Erhan Onat, Sabit Horoz, Ömer Şahin, Mehmet Sait İzgi
{"title":"革命性的碳量子点支撑钴催化剂实现破纪录的氢气生产率","authors":"Erhan Onat, Sabit Horoz, Ömer Şahin, Mehmet Sait İzgi","doi":"10.1007/s41779-023-00988-3","DOIUrl":null,"url":null,"abstract":"<p>In this study, we introduce a groundbreaking approach in the field of hydrogen production by synthesizing and characterizing a carbon quantum dot supported-Co (<b>Co-B_CQDs</b>) catalyst. Our results demonstrate that this state-of-the-art catalyst exhibits exceptional performance in the hydrolysis of KBH<sub>4</sub>, resulting in a record-breaking hydrogen production rate of 23,019.97 mL*gcat<sup>−1</sup>*min<sup>−1</sup> and a remarkably low activation energy of 19.36 kJ/mol. This is the first time that this type of catalyst has been used to achieve such outstanding results. The study highlights the remarkable potential of carbon quantum dots as a support material for dispersing metal catalysts, which opens up new avenues for research in the field of hydrogen production. The synthesized catalyst was extensively characterized using various analytical techniques such as X-ray diffraction (XRD), ultraviolet and visible light (UV–Vis), photoluminescence (PL), and inductively coupled plasma optical emission spectrometry (ICP-OES) measurements, which further confirmed its superior performance.</p>","PeriodicalId":673,"journal":{"name":"Journal of the Australian Ceramic Society","volume":"100 1","pages":""},"PeriodicalIF":1.8000,"publicationDate":"2024-01-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Revolutionary carbon quantum dot supported-Co catalyst for record-breaking hydrogen production rate\",\"authors\":\"Erhan Onat, Sabit Horoz, Ömer Şahin, Mehmet Sait İzgi\",\"doi\":\"10.1007/s41779-023-00988-3\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>In this study, we introduce a groundbreaking approach in the field of hydrogen production by synthesizing and characterizing a carbon quantum dot supported-Co (<b>Co-B_CQDs</b>) catalyst. Our results demonstrate that this state-of-the-art catalyst exhibits exceptional performance in the hydrolysis of KBH<sub>4</sub>, resulting in a record-breaking hydrogen production rate of 23,019.97 mL*gcat<sup>−1</sup>*min<sup>−1</sup> and a remarkably low activation energy of 19.36 kJ/mol. This is the first time that this type of catalyst has been used to achieve such outstanding results. The study highlights the remarkable potential of carbon quantum dots as a support material for dispersing metal catalysts, which opens up new avenues for research in the field of hydrogen production. The synthesized catalyst was extensively characterized using various analytical techniques such as X-ray diffraction (XRD), ultraviolet and visible light (UV–Vis), photoluminescence (PL), and inductively coupled plasma optical emission spectrometry (ICP-OES) measurements, which further confirmed its superior performance.</p>\",\"PeriodicalId\":673,\"journal\":{\"name\":\"Journal of the Australian Ceramic Society\",\"volume\":\"100 1\",\"pages\":\"\"},\"PeriodicalIF\":1.8000,\"publicationDate\":\"2024-01-05\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of the Australian Ceramic Society\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1007/s41779-023-00988-3\",\"RegionNum\":4,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MATERIALS SCIENCE, CERAMICS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of the Australian Ceramic Society","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1007/s41779-023-00988-3","RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, CERAMICS","Score":null,"Total":0}
Revolutionary carbon quantum dot supported-Co catalyst for record-breaking hydrogen production rate
In this study, we introduce a groundbreaking approach in the field of hydrogen production by synthesizing and characterizing a carbon quantum dot supported-Co (Co-B_CQDs) catalyst. Our results demonstrate that this state-of-the-art catalyst exhibits exceptional performance in the hydrolysis of KBH4, resulting in a record-breaking hydrogen production rate of 23,019.97 mL*gcat−1*min−1 and a remarkably low activation energy of 19.36 kJ/mol. This is the first time that this type of catalyst has been used to achieve such outstanding results. The study highlights the remarkable potential of carbon quantum dots as a support material for dispersing metal catalysts, which opens up new avenues for research in the field of hydrogen production. The synthesized catalyst was extensively characterized using various analytical techniques such as X-ray diffraction (XRD), ultraviolet and visible light (UV–Vis), photoluminescence (PL), and inductively coupled plasma optical emission spectrometry (ICP-OES) measurements, which further confirmed its superior performance.
期刊介绍:
Publishes high quality research and technical papers in all areas of ceramic and related materials
Spans the broad and growing fields of ceramic technology, material science and bioceramics
Chronicles new advances in ceramic materials, manufacturing processes and applications
Journal of the Australian Ceramic Society since 1965
Professional language editing service is available through our affiliates Nature Research Editing Service and American Journal Experts at the author''s cost and does not guarantee that the manuscript will be reviewed or accepted