从多尺度角度看基于团簇的层状材料：面向催化和储能应用的设计与功能优化

IF 6.2 3区综合性期刊 Q1 Multidisciplinary

Fundamental Research Pub Date : 2025-07-01 DOI:10.1016/j.fmre.2023.12.003

Binbin Qian , Ke Xu , Dantong Zhang , Sridhar Komarneni , Dongfeng Xue

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摘要

层状材料以其独特的结构特点和高度可调的性能成为化学和材料科学研究的热点之一。具有中尺度动态结构的团簇可以作为结构单元或客体引入到层状材料中，使基于团簇的层状材料具有不同于单个组分的增强或新特性。本文首先从多尺度角度综述了典型簇状层状材料的设计和组装策略，然后介绍了多尺度表征和仿真平台。此外，我们还讨论了簇基层状材料在催化和储能方面的最新进展，并总结了该领域目前面临的挑战和未来的发展方向。

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A multiscale perspective on cluster-based layered materials: Design and function optimization toward catalytic and energy storage applications

Layered materials have become one of the focuses in chemistry and materials science due to their unique structural characteristics and highly tunable properties. Clusters with mesoscale dynamic structures can be introduced into layered materials as structural units or guests, endowing cluster-based layered materials with enhanced or emerging new properties different from those of the individual components. This review starts with a summary of the design and assembly strategies of typical cluster-based layered materials from a multiscale perspective, and then introduces the multiscale characterization and simulation platform. Additionally, we discuss the recent progress in the catalytic and energy storage application of cluster-based layered materials and summarize the current challenges and future directions in this field.

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