publicationDate":"2024-01-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Long-term CO2 sequestration mechanisms and influence of injection mode in Zhujiang Formation of Pearl River Mouth Basin\",\"authors\":\"Tao Xuan, Xiaomin Cao, Qi Li, Fangfang Li, Liang Xu\",\"doi\":\"10.1002/ghg.2261\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>In this paper, the mechanisms of long-term CO<sub>2</sub> sequestration and the effects of injection modes (including injection temperature, injection rate and injection cycle) in Zhujiang Formation characterized by high porosity and permeability were investigated using the numerical simulation method. Simulation results showed that more than 88% of the injected CO<sub>2</sub> would exist in a supercritical state during the injection period and more than 79% of CO<sub>2</sub> would be sequestrated in the reservoir by mineral trapping after 5,000 years. Eventually, the distribution shape of SC-CO<sub>2</sub> was a quarter funnel near the injection well, while the distribution shapes of dissolved and mineralized CO<sub>2</sub> were both one quarter rotunda. During the long-term CO<sub>2</sub> sequestration in Zhujiang Formation, the dissolved minerals were anorthite, chlorite and smectite in turn, while the top three main precipitated minerals were calcite, dawsonite and albite. Moreover, higher injection temperature leads to a higher mineral tapping and more dissolved/precipitated minerals. While higher injection rate reduces the mineral tapping and total amount of dissolved/precipitated mineral. Compared to injection temperature and injection rate, the injection cycle has little effect on the CO<sub>2</sub> phase evolution and mineral dissolution/precipitation process. © 2024 Society of Chemical Industry and John Wiley & Sons, Ltd.</p>\",\"PeriodicalId\":12796,\"journal\":{\"name\":\"Greenhouse Gases: Science and Technology\",\"volume\":\"14 2\",\"pages\":\"221-237\"},\"PeriodicalIF\":2.7000,\"publicationDate\":\"2024-01-31\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Greenhouse Gases: Science and Technology\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://onlinelibrary.wiley.com/doi/10.1002/ghg.2261\",\"RegionNum\":4,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ENERGY & FUELS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Greenhouse Gases: Science and Technology","FirstCategoryId":"93","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/ghg.2261","RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
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