Deepashree Dutta, Steven C. Sherwood, Katrin J. Meissner, Martin Jucker
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引用次数: 0
摘要
观测结果表明,近几十年来中间层云(MCs)一直在增加,这可能是由于中间层水蒸气增加所致,而水蒸气增加的主要原因是中层大气中甲烷(CH4)氧化作用增强。过去的温暖气候(如白垩纪早期和古近纪时期)被认为具有比现在更高的 CH4 浓度,未来的 CH4 浓度也可能继续上升。在这里,理想化的大气化学-气候模型实验在强极性海面温度和二氧化碳(CO2)及甲烷(CH4)浓度升高的条件下,预测 MCs 将向中低纬度地区大量扩散,远远超出目前发现 MCs 的地区。灵敏度测试表明,当 CH4 浓度比工业化前高出 16 倍时,CH4 氧化产生的水蒸气增加以及 CO2 和 CH4 浓度升高产生的降温为云的形成创造了有利条件,北半球低纬度地区的 MC 分数为 0.02,中纬度地区为 0.1。CH4 的进一步增加会导致低纬度和中纬度 MC 的单调增加。均匀的表层海洋变暖、极地放大或太阳常数的变化都不会对我们的结果产生重大影响。虽然这些云的出现很有趣,但它们的冰水和液态水含量不足以造成显著的辐射效应。另一方面,这些低纬度和中纬度 MC 造成的中间层脱水有可能导致原子氢的减少,从而影响中间层的臭氧浓度,不过这还需要进一步的研究来证实。
Low latitude mesospheric clouds in a warmer climate
Observations show that mesospheric clouds (MCs) have been increasing in recent decades, presumably due to increased mesospheric water vapor which is mainly caused by greater methane (CH4) oxidation in the middle atmosphere. Past warm climates such as those of the early Cretaceous and Paleogene periods are thought to have had higher CH4 concentrations than present day, and future CH4 concentrations will also likely continue to rise. Here, idealized atmosphere chemistry-climate model experiments forced with strong polar-amplified sea-surface temperatures and elevated carbon dioxide (CO2) and CH4 concentrations predict a substantial spreading of MCs to middle and low latitudes, well beyond regions where they are currently found. Sensitivity tests show that increased water vapor from CH4 oxidation and cooling from increased CO2 and CH4 concentrations create favorable conditions for cloud formation, producing MC fractions of 0.02 in the low latitudes and 0.1 in the mid-latitudes in the Northern Hemisphere when CH4 concentration is 16× higher than pre-industrial. Further increases in CH4 result in a monotonic increase in low- and mid-latitude MCs. A uniform surface ocean warming, changes in polar amplification, or the solar constant do not significantly affect our results. While the appearance of these clouds is interesting, their ice and liquid water content is not sufficient to cause a significant radiative effect. On the other hand, dehydration of the mesosphere due to these low- and mid-latitude MCs could potentially lead to a reduction in atomic hydrogen, thereby affecting mesospheric ozone concentration, although further study is required to confirm this.
期刊介绍:
Atmospheric Science Letters (ASL) is a wholly Open Access electronic journal. Its aim is to provide a fully peer reviewed publication route for new shorter contributions in the field of atmospheric and closely related sciences. Through its ability to publish shorter contributions more rapidly than conventional journals, ASL offers a framework that promotes new understanding and creates scientific debate - providing a platform for discussing scientific issues and techniques.
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