锌离子电池无锌金属阳极的最新进展和前景

IF 5.6 2区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY
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引用次数: 0

摘要

摘要 锌离子电池(ZIB)因其低成本、高能量密度和环保等优点,被公认为是一种潜在的储能设备。然而,锌阳极在电池充放电过程中不可避免地会出现锌枝晶、钝化、腐蚀和氢进化反应,成为锌离子电池实际应用的障碍。与金属锌阳极相比,适当的无金属锌阳极可提供更高的工作电位,有效解决金属锌阳极工作过程中的锌枝晶、氢演化和副反应问题。电池安全性和循环寿命的提高为 ZIB 的进一步商业化创造了条件。因此,本研究系统地介绍了 "摇椅式 "ZIB 中无金属锌阳极的研究进展。无锌金属阳极主要分为四类:过渡金属氧化物、过渡金属硫化物、MXene(二维过渡金属碳化物)复合材料和有机化合物,并讨论了它们的性能和锌储存机制。最后,提出了无锌金属阳极的发展前景。本文有望为进一步推广商用可充电 ZIB 提供参考。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Recent advances and perspectives of zinc metal-free anodes for zinc ion batteries

Abstract

Zinc-ion batteries (ZIBs) are recognized as potential energy storage devices due to their advantages of low cost, high energy density, and environmental friendliness. However, zinc anodes are subject to unavoidable zinc dendrites, passivation, corrosion, and hydrogen evolution reactions during the charging and discharging of batteries, becoming obstacles to the practical application of ZIBs. Appropriate zinc metal-free anodes provide a higher working potential than metallic zinc anodes, effectively solving the problems of zinc dendrites, hydrogen evolution, and side reactions during the operation of metallic zinc anodes. The improvement in the safety and cycle life of batteries creates conditions for further commercialization of ZIBs. Therefore, this work systematically introduces the research progress of zinc metal-free anodes in “rocking chair” ZIBs. Zinc metal-free anodes are mainly discussed in four categories: transition metal oxides, transition metal sulfides, MXene (two dimensional transition metal carbide) composites, and organic compounds, with discussions on their properties and zinc storage mechanisms. Finally, the outlook for the development of zinc metal-free anodes is proposed. This paper is expected to provide a reference for the further promotion of commercial rechargeable ZIBs.

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来源期刊
CiteScore
9.30
自引率
16.70%
发文量
205
审稿时长
2 months
期刊介绍: International Journal of Minerals, Metallurgy and Materials (Formerly known as Journal of University of Science and Technology Beijing, Mineral, Metallurgy, Material) provides an international medium for the publication of theoretical and experimental studies related to the fields of Minerals, Metallurgy and Materials. Papers dealing with minerals processing, mining, mine safety, environmental pollution and protection of mines, process metallurgy, metallurgical physical chemistry, structure and physical properties of materials, corrosion and resistance of materials, are viewed as suitable for publication.
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