伊朗德黑兰空气污染物的可能排放源和大气光化学过程:微气象因素对空气质量的作用

IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES
Mohammad Saleh Ali-Taleshi, Alireza Riyahi Bakhtiari, Mauro Masiol
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引用次数: 0

摘要

研究人员对中东某特大城市(伊朗德黑兰)城区一年内(2018 年 1 月至 2018 年 12 月)与人类健康和气候相关的八种空气污染物(PM2.5、PM10、O3、NO、NO2、NOx、SO2 和 CO)的小时浓度进行了调查。通过站点间相关性和分歧系数检测了空气污染物的空间分布。通过解释空气污染物的季节、周和日模式以及污染物之间的滞后相关性,确定了最可能的主要大气过程和来源。通过研究气象因素与主要天气因素的关系,评估了气象因素对空气污染物的影响。通过双变量极坐标图和条件双变量概率函数整合大气环流和空气污染物数据,确定了可能的本地污染源位置。利用潜在污染源贡献函数和浓度加权轨迹检测了潜在的跨界污染源区域。结果表明,排放因子、天气和光化学过程主要决定了空气污染物的日和周周期。与其他污染物相比,二氧化硫的日周期在不同地点差异很大,并呈现出双峰和单峰模式。虽然 O3 的 WPSCF 图没有显示出显著的模式,但主要气态污染物呈现出类似的分布模式,西部地区是 WPSCF 值较高的潜在污染源区域。通过提供本地和跨境范围内空气污染物的有用信息,本研究最终增强了对德黑兰大都会地区大气过程和空气质量状况的总体考虑。 图表摘要
本文章由计算机程序翻译,如有差异,请以英文原文为准。

The possible emission sources and atmospheric photochemical processes of air pollutants in Tehran, Iran: the role of micrometeorological factors on the air quality

The possible emission sources and atmospheric photochemical processes of air pollutants in Tehran, Iran: the role of micrometeorological factors on the air quality

The hourly concentrations of eight air pollutants relevant for human health and climate (PM2.5, PM10, O3, NO, NO2, NOx, SO2, and CO) were investigated for 1 year (January 2018 to December 2018) at an urban location of a megacity in the Middle East (Tehran, Iran). The spatial distributions of air pollutants were detected via inter-site correlations and coefficients of divergence. The most likely predominant atmospheric processes and sources were determined by interpreting the seasonal, weekly, and diel patterns of air pollutants and the lagged correlations among pollutants. The effect of meteorological factors upon the air pollutants was evaluated by investigating the relationships with key weather factors. The locations of the possible local sources were identified by integrating atmospheric circulation and air pollutant data through bivariate polar plots and conditional bivariate probability function. Potential transboundary source areas were detected using potential source contribution function and concentration-weighted trajectory. Results show that emission factors, weather, and photochemical processes mainly shape the diel and weekly cycles of air pollutants. Compared to other pollutants, daily cycles of SO2 are quite different among sites and show both bimodal and unimodal patterns. While the WPSCF map for O3 does not show a remarkable pattern, primary gaseous pollutants presented similar distribution patterns with the most potential source areas with high WPSCF values from the western areas. By providing useful information on air pollutants at local and transboundary scales, the current study finally empowers general considerations upon the atmospheric processes and air quality status over the Tehran metropolitan area.

Graphical Abstract

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来源期刊
Air Quality Atmosphere and Health
Air Quality Atmosphere and Health ENVIRONMENTAL SCIENCES-
CiteScore
8.80
自引率
2.00%
发文量
146
审稿时长
>12 weeks
期刊介绍: Air Quality, Atmosphere, and Health is a multidisciplinary journal which, by its very name, illustrates the broad range of work it publishes and which focuses on atmospheric consequences of human activities and their implications for human and ecological health. It offers research papers, critical literature reviews and commentaries, as well as special issues devoted to topical subjects or themes. International in scope, the journal presents papers that inform and stimulate a global readership, as the topic addressed are global in their import. Consequently, we do not encourage submission of papers involving local data that relate to local problems. Unless they demonstrate wide applicability, these are better submitted to national or regional journals. Air Quality, Atmosphere & Health addresses such topics as acid precipitation; airborne particulate matter; air quality monitoring and management; exposure assessment; risk assessment; indoor air quality; atmospheric chemistry; atmospheric modeling and prediction; air pollution climatology; climate change and air quality; air pollution measurement; atmospheric impact assessment; forest-fire emissions; atmospheric science; greenhouse gases; health and ecological effects; clean air technology; regional and global change and satellite measurements. This journal benefits a diverse audience of researchers, public health officials and policy makers addressing problems that call for solutions based in evidence from atmospheric and exposure assessment scientists, epidemiologists, and risk assessors. Publication in the journal affords the opportunity to reach beyond defined disciplinary niches to this broader readership.
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